u i ’4 ‘ <' V (x J; ‘5"? ‘k‘ ; _, 'A~3"u'-:Z-- 3. $4.3 \ 5 ,3; _ “Fm-3:”. x7.“ nun \— iu ' a s-;. ~ .H ; A 49);.“ fl; .1 ‘l v c I "4 ”353:3." '2‘. I .. T . 4!... 143‘ $3.3 43:- “ ' "’11:; m,‘ a . r; .. r ? unfit“ n!‘"',’; "‘.'...;1‘.’. n - - a - -34” mm“- ,«r— v- f “O'JN’:‘:_‘ v4 .‘u—‘ 1 wyfizfizfi’k‘r . . l" '3‘ (L; n" - W V . n- ' an">4"rl. “ -A-.p-z‘v‘;‘/_t' I .m- p " v 5-2:.“ "fl 1 w. 9‘ 4 ”iii L" r. .1; 4 J‘lfia ‘E’ r55 x; r“ IllllllllllllllllllllllllfllWilli 3 1293 01055 9718 This is to certify that the dissertation entitled THE EFFECT OF SPACE CHARGE FORCE (N BEADS EXTRACIED FRa‘d EIIR ICN SOURCES presented by Zu Qi Xie has been accepted towards fulfillment of the requirements for 21; D. degree in Bhysms_' M fr’ WrfiJ— Major profess? Date A119 31’ 1989 MS U is an Affirmative Action/Equal Opportunity Institution 0-12771 “ LEBRARY Michigan State University PLACE IN RETURN BOX to remove We checkout from your record. TO AVOID FINES mum on or before dde due. | DATE DUE DATE DUE DATE DUE l l—__Il l! MSU to An Affirmative ActlorVEquel Opportunity Institution chns-nt THE EFFECT OF SPACE CHARGE FORCE ON BEAMS EXTRACTED FROM ECR ION SOURCES by Zu Qi Xie A DISSERTATION Submitted to Michigan State University in partial fulfillment of the requirements for the degree of DOCTOR OF PHILOSOPHY Department of Physics and Astronomy 1989 \J 7 . ‘ 2 C) '. «f7 "‘ (c 05 ABSTRACT THE EFFECT OF SPACE CHARGE FORCE ON BEAMS EXTRACTED FROM ECR ION SOURCES by Zu Qi Xie A new 3 dimensional ray tracing code BEAM_3D, with a simple model to calculate the space charge force of multiple ion species, is under development and serves as a theoretical tool to study the ECRIS beam formation. Excellent agreement between the BEAM_BD calculations and beam profile and emittance measurements of the total extracted helium 1+ beam from the RTECR ion source was obtained when a low degree of beam neutralization was assumed in the calculations. The experimental evidence indicates that the positive space charge effects dominate the early RTECR ion source beam formation and beamline optics matching process. A review of important beam characteristics is made, including a conceptual model for the space charge beam blow up. Better beam transport through the RTECR beamline analysis magnet has resulted after an extraction geometry modification in which the space charge force was more correctly matched. This work involved the development of an online beam characteristic measuring apparatus which will also be described. ACKNOWLEDGMENTS I wish to thank the staff and faculty of the National Superconducting Cyclotron Laboratory for their support of my education and the completion of this dissertation. First and foremost, I owe my deepest gratitude to my thesis advisor Dr. Timothy Antaya for his guidance, supervision and friendship during the fOur years that I have worked with him, without his help, this thesis would be all blank pages. Second, I would like to specially thank Professor Jerry Nolen, for his guidance in my early graduate career and the freedom he gave me to work on ECR Ion Source to pursue my academic interests. In addition, I wish to thank Dr. Thomas Kuo for his encouragement and the friendship we shared over the past years, and Dr. G. Mank for performing the 6108 calculations used in Chapter 5 of this thesis. Finally I am greatly indebted to my wife Li Su, for her love, patience and encouragement to make it through. I am also very grateful to Michigan State University and the National Science Foundation for the financial support during my graduate study. ii LIST OF LIST OF Chapter 1.1 1.2 1.3 Chapter 2.1 2.2 2.3 Chapter 3.1 3.2 3.3 Chapter 4.1 4.2 4.3 4.4 Chapter 5.1 5.2 TABLE OF CONTENTS TABLES.. ................................................. FIGURES .................................................. 1 - Introduction ......................................... Motivation. ............................................. RTECR Source and Its Beam Analysis System ............... He Beam Technique ....................................... 2 - The BEAM_3D Code ..................................... Motivation .............................................. General Organization .................................... Special Features ........................................ 3 - Emittance Measuring Apparatus ........................ Theoretical Review of Emittance Measurements ............ Online Slit-Wire Scanner ................................ Kapton Camera ........................................... 4 - Extraction Geometry Study ............................ Motivation .............................................. Theoretical Review ...................................... 4.2.1 Equations of Motion ............................... 4.2.2 Effects of Ion Temperature, Magnetic Field and Q/M Ratio on Beam Emittance ......... . ............... 4.2.3 Extraction Electrode Design..... .................. BEAM_3D Predictions on the Extraction Electrode Design.. Results ................................................. 5 - Space Charge Force and Pre-analysis Beam Transport... Space Charge Force ...................................... Beam Transit of the Solenoid Magnet ..................... iii vi 10 13 13 14 22 28 28 4O 42 46 46 50 50 58 64 69 73 77 77 85 5.3 Transit of the Analysis Magnet... ........ . .............. 94 5.4 Matching the 90° Analysis Dipole under the Effect of Space Charge ................ ... ....................... 98 Chapter 6 - Summary and Conclusions .............................. 102 6.1 Extrapolation to Multiply-Charged Ion Beams ............. 102 6.2 Summary and Conclusions ................................. 103 Appendix - Introduction to ECRIS ................................. 107 [1.1 'Unit' ECR Cell.. ....................................... 107 A.2 ECR Operating Characteristics ........................... 114 LIST OF REFERENCES ............................................... 125 iv LIST OF TABLES TABLE PAGE 1.1 RTECR source DC performance for gaseous feed materials.... 6 1.2 RTECR source DC performance for solid feed materials ...... 7 5.1 Beam envelope at the 90° dipole entrance.... .............. 100 LIST OF FIGURES FIGURE 1.1 A schematic diagram showing the main features of the RTECR ion source..... ..... . ..................... ...... ........... 1.2 A schematic view of the RTECR analysis system and the beam analysis systems built for the studies presented in this thesis ................................................ 1.3 A helium spectrum is shown here. 300 euA helium 1+ was produced by the RTECR source at Vex = 10 kV, Vp = 0 and 80 watts of RF power, while less than 51 helium 2+ was produced ............... . ................................... 2.1 Flow diagram of the BEAM_3D code.... ........ . .............. 2.2 This figure shows the grid points involved in the interpolation of field components of an intermediate point P(r,z) .......... ..... ............ ....... ..... .. ............ 2.3 The geometry used in the calculation of the space charge force ........................................... . .......... 2.4 A schematic view of the extraction geometry and the initial beam transport line of the RTECR source fer BEAM_3D calculation ......................... . ...... . ....... 2.5 The axial and transverse ion orbits of He1+ and Re?‘+ calculated by the BEAM_3D code ............................. The initial and final ion position distributions...... ..... The initial and final charge state distributions (CSD) ..... 2.8 The emittance fittings. A. At the beam defining slit. B. At the entrance of the 90° dipole ...................... 3.1 Schematic cross section of a beam .......................... 3.2 The phase area of a beam with rotational symmetry is described by an ellipse ............................. . ...... 3.3 The particles which lie in the shaded area of the shown ellipse (z = 0) will evolve to either of the cases in B (2 = l) or C (2 = L) after a drift distance .............. vi PAGE 12 15 18 2O 23 24 25 26 27 29 31 33 A comparison, fer the case Figure 3.33 with drift distance 100 mm, of the line current density and the calculated current profile if measured with a wire of 0.3 mm wide. The particles are in the area determine by x, = 9 mm and x2 = 11 mm for an ellipse with a 45° orientation, a = 5 mm andb=20 mrad, atz:0 0000000000 ......OOOOOOOOO ......... A comparison, fer the case Figure 3.3C with a drift distance 500 mm, of the line current density and the calculated current profile if measured with a wire of 0.3 mm wide. The rest conditions are the same with the case in Figure 3.4.. ..... ............... ....... ..... ....... The assembly of the wire scanner .......... . ................ 10+ A 3 euA Ar beam profile after the analysis magnet is shown. The large tail is believed due to the high divergence beam component. An ellipse fit at 901 intensity gives emittance e = 245 mm mrad ....... . .......... The assembly of the 'Kapton camera' ............ ... ......... A. A schematic view of a three electrode extraction system. B. Accel-decel voltage distribution. C. Accel- only voltage distribution. D. Accel-accel voltage distribution ............ . .................. .... ............ A schematic view of the two extraction electrode systems utilized in the RTECR. A. The puller has a face angle at 45°. B. The puller has a Pierce spherical face shape [P154] ................. .. ................... ... ............ The extraction region of an ECRIS with an axial magnetic field. Ions are extracted from the source at radius r .... 1 Schematic view of a group of identical ions on a circle travelling along the optical axis.... ...................... The correlation in phase space. Point 1 in the XX' plane corresponds with point i in the YY' plane ....... . .......... The effects of ion temperature on the ideal argon beam emittance as a function of charge-to-mass ratio. Ions are assumed extracted at 10 kV, extraction aperture raz 4 nm and with 82: 0.25 T (approximately the same conditions as fer the RTECR extraction) ......... .... ....... vii 37 38 41 43 45 47 49 53 53 55 61 Argon beam emittances with the ion temperature taken as T1: t0 eV x q. Other conditions are the same as in Figure 4.7 ......................... ..... ................... 62 Emittances of cold argon beams with different extraction voltages and various extraction magnetic fields. The extraction aperture is r3: 4 mm .......... . ................. 63 Plot of the electrode shapes (heavy lines) and the equipotential lines external to a planar space-charge- limited electron beam as determined from Eq. (4.29) [P154]. 66 Electrodes for obtaining axially symmetrical electron flow of uniform diameter [P154] ............... ....... ...... 68 A comparison the axial and electric field strengths of 45° (denoted by "M2a") and a Pierce spherical pullers. In both cases the extraction gap is 3.3 cm and the first electrodes are the same .................................... 70 BEAM_3D calculated beam profiles at a space charge limited current for the extraction system with a 45° angle on the puller electrode face and a Pierce spherical puller. A drum shape in the first gap, and a fOcus in the puller electrode are seen for the 45° puller of Figure 4.2A................ ...................... 71 A comparison of the effective emittance after extraction for the 45° and a Pierce spherical pullers in the RTECR, for a space charge limited He1+ beam of 1.3 emA at D = 3.3 cm, with Vex = 10 kV. BEAM_3D predicts the effective emittance of the 45° puller is about three times that of the Pierce spherical puller .................. 72 Using the He1+ technique, the total extracted current of the RTECR was measured directly at FCl1 as a function of extraction voltage, for 3 operating pressures. At low voltages, the extracted current is space charge limited, fellowing the Child-Langmuir law (marked Theory). At higher voltages the extracted current is seen to saturate.. ................................................. 74 A transmission study on the analysis magnet for different extraction gaps and helium 1+ currents S 0.5 viii 5.2 5.3 5.4 5.5 5.6 emA. A beam extracted at the space charge limit gives the best transmission, with decreasing transmission as the beam intensity falls increasingly below the space charge limit ...................... . ........................ 76 He1+ beam maximum divergence versus the beam edge radius, for different beam intensities, after a waist. The maximum divergence is a constant if the space charge is zero. But as can be seen, if the space charge force is taken into account, then the beam maximum divergence will increase rapidly with the level of the space charge force ...................................................... 81 A comparison of the beam edge radius with axial drift distance for various levels of the space charge. The starting conditions are the same as in Figure 5.1. For high uncompensated space charge, the beam envelope rapidly increases with axial drift ........ . ................ 82 A schematic view of the evolution of the emittance envelope after a waist with and without space charge ferce. The emittance is the same for both cases, but with space charge the maximum divergence and beam size significantly increase .............. ............ ........... 84 A comparison of the divergence versus beam intensity for space charge limited extraction using the BEAM_3D code. Even though a parallel beam profile at the first gap is ensured, the effect of space charge, which increases the divergence, is clearly seen .......... ... ..... . ............. 86 The effective emittance of He1+ after crossing the focussing solenoid for various beam intensities . In each case the extraction is space charge limited, the beam energy is of 10 keV, and the emittance after extraction is 69 mm mrad. The 1.0 emA case shows very large emittance growth due to its large beam profile in the solenoid, thus the aberrations have become very severe.. ..... ....... ................... ............. ....... 89 A and B are Kapton foil burns at the divergence box with He1+ beams of 65 and 550 euA respectively. The beam ix 5.7 5.8 5.9 5. 11 passes through a defining slit plate 8 cm upstream of the foil, giving horizontal marks on the foil. BEAM_3D predicts for 65 euA He1+ with a space charge limited extraction (vex = 10 kV, Vp = 8.5 kV), beam profile at the divergence box will be 1.6" and that is experimentally seen. A 550 euA He1+ extracted at space charge limit fills the Kapton foil at the divergence box, also agreeing fairly well with a BEAM_3D calculated profile of 3" ............... .. ..................... ........... ..... 1+ beam in The measured emittance for the 65 euA He Figure 5.6A is e = 69 mm mrad, which agrees very well with the BEAM_3D calculation (see Figure 5.5), in which the ion thermal energy was taken to be zero................ A 65 euA He1+ beam extracted (Vex = 10 kV, Vp = 0) well below the space charge limited (Vex = 10 kV, Vp = 8.5 kV) current results in high divergence and large beam profile. For this case, BEAM_3D predicts a diameter of 5.5" at the divergence box... ............................... . ....... ... BEAM_3D predicts that a 200 euA He1+ extracted at 7, 10, 15 and 20 kV with an extraction gap of 3.3 cm will have very high divergence and large beam profile at the divergence box, because the extraction is far below the space charge limit. Measurements, limited by the measuring apparatus to a maximum divergence 65 mrad, show that the actual divergence is higher, in fair agreement with the calculations ........... ...... ..................... A triangular beam mark is seen on the face of the collimator of FCl2 assembly for the CPECR. The cause of this triangle shape is believed to be the space charge effect on the beam divergence before the magnet entrance, resulting in filling the magnet aperture and causing 2nd order aberrations .............................. A 0105 beam transport calculation for the case in Figure 5.10. The transit of the analysis magnet with an unneutralized 1.0 emA helium 1+ beam of starting emittance 200 mm mrad will result in a triangular shaped 90 91 92 93 96 beam after analysis........ ...... ................. ......... 97 A schematic illustration of better matching of the 90° dipole for beams with space charge compared to the case of no space charge ........................ . ........ . ....... 99 A 330 euA He1+ is extracted with space charge limit and transported through the 90° dipole, this beam has a waist at the dipole object when the focussing solenoid is excited with 81 A. However the optimized transmission occurs at I(sole) = 78 A, for which the beam waist is about 10 cm closer to the dipole... .......... 101 BEAM_3D code predicts that after crossing the fOcussing solenoid the effective emittance of Ar8+ (S shaped, due to the solenoid spherical aberrations) is doubled compared to its effective emittance before the solenoid. The CSD and focussing solenoid excitation are based on actual operating values...............§ .................... 104 A 'Unit' ECR Cell consists of a vacuum vessel, microwave generator, a minimum-B field and an extraction system ...... 108 A typical axial magnetic field profile produced by a set of solenoid coils fOr a single stage ECRIS ...... . .......... 109 This figure shows the strength of a hexapole as a function of radius along one of the poles and in a gap ..... 111 A "minimum-B field" topology as a result of the superposition of a hexapole and a set of solenoid fields... 112 Single ionization potentials of some atoms and ions ........ 115 Performance comparison between 2-stage and second stage only RTECR operation for the production of nitrogen ions. Helium is used as a support gas. Each next higher charge state shows a large percentage increase in current with the first stage on ......................................... 116 Ionization rate coefficients S for single ionization of argon atoms and ions from the ground state by electron- impact in plasma (Maxwellian distribution, no collision limit) ......................... ..... ....................... 119 A high temperature oven for producing metal vapor is equipped with the CPECR Ion Source at NSCL/MSU ............. 122 xi A.9 The direct dependence of gas mixing effects on mass is seen in the mixing of lighter gases with argon.. ........... 123 xii 1 Chapter 1 Introduction 1.1 Motivation The ECRIS (Electron Cyclotron Resonance Ion Source, an introduction to the ECRIS is presented in the Appendix), is now the most frequently used new ion source for producing high charge state positive ions for accelerators and for atomic physics research. ECRIS originated from plasma fusion developments in the late 1960's and early 1970's. Observations were made as early as 1969 in during the use of ECRH (Electron Cyclotron Resonance Heating) in plasma devices to produce high charge state ions [Ge70,Po70], and the early extracted beams from these devices were reported in 1972 [8172,Wo72]. Following the pioneering work of R. Geller and his coworkers at Centre D'etudes Nucleaires de Grenoble, France, where the ECRIS originated, there are now about 40 ECRIS in operation or under construction around the world. The coupling of ECRIS to cyclotrons has resulted in significant performance gains in energy, intensity, reliability and in the variety of ion species available. At least five ECRIS have been dedicated for atomic physics research, and at many facilities atomic physics programs share ECRIS with nuclear science programs. Although ECRIS have wide application, it is still a relatively young technology. The dynamical processes are still not understood in detail. Important unknowns include the detailed mechanism of microwave coupling for electron heating, the nature of ion heating in the plasma and the effect on ion confinement, the systematics of the 2 gas mixing effect [Dr85, Ma86a, An88], and the relationships between the emittance of the beams extracted from the ECRIS and the magnetic field, charge state, ion mass, ion thermal energy, space charge force and electron neutralization and so on. Further development of ECRIS will require greater understanding of these and other important issues. For ECRIS coupled to accelerators, the last area mentioned above, the beam formation process, is critical to the design and operation of the accelerator coupling line. Most ECRIS have been built for multiply-charged positive ion injection into accelerators. The sources and injection lines generally must operate over a broad range of charges and intensities; the injection rigidity is generally set by accelerator characteristics. The pressure in the coupling line between ECRIS and accelerator is low because the ECRIS main stage pressure is low, in the range of 10'7 T, and it is desirable to avoid the beamline constitute a source of gas for the main stage operation. IT“: specifications for the beam transport elements are generally obtained by assuming (or extrapolating from existing data) a starting emittance at the source extraction aperture, and tracking that emittance with transport optics codes up to a match condition near the accelerator. Generally beams are extracted DC from ECRIS. If the charge unthin an ion beam is not neutralized, then the charge density in space is not zero. The consequence of this nonzero charge density is that it creates an electric field within the extracted beam. For a DC ion beam with rotational symmetry, this force is predominantly outward and it will cause the beam to expand in diameter and continuously change the beam divergence due to the repulsion effects. Such space 3 charge effect can severely alter the beam optics if the space charge force is very strong. Due to the lack of detailed knowledge of ECRIS beam formation, the space charge effects have heretofore never been seriously addressed. Thus the space charge effects on the ECR beam transport optics have been either ignored or assumed to be non- important, though space charge effects are often studied during the design of the ion source extraction electrodes themselves. A systematic investigation of the characteristics of the ion beams extracted from ECRIS is a complex study involving many parameters, most of which are without detailed knowledge as mentioned previously. Though the importance of studying the ECR ion beam formation has been realized by many ECR workers, up to now, only a limited number of emittance measurements of ECR ion beams with very little systematics [3386, C187, Dr83, Dr85, 0e79, Ma83a, Ma83b, M386b, Kr86, Tu80, 9086, An88] have been reported since the first high charge state ion beams were extracted from ECRIS in 1972. None of these measurements has clearly revealed the characteristics of the ECR beams, partly because of the lack of systematics, and partly because good emittance measurements are difficult to make. In an effort to understand better the requirements for matching ECRIS beams to the superconducting cyclotrons at NSCL, we have undertaken an analysis of the beam formation process on the RTECR [An86a], including the interaction of the initial beams with the first element of the beam transport system. We have found excellent agreement between BEAM_3D calculations (presented in Chapter 2) and helium beam profile and emittance measurements as a function of the total extracted beam from the RTECR, when a low degree of beam u neutralization is assumed in the calculations, as will be presented in Chapter 5. Space charge effects dominate the early beam formation and beamline optics matching process. Initial emittance measurements on analyzed helium and multiply charged argon beams indicated rather large divergences [An88], and often triangular shaped beams in real space. To understand these measurements, we shifted to measurements on the total extracted beam before analysis, where we could make direct comparisons with the BEAM_3D code under development at NSCL. 1.2 RTECR Source and Its Beam Analysis System The RTECR source, shown in Figure 1.1, is built for multiply- charged ion production and injection into the superconducting cyclotrons at NSCL. The solenoid coils provide the plasma axial confinement while the hexapole magnet provides the transverse plasma confinement. Microwaves can be simultaneously launched.hfix>both stages or the main stage (second stage) only. A high density lowly ionized plasma, produced in the first stage, diffuses to the main stage where highly charged ions are produced at lower pressure. The plasma chamber is positively biased with 5 - 17 kV (depending on the beam requirements), and ions leaking out of the bottom magnetic mirror are formed into a beam by the extraction electrodes located at the bottom of the source. The performance of RTECR is summarized in Table 1.1 and Table 1.2. The beam analysis system for the RTECR is shown in Figure 1.2. The first acceleration gap was designed to be adjustable over the MICROWAVE HIGH 2ND STAGE VOLTAGE JOINT (2) WAVE GUIDE GAS FEED VACUUM PUMP OUARTZ VACUUM W'NDOW IST STAGE CHAMBER INJECTION POSITION VACUUM 80X ADJUST/ALIGN PLASMA MECHANISM CHAMBER CIRCULAR COIL SAMARIUM/ COBALT HEXAPOLE YOKE MACNET RADIAL PLASMA POLE CHAMBER PORTS . IMLZS (REFJ PIERCE-TYPE EXTRACTION \\ _PUMPING ELECTRODE PORT EXTRACTION p A MA PUMP BOX CHAMBER INSULATOR /—EXTRACTION aggr- am... PUMP ADJUST/ALICN " I MECHANISM Figure 1.1. A schematic diagram showing the main features of the RTECR ion source. Table 1.1 RTECR source DC perfbrmance for gaseous feed materials ‘ZC ‘“N “0 2°Ne “°Ar “‘Kr '=°Xe ‘271 q 4 25 5 100. 87. 67 19 5 5 6 68. 61 50 5 * 6 * 25.5 52. 41.1 42. 7 * 12.2 16.5 55. 8 * 5.0 94. 9 1.0 44. 10 * * 23 11 7.6 * 12 2.0 23.3 2.3 13 .33 29.0 2.5 1.7 14 15 29.0 2.7 2.3 15 23.2 2.9 3.0 16 * 3.1 * 17 6.8 3.0 2.7 18 3.2 2.7 * 19 1.4 2.3 2.5 20 0.4 1.4 2.3 21 0.8 2 1 22 .45 1 8 23 .20 1 0 24 11 * 25 .035 Conditions: 10 kV extraction voltage; 8 mm extraction aperture; All currents in unit euA. * Mixed Q/M. 7 Table 1.2 RTECR source chperfOrmance for solid feed materials 7Li ‘9F 2“Mg 2°81 5‘V ‘°‘Ta Q 1 14.5 5.0 4.5 2.5 2 14.5 5.0 8.4 1.0 6.1 3 1.5 8.0 11.3 0.6 7.8 4 14.0 13.5 1.7 8.7 5 12.0 16. 2.1 11.7 6 * 3.0 12 6 7 0 7 * 15 2 8 0.6 13 5 9 0.2 6 5 0.4 10 0 I 11 1.7 0.5 12 1.0 13 * 14 1 6 15 * 16 3.1 17 3.6 18 3.6 19 3.1 20 2.7 21 2.0 2A 0.6 27 0.11 29 0.08 Conditions: 10 kV extraction voltage; 8 mm extraction aperture; All currents in unit euA. * Mixed Q/M. 8 range of 0 - 3.3 cm. The source extraction aperture is placed at the object of a solenoid focussing lens which focuses it, with unit magnification, to the object of the 90° dipole magnet at Faraday Cup #1. The solenoid focal length was chosen to put the ion source on the main floor level and to allow Ar1+ ions to be focussed at a source bias of 10 W. The double focussing dipole images the beam with unit magnification at Faraday Cup #2. The beam pipe and solenoid I.D.'s are 15 cm, while the dipole aperture is 10 cm. An emittance of i 5 an x t 40 mm mrad at the source extraction aperture was assumed in the design of the analysis system. Space charge effects were ignored in these design calculations. The acceptance of the dipole can be limited by changing adjustable object, divergence and image defining slits. Emittance measurements are possible on both the object and image sides of the 90° dipole. In a vacuum box at a position of large beam size before the 90° entrance, emittance measurements are made by imaging a defining slit pattern on Kapton film, which darkens on exposure to the beam, making an image with well defined edges. In the FC#2 box, we can make emittance measurements in either transverse plane with an on-line wire scanner, or with Kapton film exposures or both. These measurement techniques are discussed in Chapter 3. The two methods are complementary. The wire scanner method allows quick determination of the emittance for a variety of tuning conditions but obscures the coherent emittance, while the Kapton film method shows coherent effects such as relative beam motions and multiple beams. The initial performance of this analysis system, as described above, is as follows. With a total extracted current of 0.5 - 1.5 emA at 10 W (with various source geometries and tuning conditions), the It. 05...... 9* DIVERGENCE )L” 30" I 1 III 1 I I RT-ECR q—'i—'K\Im=mau can Hmfixm one .m.m mazmum +N .1. A 00 v N . . . 00.0000 00.000“ 00.000N 00.005. 00.00.: 00.00: 00.0mm 00 0mm on cam mm 31.. . . um.\\\ 38 32.28 \ / .. pomnno oaocoaom Nm fl moazom n 00.0. 00.00 00.00 00.0— A “.a 0010—. 00.00. 00.00.. 00.uuq..l I“ TIIIII . . . . I 1 14 u . o m In) . um .w rt ,. e u . 9 TUA I. r w 0 9 . I 0 .un - 7“ I 1 I w e n O In fi" . .o . .u 0 m can: enema—8.5. ...». ea msaeeo :oH mmcoapomam cannon .mcoasseaesmae cougamoa cos Anzac use Hessaen one .o.~ oeamaa 25 ee . - 8.2 a 8.. 8x2- 8...- ...... 8d.-. 8 a 2.. 3- 2. no 7 3 u . 1 n . a u 1 . JI 1 a . 4 a .I z ' .- e . .x x .... x x xx x x . x a A A .. : as. e x x x l x x u ..u. x x x xx Xx xx x xx a x x u... x 5. x v. xx xx u x x x x x in x x x x x . ax ‘X X X 132' . 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I 3.2. . 8.... n, 88 I 8.2. . 8b. n 00.8 00.... 0 III» a... 00.0. o 18> to... :6 u ...: .w 10.8 3.: .. .5» r. 805.30! . 800.003 .” .... a... .. ...... u 8 2... .. ...: u 8 8. . 2 8 8. . 2 o... . ex 1 8. . on T» 8.88 . u .o 8..8. . u .o u u c . .... .... u- u u .m . «m u .... h u u m a < .n u u h flu u u 0 r A IN“) 28 Chapter 3 Emittance Measuring Apparatus 3.1 Theoretical Review of Emittance Measurements At each point of any transverse section of the beam, in a region free of accelerating fields, we have an ensemble of rectilinear trajectories that form a cone of angular aperture 2da, as shown in Figure 3.1. The slope of each ray can be simply expressed as a function of the transverse momentum px and of the longitudinal momentum p2 of the particle by the relation x' = px/pz (3.1) The x-x' phase-diagram of the beam is a plot of the range of values of x' as a fUnction of x, at constant 2 and integrate over all y values. The area of this diagram A(x,x'), gives us a measure of the transverse emittance e, e = A(x,x')/n (3.2) where we have followed the definition of Septier [Se67]. For a beam with no losses in a drift space without an external accelerating field, say V(z) = constant, this emittance is an invariant of motion (Liouville's theorem [Be67]). As mentioned in the previous chapter, ECRIS produce multiple ion species and these ion species are extracted out of the source 29 Figure 3.1. Schematic cross section of a beam. 3O simultaneously. However, we generally are interested in the emittance of an ion beam of single species within this ensemble. We will use the term "beam" to refer to a beam of a single ion species unless otherwise specified in the text. The emittance of a beam with rotational symmetry in the phase plane is described by an ellipse, as shown in Figure 3.2, and this ellipse is described by the following equation, in generalized x-x' transverse coordinates (Ax'-Bx)2 (Ax+Bx')2: a + b 1 (3.3) where A : cose, B = sine and a and b are the minor and major axes of the ellipse as shown in Figure 3.2. Let D(X) denote the distance between two points (1,2) on the ellipse with the same x coordinate D(X) = X'(1) - X'(2) (3.“) Solving Eq. (3.3) yields 1 A2b2+ 82 2 2 2 2 - x 2 [AB(b2- 32)x + ab(A2b + B a 1/2 a X'(1) ) ] (3.5) 1 [AB(b2- a2)x - ab(A2b2+ Bzaz- x2 1/2 2 2 2 2 A b + B a X'(2) ) ] (3.6) thus D(x) is given by 2ab A2b2+ 8282 D(x) = (A2b2+ Beaz- x2)1/2 (3.7) 31 Figure 3.2. The phase area of a beam with rotational symmetry is described by an ellipse. 32 Eq. (3.7) indicates that D(x) is an even function of x and reaches its maximum at x = O. The importance of D(x) is that it can be related directly to measurable parameters. In order to measure the emittance, one generally intercepts a beam with narrow slits (to set x i = 1, 2, 1: .), followed by a scanning system, to measure the beam divergences (to measure x'(i)). Therefore we first consider what happens when a beam is intercepted by a slit. For a beam with uniform density 0 in the phase ellipse as shown in Figure 3.3A (assume at z = O), and the beam divergences are constants of the motion, then if one traces the particles that go through a slit (shaded area determined by 4 points (1,2,3,N) as shown in the ellipse), to a distance of l or L , one will find these particles evolve to an area still determined by those 14 points (1,2,3,u) as shown in Figures 3.38 and 3.3C. And the particle's coordinates in X-X' have the relationships to the coordinates x-x' at z = O .. ' ' Xi - xi + 1X (1) X'(i) = X'(i) ' (3.8) The detailed expression of D(X) for the two cases of Figure 3.38 and 3.3C will be derived below. For Figure 3.38, the ‘4 points (1,2,3,14) in the X-X' coordinates are given by X I - x, + lx'(1) X'(1) = x'(1) X N N x, + lx'(2) X'(2) X'(2) 33 .oocmumfiu phase a Locum A4 u my NV m cm momma on» no Losuao op o>~o>o Ha“: Ao u my omafiaao :zozm on» mo mono noomsm on» c“ oHH sown: moaofiusma och .m.m ossmfim 0.5:... ._nN wuN N Mari; .M-Eii N :3” an; 34 X3 = x2 + IX'(3) X'(3) = X'(3) X. = x2 + lx'(u) X'(u) : x'(h) (3.9) Graphically one can see that - X'(J) - x'<2> _ x'(1) - x'gz) _.1 Tan¢ ' X- - X. ‘ ltx'(1) - x'(2)1 ‘ 1 (3'10) then the divergence of particle p on the line 1-2 would be x. - x, X'(p) = x'(2) + (x1- X.)Tan¢- = x'(i) + -l—I——— (3.11) Thus the vertical distance between point p and point i is given by x. - x1 - _ - -._L____. < < D(X)p_i- X'(D) X'(l) - l Xz-Xi-X- (3.12) likewise, the distance between X'(j) and X'(q) is x2 - x D(X)J_q= "'_I__l x.sxjsx, (3.13) In the interval between X. and X,, the vertical distance between points n and k is determined by X,SX SX. (3.14) k Although x, and x2 are known, the other xi between region [x,, x,] are not. In order to have a distribution of D(X) in the X-X' coordinates, 35 D(X) should be expressed as the function of X. Let a : A2b2 + Beaz, B = ABl(b2 - a2) and Y = abl, we use the relation X'l + X : X (3.15) to obtain the following equations, _ .1. 1 2 D(X)p_l— 1{Y2 + (a + B)2[a(a + B)X + Y(a(Y (a + 3)2) - a2x2)‘/21 - x,} xzsxsx- (3.16) 1a2x2 1/2 D(X)n_k: 1[Y2 + (a + B)2][(a(Y2 + (a + B)2 ) - X] x,sxsx. (3.17) - l. -1 _ 2 D(X)J_q- l{Y2 + (a + B)2[a(a + B)X Y(a(Y (a + 3)2) - a2X2)1/2] + x2} x.sxsx. (3.18) Similar analysis gives the D(X) distribution for the case of Figure 3.3C D(X)p_i:-% 2 + Ea + B)2[a(a + B)X + Y(a(Y2 (a + 3) 2) - 02X2)1/2] - x,} xzsxsx. (3.19) D(X)n_k= Ez—E—il =-—§— x.sxsx1 (3.20) D(X)J_ _q- {(2 +‘2a + 3)2[a(a + B)X - Y(a(Y2 36 (a + B)2) - a2x2)‘/21 + x2] x,sxsx, (3.21) where<1==A2b2+ B2a2, B = ABL(b2- a2), Y = abL, and s is the slit width. Based on the assumption that the particle density 0 is a constant, then the product of D(X) and 0 gives the line current density along the X direction by A(X) : D(X)o (3.22) and in arbitrary units l'(X) = )((X)/o = D(X) (3.23) Hence D(X) is simply a line current density function. If one uses a finite width wire to scan the current after a slit and put the current intensity on the center position of the wire, one would however see a (rifferent current profile than the profile given by this line current density function D(X), because of the wire width effect. Comparison of the D(X) and a wire scanner current profile, if continuously measured by a finite wire of diameter ¢ = 0.3 mm, are given 111I?igure 3.1% for the case of Figure 3.3B, and in Figure 3.5 for the case of Figure 3.3C. One can see that due to the finite size of the wire, the locations of X,, X2, X3 and X. are wiped out by small curvatures. But X2 and X3 can be determined from the locations where the bean1am ssamcosca goo um use mundane as soon coco??? :3: on» 0... one 3533 3 3m... omen: o5. m“ nocmme mammamcm on» Locum mammona amen .umes .ucocoasoo .czosm as sea m e .e.m oesmse O¢1 62.5 o x \ +op 2.5 x cm Om ON 0. O 0..- ON1 Om.- . q _ . _ _ .- no..E.EE mvNuw m. H .1 AXVAVmwnuHH 1 1 050 "Odin. -. nu >x 0. +0. 5 O? 0.0 A“ imais Kapton camera is mounted on an 8" del-seal blank flange as shown in Figure 3.8. An aluminum frame centered on the beamline axis holds the two Kapton spools. Two indexing vacuum feedthroughs control the revolution of the spool, with two revolutions to advance (nus foil exposure. The burning time depends empirically on the beam intensity. For example, for a 10 euA/cm2 beam intensity, the burning time is approximately about 10 minutes. A well defined beam image on the foil can be obtained. At beam intensities in the range of 100 euA/cm2 or higher, ion charging effects on the Kapton foil start to blur the image. At these current densities, we image the beam onto the metallic side of aluminized Kapton foil and obtain well defined images on the Kapton side. The emittance of the beam can be obtained by using a 5 to 10X magnifying lens to read out the beamlet edges, giving x'(2) and x'(3) sets for each (x,, x,) pair which can be used to build the phase space diagram. Results of such measurements are presented in Chapter 5. 45 'Ihe assanbly of the 'Kapton camera' . Figure 3.8. N6 Chapter 11 Extraction Geometry Study “.1 Motivation The ion beam extraction system is usually located near the peak field of the end mirror. The most common extraction system that has been used to form beams of ions from ECRIS is shown schematically in Figure H.1A. It is a three electrode system with applied voltages Va, Vb and Vc on the relevant electrodes respectively. Positive ions are expelled from the source and the beam transport line is at ground potential, which results in the requirements that V0: 0 and Va) 0. The intermediate electrode with voltage Vb is used to obtain adequate ion focussing. The beam energy is determined by 113- V0: V3, which is set by the application, while the voltage difference Va- Vb and the spacing D between these two electrodes determine the maximum current that can be extracted from the source for a given plasma. The variation of the voltage V from negative to positive will enable the b extraction system to be one of the 3 cases: 1. accel-decel (Vb< O), as illustrated in Figure 4.13, the region between Va and Vb is accelerating and radially focussing while the region between V and V0 b is with decelerating and defocussing, though the net effect of the extraction system is focussing if the focussing strength in the acceleration gap is stronger than the defocussing strength, 2. accel- only (Vb: V0: 0, electrode b and 0 can be combined as one), as shown in Figure 11.1C, which produces only a focussing effect in the region between Va and Vb, 3. accel-accel (Va>V > O), as shown in Figure H.1D, b M7 mfg-1°11) ; / HH 7 Vo>° Vb<0 V630 B X Vbj>0 Vb=V°=() C Va))Vb>() Vc=0 D Figure “.1. A. A schematic view of a three electrode extraction system. B. Accel-decel voltage distribution. C. Accel-only voltage distribution. D. Accel-accel voltage distribution. A8 with focussing strength in both gaps. For historical reasons, only cases 1. and 2. have been used in ECRIS [J083, 0183, 6e79, An86, Pa87]. Such accel-decel systems used in ECRIS generally have a Pierce-type [PiSA] first electrode and various second electrode shapes (puller electrode), while the third electrode is simply a large bore ground ring. Figure A.2A shows a schematic view of the original RTECR extraction electrode system which has a puller of a face angle ”5° tn) the optics axis, and the first gap was adjustable from O to 3.3 cm by moving the puller (the second gap is fixed and moves with the puller). Shown in Figure 11.23 is the current extraction system, which has a Pierce spherical puller, and the first gap can be adjusted from 3 to 6 (an. A negative high voltage power supply feeds the puller electrode, thus the source has the ability to extract ion beams under the conditions of accel-decel or accel-only. Although ECRIS have been under development for about 12 years, the best extraction geometry for all ECRIS or whether the best extraction geometry has a source dependence is still an open question. During the first operation of the RTECR, we have found the transmission from FC#1 to FC#2 to be low, as mentioned in Chapter 1 -- only about 110% to 115%, implying a large mismatch between the source and beam transport system. Thus an extraction geometry study on the RTECR source has been undertaken in order to ascertain the nature of this poor transmission. “9 End Plcie Puller Ground Ring £37.55. ‘455‘ . End PIOTB Pierce Puller Ground Ring 1 _Z_ Figure “.2. A schematic view of the two extraction electrode systems utilized in the RTECR. A. The puller has a face angle at “5°. B. The puller has a Pierce spherical face shape [Pi5H]. 50 “.2 Theoretical Review A.2.1 Equations of Motion For a magnetic field produced by solenoid coils, Ae(r,z) is the only nonzero component of the vector potential A. Then a charged particle of charge Q and mass M moving non-relativistically in a combinatnn1cfi‘an azimuthally symmetric electric field and a solenoidal magnetic field, the Hamiltonian (in cylindrical coordinates) is of the form 2 P 2QP 1 2 9 2 2 2 9 .- a—w + .2 ..Z.Q-9-_,._-e,.Q--.,.- <11). where Pr: pr: Mvr, P9: pe+ QrA9= Mver + QrA9 and P2: p2: Mvz are the generalized momenta in which pr, p9 and p2 stand for the mechanical momenta, and vr, v9 and v2 are the linear velocities in the r, O and 2 directions. V(r,z) is the electric potential. Lacking the exact knowledge of space charge, for simplicity, it is assumed that the space charge has only the radial component for DC beams, then V(r,z) = Vex(r,z) + Vsp(r), where Vex(r,z) is due to the applied extraction potential and Vsp(r) is the potential due to the space charge based on the above assumption. Therefore the Hamiltonian becomes P 20? 2 e 2 + 021: _ O 2 + Pz r A9) + r Q(Vex(r,z) + Vsp(r)) (4.2) 51 The equations of motion are then obtained by differentiating Eq. (4.2) with respect to the corresponding coordinates 2 f3:_§.}i=_l[_:.e.+Q2A 3:9._Qp(_.A£+lEE_9.)] r 3r M r3 9 3r 9 r2 r 3r 3V Q(Eexr+ Espr) where Er' - 3r . (4.3) F - - Qfl - O that is P - + QrA - constant (4 4) 9‘ ae ‘ ' 9' pa 9‘ ° ' . __3fl ‘1-(Q2A Egg .Q_P_a_A§)+QE z' 32 M B 32 r z exz Qp 3A -—r_9-§z2+QEexz (“5’ Eq. (4.4) shows that P6 is a constant of motion. (ha important consequence of this result is that if an ion moves from a region with the above mentioned magnetic field to a magnetic field free region, the magnetic angular momentum QrAe will be converted into the mechanical angular momentum P91: 991* QriAOi ‘ Per: per (Aer: 0) (”'6’ where the subscripts i and f stand for the initial and final regions. . In ECRIS the extraction apertures have azimuthal symmetry, with an ion being extracted at a radius ri with respect to the optical axis, as shown in Figure 4.3. Such an ion has the generalized angular momentum Pei: pei+ QriAei (4.7) 52 The other important consequence of Eq. (4.4) is that since the magnetic field contributes to the final transverse momentum, it also then contributes to the emittance, as we will now demonstrate. Imagine that we have a group of ions with the same mass M and charge Q, being extracted at the same initial radius r11: 0 and having the same initial generalized angular and radial momenta P and P Bi ri’ distributed on a circle of radius ri, and that there are no collisions among ions during transit. If we trace all these ions from the extraction aperture to a region of zero magnetic field, as is schematically shown in Figure 4.4, we will see all these ions distributed over a circle of radius rf. and having the same mechanical angular and radial momenta. The phase diagrams enclosed by these ions can be given by projecting the radial and the angular velocities and positions of these ions in the cylindrical coordinates into the X-X' and the Y-Y' Cartesian phase planes. For a convenient derivation, Vrf and ”er are assumed to be positive, and from the following analysis one will see the directions of Vrf and "91‘ do not then contribute to the phase space area. The relations between Vrf’ “er and vx, vy are given below vx= vrfcoso - VOfSin¢ (4.8) vy: vrfsino + vefcos¢ (4.9) 2 2 vx + v = vrf + v9f (4.10) 53 U/Exirqcflon Aperiure Figure 4.3. The extraction region of an ECRIS with an axial magnetic field. Ions are extracted from the source at radius r1. Figure 4.4. Schematic view of a group identical ions on a circle travel along the optics axis. 54 It is obvious that v = 0 when v = (v2 + v2 )1/2 at a position X = y xmax rf Of rfcosox, while ox is determined by v 1) = - tan-Wig) (4.11) x v rf Similarly v = 0 when v = (v2 + v2 )1/2 at Y = r sin¢ and (b is x ymax rf Of f y’ y given by v <1 = tan"(——"f) (11.12) 3’ Var As Figure 4.5 shows, ion 1 (coincident with X-axis) gives xmax: rf. in ”91‘ the X-X' plane and Yintho) = 7— in the Y-Y' plane. Ion 2 z (coincident with Y-axis) gives ymax: rf in the Y-Y' plane and ”er Xint(X:O) = - v_— in the X-X' plane. Ion 3, at a point where the 2 contributions of Vrf and VOf to vy cancel each other, that is, where vx (or x' = x' ax) is maximum at this point. Similarly ion 4 gives I - U - Vymax (Y - Y max)' The total projection of all v”, and v62 (2 - 1,2 ...) to the X-X' and Y-Y' planes constructs an ellipse in the respective phase planes. Noting that xint and Yint are dual value 1 .. 1 .. > functions of X or Y, namely xint - 1 C1 and Yint - 1 C2 (C1 - O and C2 1 _ 1 - Z O ), xint - C1 and Yint - C2 are used to determine the areas enclosed by these ellipses. The areas due to such ellipses in these two planes are then determined as 55 1? v,0 V, V! 2 V, 4 ¢y V. V. 1°. 1 ' * x V5 V \1 1’. 3 . XI y’ p---_._....-- \. 5 it 1 Figure 4.5. The correlation in phase space. Point 1 in the XX' plane corresponds with point i in the XY' plane. 56 Mv p 9f 9f _ I - - — AXX" “xmaxxint' 1nflf'Mvz I ' 1'lpz I (“'13) Mv p 9f 9f _ I _ _ .. .— AYY" “ymainnt’ “rflez ' ' 1'lpz I (”'1”) We then have the following expressions for the beam emittance due to such group of ions on a circle per EX)“: EYY': le—l ((4.15) . per Here we see that the Sign of B_— does not affect the phase space 2 areas. EXX'= eyy, is the natural result of such azimuthal symmetry of the extraction system. From the above analysis one can further imagine that a beam consists of many such circular layers; ions have the same momentum within a layer and various momentum among layers. Each layer of ions defines an ellipse with a common center in the X-X' and Y-Y' planes. The total phase area in the X-X' or Y-Y' plane is then normally equal to the area enclosed by the largest ellipse. In some cases the emittance could be larger than this when aberrations distort the ellipse orientations. Thus the beam emittance can be expressed as E = {A.}/fl (4.16) 57 where {A1} stands for the total phase area due to all the individual ellipses. If all the remaining ellipses are enclosed by the largest ellipse of A1 then e reaches its minimum max’ E . = A. /R (”.17) And if the largest ellipse of A1 max is defined by the edge-extracted group of ions, then E min: Aedge/fl (“'18) From the above analysis a conclusion could be drawn here; for any charged particle source with azimuthal symmetry in the extraction system (fields, electrodes), if the edge-extracted particles have the largest initial generalized angular momentum, the minimum emittance is given by P9 ed e Emin = |-———JL’( (8-19) p2 In ECRIS, the edge-extracted ions of the same charge do have the largest generalized momentum, because of the rA9 term, so that if ther13.is no lens aberration during the extraction, the beam emittance should be no smaller than that described by Eq. (4.19). Comparison of cold ion BEAM_3D calculations with RTECR emittance measurements do closely follow the emittance given in Eq. (4.19), as will be shown. 58 4.2.2 Effects of Ion Temperature, Magnetic Field and Q/M [htio on Beam Emittance Ion-ion collisions are the fastest process in the plasma and should result in thermalization [He82]. Since the thermalization should not have any direction preference, the ion velocities should be isotropic before extraction, and thus the ion thermal velocity will contmdlnlte to the beam emittance by increasing the mechanical angular and radial momentum. As indicated by Eq. (4.7), in a field free regixn1, the maximum mechanical angular momentum of the edge-extracted ion is of the form p9,. = ramei + QAea) (1.20) where ra is the radius of the extraction aperture and A is the Ga azimuthal vector component at that location. The linear angular velocity v91 is the signature of the ion temperature inside the ECRIS. Then the emittance is | (4.21) The magnitude of the angular velocity is related to the ion 1/2 1/2 temperature Ti by v91: (Ti/M) and pz: (2MQVex) , hence T _ 1 1/2 Q 1/2 Emin' ran—20V“) +11 ) ] (11.22) ( 9a 2MVex 59 Eq. (4.22) shows the contribution of the ion temperature to the beam emittance. If the extraction voltage vex is constant, one can clearly see that: T. 1. if (-é—)1/2>> A9a(_%—)1/2’ the emittance is dominated by the ion temperature Ti and has the value of T E . z 1 1/2 min Pa(§av-) (4.23) ex Thus the higher the ion temperature, the larger beam emittance. The emittance is independent of ion mass M but varies with 0'1/2. If T1 = t0 eV x q, here tc is constant, then all ion beams will have the same emittance to 1/2 Eminz ra(2v ) = constant (4.24) ex Ti 1/2 0 1/2 2. if (_6_) << A9a(-fi_) , the emittance is dominated by the magnetic field and the Q/M ratio, and is given by e ( 9a 2MVex min: Pa (4.25) Then the higher magnetic field in the source extraction, the larger the emittance. Also an ion beam with a higher Q/M will have a larger emittance. 60 T Otherwise. if (%)1/2 is comparable to A Q )“2 ea( M , then the ion temperature, magnetic field and Q/M ratio all play important roles in the ECR ion beam emittance, with the emittance is given by Eq. (4.22). The conclusions that increasing magnetic field or increasing ion temperature results in larger emittance still holds, but if the ion temperature and the magnetic field are kept constant, at the case 1/2/A where (MTi) ea= Q, the emittance will reach a minimum of cm. In . - 1/2 1/4 emigin) - ra(2Aea/Vex) (Ti/M) (4.26) Finally if the thermal energy scales with charge (T1 = to eV x q), one would see that 1/2 E + A -—Q-—)1/2] (4.27) ( 9a 2MVex min: ra[(2V:;) Again a stronger magnetic field or the higher Q/M ratio would result in a larger emittance if the other parameters are constant. The dependence of ion temperature, magnetic field and Q/M on the theoretical emittance for ideal argon beams, assuming the emittance is determined by the edge extracted ions and no extraction aberrations, is numerically calculated and shown in Figures 4.6, 4.7 and 4.8. Figure 4.6 shows, if all the argon ion species have the same temperature, one would obtain a minimum emittance for a particular Q/M if all other parameters are held constant. Figure 4.7 shows this effect for argon ions with an ion temperature expressed as a constant 61 Ar Beam Emittance of Ideal Beam 250 ’- I I I I ‘l I I I I l I I I I I f I I I I Ii 3 . Vex = 10 IN I r ra = 4.0 mm '1 2°° _ 132 = 0.25 '1' '1 A j 1o a -—-1 E - e '1 .5. .- w I I 60 — — E i o ’- 1 1 l l I l 1 l 1 l l 1 l l L l l 1 1 I l d O 5 10 15 20 Figure 4.6. The effects of ion temperature on the ideal argon beam emittance as a function of charge-to-mass ratio. Ions are assumed extracted at 10 kV, extraction aperture r3: 4 am and with 82: 0.25 T (approximately the same conditions as for the RTECR extraction). Ar Beam Emittance of Ideal Beam j I II I I I TI l I I IIII I I I I I 200-— ( Ti=tc(erq)T _ ioxq‘ -. ..J .. 5XQ‘ 150):- 3xq—: /"\ 'U .. - (U 1.. ~ - a - - E 100-_—- 0 ‘j E ; j w T' .. 50—— —a _ Vex=10kV _ : ra=4.0mm - _ 92:0.25'1' , 0 l l l l l 11 l l [111 lel l 1 LL 0 5 10 15 20 ‘1 Figure 4.7. Argon beam emittances with the ion temperature taken as T1: tc eV x q. Other conditions are the same as in Figure 4.6. 63 Ar Beam Emittance of Ideal Beam IIIIIIIIII’TrIIrIIIIll 1' 150 —- 6 (mm mad) 8 C) r 1 Figure 4.8. Emittances of cold argon beams with different extraction voltages and various extraction magnetic fields. The extraction aperture is ra= 4 11m. 64 times eV x q. A maximum emittance of about 200 mm mrad occurs for argon 18+ for an ion temperature equal to T1 = 10 eV x q. Figure 4.8 shows the case of zero ion temperature, equivalent to the hard edge model [De83, Ha87]. In this case the magnetic field determines the emittances, and further the ions with higher Q/M will have larger emittances. Argon 18+ has the maximum emittance of about 100 mm mrad for the specified conditions (extracted at 10 kV) in Figure 4.£3. The ion temperature in ECRIS is in the order of a few eV x q [Me86, An88], and based on the above arguments, we could draw a theoretical conclusion that the maximum emittance should be about 200 mm mrad for ECR ion beams extracted at 10 kV, for an aperture radius of 4 mm and a magnetic field of 0.25 T. 4.2.3 Extraction Electrode Design In ECRIS, the first electrode is generally designed by following Pierce's design theory [Pi54], which was originally developed for electron guns. It is based on the following assumptions: (1.) zero magnetic field; (2.) zero thermal energy; (3.) conservative electric field; (4.) electrons uniformly emitted from a planar cathode. Following Pierce, one solves the POISSON equation with the full space charge taken into consideration, which yields the following solutions for a rectilinear beam, with a parallel beam profile, in an accelerating gap. Inside the beam: “/3 (4.28) in” 65 while outside the beam: 2 2/3 V = A (22+ y ) B. -1 2. out c08(3 tan 2) (4.29) with 9J 2/3 A = [ ] (Ll-30) 4e,(2e/m)1/2 where z is the optic axis, J is the current density, e and m are the electron charge and mass. Eqs. (4.28) and (4.29) are subject to boundary conditions V = O at z = O and dV/dz = O at z = O. The condition voutz O at z = 0 gives the shape of the first electrode, which requires the electrode has an angle of 67.5° with respect to the z axis. Voutz Vex at z = D gives the shape of the second electrode. Such electrode shapes and the equipotential lines for a rectilinear beam is shown in Figure 4.9. Finally, at z = D we 4/3 have V - V = AD in - ex , and rearrangement yields the limiting value of nonrelativistic current density flow 3/2 1/2 V _ 4e,(2e/m) ex 9D which is the so called Child-Langmuir Law for the space charge limited emission [Ch11]. If the current available is less than this maximum current, then a converging beam profile will result in the transit of the gap. In the case of a cylindrical beam flow, where %¥-= ()1vithin the beam in the extraction gap is required, solutions of the POISSON IA 1.2 [.0 0.! 0.6 0.4 0.2 DISTANCE FROM EDGE OF BEAM (y) Figure 4.9. 66 -o.osov° zoo: 06—95511. —" 3: I-I '3 e: "'53 ‘-Z=‘- = 3:22 cameos suancz "1.3"."°".-’,:’I-’:-:':':':':'::.3:=::: ‘ 1 1 1 1 °I:’.°}}I1':-'.-131°3-2:231:232'335353'51:-313-1313.:3':Z. - 0.8 - 0.4 O 0.4 0.8 LZ DISTANCE FROM CATHODE (2) Plot of the electrode shapes (heavy lines) and the equipotential lines external to a planar space-charge-limited electron beam as determined from Eq. (4.29) [P154]. 67 equation can only be numerically obtained, but the results are very similar to the case of a rectilinear beam. According to Pierce, the first electrode still makes an angle of 67.5° with respect to the optical axis, while the puller has a spherical face, as Figure 4.10 shows. For positive ion beams, the above arguments hold except for a reversal of the extraction electric field direction, and changing e to Q and m to M. For a beam of multiple ion species, in which it is assumed that every ion species is uniformly distributed, the Pierce constant A is then of the form J1 (Oi/Mi) 2/3 A=[ 46,2 (4.32) 1/2 X 1/2] where Ji is the contribution of the i-th ion species of charge Qi and mass "1' The space charge limit current density is then replaced by the following expression 1/2 v 3/2 ex J1 _ 4en2 1/2 ' (Qi/Mi) 90 This would be the equivalent Child-Langmuir Law for an ion beam of multiple ion species. 68 12 IO 51" / 9 BEAM N '\ 5‘0 CATHODE RADIUS o N \ _: ommce snow mus or bLUI \ \ *‘q J“. "0 U ' ' 00 o .0. ..I o 0'90' 0 a“... " EDGE 35-33-2923 ::'::.’-’:".3:- -.'-:'-.=:'-:-’-. -" '::’-'-'1 TI“ '.°-°.°.°.'-:-.‘-: .::=: .’-:-’. ' .:::.:..o... Ezia::::£: :.:. 9...... :::.:.:.o.o:. P.}:.:.:.::.1P O (r .::.0..:.: .00 o .0 o o. o o ..... r ):.-.-.:.°-°--- 3:453:51? :13: 3" :1 35:3:{5-1'::_ i-‘:'.-::.';',‘-, AXIS o . ’ ’ ' ~::-, .- gm. ”5:: - O 5 6 7 _z_ DISTANCE FROM CATHODE Po ’ CATHODE RADIUS Figure 4.10. Electrodes for obtaining axially symmetrical electron flow of uniform diameter [P154]. 69 4.3 BEAM_3D Predictions on the Extraction Electrode Design The RTECR source has a three-piece electrode system, as shown in Figure 4.2. For historical reasons, the original puller electrode in the RTECR had a 45° angle, while the first electrode following the Pierce's theory is at a 67.5° angle with respect to the optic axis as shown in Figure 4.2A. A comparison of the electric field geometry between the 45° and Pierce spherical pullers is shown in Figure 4.11, in which the term "112a" denotes the 45° puller. It is seen that, compared to the Pierce puller, the axial and radial electric fields of the 45° puller are weaker at the extraction aperture and very strong at the aperture of the puller. BEAM_3D calculations have suggested that such an extraction system with a 45° puller does not work properly when the extracted current is at or below the space charge limited current. It has less focussing strength at the beginning of the extraction, and too much at the end, resulting in a drum shape beam profile in the first gap as shown in Figure 4.12A. A distortion in the phase area after extraction results in a large initial emittance, as shown in Figure 4.13. BEAM_3D suggests that an exact Pierce spherical puller, shown in Figure 4.28, is better than the 45° puller in ensuring a space charge limited current with a parallel beam profile in the extraction region, as shown in Figure 4.128, and less phase area distortion after extraction, see Figure 4.13. Therefore a better matching of the downstream beamline should result since the beam brightness is inversely proportional to the square of the effective beam emittance. Having demonstrated theoretically that a Pierce geometry is better (smaller initial emittance), the first of two consequences will 7O - COMPARISON BETWEEN PIERCE AND MZA ELECTRODE 300000 PI I T fir I r I I I I I I I I I T I 1 I; I I I l’ T4 I : Pierce: ———- " . 1 1 . zooooo — M23; --—---- 11 T p. I \ r r=O..05..1..15 in ; E 100000 . --‘ In )- . [I] L .1 )- .1 0 —“ _____—z ' *1 L. - ::"' __.‘.:‘.-----’,' 1- . ' N ‘ .: _, I .- L- / .- ’ 1 1 1 8 1 1 1 -100000 L 1 1 1 1 1 1 1 1 L 1 4 ._L_L._ 1 1 m 1 m 1 o 1 z a I. 2 (cm) COMPARISON BETWEEN PIERCE AND MZA ELECTRODE 1000000 I I I I fir I r I I I I l’ I I 1 I I I j T I T I fl 1 1 800000 L— Pierce: “ . 11211: ---.-~- T I r-O..05..1..i5 in .' 1, .1 .. oooooo -— I- 1 —J 3 h .541 1‘ 4 9 C I" ‘ ,- 3 U )- ../ ‘ -1 s 400000 :- .’ I -—‘ zooooo - -: » l o L L l l m L .l o 1 z a 4 2 (cm) Figure 4.11. A comparison the axial and electric field strengths of 45° (denoted by "M2a) and a Pierce spherical pullers. In both cases the extraction gap is 3.3 cm and the first electrodes are the same. 71 up.” up... qr... 45° Puller m.» u l ( n ). "~00 It.“ to... 70.00 07.00 100.00 “0.00 m.» m." up... up... 1; Pierce Spherical Puuer 3.00 0,... Q.” r 30.00 II.“ 00.0. 70.00 01.00 m... m.“ m.“ ""”zmi”ou.)'.' Figure ”.12. BEAM_3D calculated beam profiles at a space charge limited current for the extraction system with a “5° angle on the puller electrode face and a Pierce spherical puller. A drum shape in the first gap, and a focus in the puller electrode are seen for the “5" puller of Figure lLZA. 72 BEAM_3D Cal. He”. Vex=10 kV, I=1.2a4 em‘A loo '- I F I I I I I I fi—r I I I I I I I I? r .. ' . ' / P ‘ ‘1 L- .1 50 — _ b -1 b 4 T ' 4 a 0 ... _. ........................... _ v I" d 5< : q -60 t- —- 45° Puller -‘ f / i - - Pierce Puller ‘ 1 l l l l L I K 1 l I L l L l l l L l -100 -40 -30 0 20 4O X(mm) ¢>=Bmm.Tm=O.D=3.3cm.Z=4-1cm Figure ”.13. A comparison of the effective emittance after extraction for the 145° and a Pierce spherical pullers in the RTECR, for a space charge limited He1+ beam of 1.3 emA at D = 3.3 cm, with Vex = 10 kV. BEAM_3D predicts the effective emittance of the 115° puller is about three times that of the Pierce spherical puller. 73 be noted here (the other will be discussed in Chapter 5). It concerns the adjustment of the Pierce extraction geometry. Figure ”.118 shows the dependence of total helium 1+ current extracted from the RTECR, for 3 different main stage operating pressures [An88]. For these measurements, the source aperture was 8 mm, the extraction gap was 3.3 cm and the puller voltage was zero. The total extracted current is seen to follow the Child-Langmuir limit (labelled theory) up to a saturation voltage, and the saturation voltage is seen to increase with main stage pressure. Along the line labelled D = 3.3 cm, a parallel beam will be produced in transit of the first gap (as shown in Figure 14.128). To the right of the theory line, a gap of 3.3 cm will result in excess focussing in first gap and therefore higher divergence after extraction. This high divergence will result in a large beam envelope inside the focussing solenoid, and the solenoid spherical aberration will become very severe (this will be discussed in more detail in Chapter 5), and therefore poor beam transport results. I.“ Results In matching ECRIS beams to accelerators, the source tune is set by the ion production requirements, and the extraction voltage is set by the injection rigidity. So for example, we might find it necessary to operate the source on the lower pressure current curve of Figure 4.1” at a net extraction voltage of 10 W. In that case, to minimize the divergence after extraction, we must decrease the electric field strength in the first gap, by increasing the gap (D = 5 cm line) or reducing the voltage (AVp = 5 kV). 7‘4 FC#1 Current vs Extraction Voltage 101 p r T— I I I I I Fr d EU a 3.5x10': '1' E :X X 1.9210- T 2 _ a 0 1.11110" '1' . - — Theo - 17 D a I a ' a 100 5' . a x X " x xx ‘1 A Z a a 10 use»: ; a : D = 3.3 cm . a " . 3 01 .. . ' ! v ‘ | I 1 «It 10"1 _ ‘ . I —. (D I H ‘AVP=5 kV ; : :L': E :1 ‘ 1 D = 5 cm ‘ 10—2 1 L 1 1 1 1 1 1 L 2 3 4 5 6 7 8 910 20 Vs-Vp (kV) Obj Slit = 30 mm 1+ technique, the total extracted current of Figure “.1“. Using the He the RTECR was measured directly at PC“ as a function of extraction voltage, for 3 operating pressures. At low voltages, the extracted current is space charge limited, following the Child-Langmuir law (marked Theory). At higher voltages the extracted current is seen to saturate . 75 To do this properly, one should know when the extracted current is space charge limited. This can be achieved operationally by making the gap and puller voltage tuning parameters. For the RTECR injection into the cyclotrons at NSCL, we have in fact generally operated to the right of the D = 3.3 cm line. Since this was the maximum design gap, the least over-focussing would occur at Vp = O (Vp > O was not a possibility), which is exactly how the system did operate. Once we realized this limit, the first gap was modified to work over the range of 3 to 6 cm. This modified extraction system works better than the old one in better matching the following beamline and the 90° magnet, as an increase in transmission of the analysis magnet is observed. Shown in Figure “.15, are the transmission measurements from PC“ to FC#2 versus the extraction gap for a helium 1+ beam of intensities (I .<. 0.5 emA) extracted at 10 W with zero voltage on the puller (below space charge limited extraction), or a positive voltage on the anller (D = 3.3 cm, at space charge limited extraction). It can be clearly seen that, for this current range, space charge limited extraction gives the best transmission, which we learned theoretically also has the smallest divergence and emittance after extraction. When the total extracted current is below that for a space charge limited extraction, the larger extraction gap gives an extraction closer to the space charge limit thus has also smaller divergence after extraction, and better matching to the beamline therefore results. 76 Transmission Study on the lst 90° Dipole 400 ’- I I I I I I I I T TIT T I I r T r Ifi I I I I I I I [.1 P D D D=3.3 cm. VP=0 ~ 1- K 1‘ D=4.0 cm - _ x x D=5.0 cm _, __'1‘ ‘3 D=5.9 cm __ 300 _ + + D=3.3 cm. Vp Positive 697° 53% 1 A l" x . <1 - 78% « a . - 1 .. I" 4 o " . (\1 ,. - 2‘): r 0 ‘ r 85% ‘ E; 100— , '- _ ._ 1’ Z?) n .1 I /‘ 1 1 1 1 1 " o 1 L L l 1 1 1 1 l 1 p L I L 1 L L 1 l 1 0 100 200 300 400 500 I (FC#1, e,u.A) He“, Obj. Slit=15 mm, Ima. smazs mm, Vex=10 kV Obj. and Image slit Bias: —100 V Figure 4.15. A transmission study on the analysis magnet for different extraction gaps and helium 1+ currents S 0.5 emA. A beam extracted at the space charge limited gives the best transmission, with decreasing transmission as the beam intensity falls increasingly below the space charge limit. 77 Chapter 5 Space Charge Force and Pre-analysis Beam Transport 5.1 Space Charge Force Typical extracted currents from ECRIS are in the range of 1~2 emA for extraction voltages of 5~3O kV, which in turn are set by the injection requirements of accelerators or research. The energies of ion beams extracted from ECRIS are then 5~3O keV x q -- ion motion is nonrelativistic. Low beam energy coupled with high beam intensity will result in beam growth, if the space charge is not compensated. The space charge force will exert a relevant influence on the ECRIS beam transmission, especially when this force is very strong. For a beam with rotational symmetry, the space charge fOrce does not have an angular component, thus it has no effect on the ion angular momentum. As indicated by Eqs. (11.3) and (11.11), the space charge force affects only the radial velocity, and hence the beam maximum divergence, as will be demonstrated in the following discussion. As mentioned in Chapter 2, the space charge force for a rotationally symmetric beam of multiple ion species uniformly distributed is of the form 1 1 x v. 15.11 78 In a drift region after extraction, an ion on the outmost surface of a beam consisting of multiple ion species, experiences a radial force of (in cylindrical coordinates), 2 . p I. p =—3 -—°——£ 1 (5.2) where pe is the mechanical angular momentum, a constant of motion, and r is the radius of the beam. As indicated by Eq. (11.3), the first term originates from the initial canonical angular momentum after extraction from the source, while the second term is the radial space charge force in Eq. (5.1). Rearrangement of Eq. (5.2) yields 2 " pe Q Ii r : M2r3 + ZuMeor X vzi (5'3) Integrating Eq. (5.3) once with respect to the time t gives the radial velocity vr equation 2 pa 1 1 Q r 1 1/2 vr : [_§( 2 - 2) I uMe,ln( r ) Z v 1 (5.“) M r m zi m where rm is the radius of the beam where VF: 0. p9 Recalling the angular velocity is v9 = i?“ one finds the maximum . . . . 2 2 1/2 . transverse divergence at by d1v1d1ng Vt: (vr + v9) tw'the axial velocity vz of the ion in question 79 2 V P ,_t _ 9 Q Ii 1/2 at ’ v " [ 2 2 2 + 21“(p r) X —] (5.5) 2 M vzrm nMeovz m vzi Eq. (5.5) clearly indicates that particles on the beam surface will have a constant maximum transverse velocity, and a constant maximum divergence, if the space charge force is zero since Pe after extraction is constant. This is precisely the condition that is assumed in beam transport calculations when one omits the space charge force. Otherwise a is a function of r, which we will show is a t function of the axial drift distance 2. Thus at will be a function of 2, that is, the maximum divergence of the beam changes along the optic axis if the space charge is not fully compensated. The beam profile is obtained by integrating Eq. (5.11) once more with respect to the time t - 71-11111—1): 1 ——]"/2c1 = 1: (5.6) I" 0M6, v21 '1 H '3 KICDUN A '1 a 10].. here t = €_z_ is simply the time that it takes the i-th ions to travel zi from rm to r, assuming t = O at r = rm. There exists no analytical solution for the left side of Eq. (5.6), but numerical integration techniques can be used to give a reasonable result. To get a feel for the nature of Eq. (5.6) we can formulate an approximate solution. Let r : rm + X and assume X is small (i.e. a short drift). Then we have 02 I .9. _l_. _l_. ...Q. ..2. 1 M2 ( 2 ‘ 2) * uMe,ln( r 1 X v . r m 21 m 2 2p 1. 9 94, 1 ~[ + X ]X (5.7) M2r3 «Mcorm vzi and Eq. (5.6) becomes 2 2p I X t = [ 293 + “M2 r X v1 1‘”2 I cur/w“2 (5.8) M r ° m 21 0 m Performing the integration and re-arranging terms yields 2 2 r-r‘=l[2pe Q X11 Z_ (59) m H 2 3 “Hear v 2 ' ’ M r m 21 v . m 21 The beam envelope is seen to have a quadratic dependence on 2, with two terms, one due to the initial momentum of the edge particle and the other arising from the space charge force. For unneutralized ECRIS beams, we will now show that the second term dominates. We have solved equations (5.5) and (5.6) numerically for a helium 1+ beams of 10 keV energy and of various intensities after a waist, and plot these results in Figures 5.1 and 5.2. At zero intensity, Figure 5.1 shows that the maximum divergence is independent of the drift distance, and Figure 5.2 shows that a slow increase in the beam radius with the drift distance will be observed. As the intensity increases both the maximum divergence and beam radius sharply increase with the drift distance. An unneutralized 1.0 emA 81 Vex=10 I(V. Vp=0 KV. Rm=4. mm. Ra=4. mm. Bz= .251 T. He1+ 100 ijI IIIfiIIIIIIIIIII'IIII II : ‘15 \no DBB' q A 80'— -—1 '3 " 1505“» 1 H " fl E L' ‘506mh '1 f; 60:— I=O.4mA ‘ O - -1 ‘5 P I-OZinA ‘ E I -' . -1 4°1— ' -' C3 P 1 q t .. g ' 4 E 201" I=0.0mA _j 0" r g _ . or-PI ILLLLLLlllLlllllllllLlfi O 20 40 60 80 100 R(mm) Figure 5.1. He1+ beam maximum divergence versus the beam edge radius, for different beam intensities, after a waist. The maximum divergence is a constant if the space charge is zero. But as can be seen, if the space charge force is taken into account, the beam maximum divergence will increase rapidly with the level of the space charge force. 82 Vex=lD KV. Vp=0 KV. Rm=4. mm, Ra=4. mm. Bz=.251 T. He1+ 100 - I I I I rfI I I I I I I I I I 1 I I I I I I I I I I 80 L _ _ 60 r— °&. .... A P .1 E: b / ..,. 66$. 1- ’ . .1 V - \ ¢° %& . I" 40 — X ’0' &. -—1 I \ o?‘ 3 I ‘I 0?, 19" I 20 r- \ ‘ .— E i 5 00 “1" . .- _’-/ 1 o I L I L I I L I J L I I ILL l I J L L1 I I IL I l L L I I q 0 25 50 75 ‘ 100 125 150 Z (cm) Figure 5.2. A comparison of the beam edge radius with axial drift distance for various levels of the space charge. The starting conditions are the same as in Figure 5.1. For high uncompensated space charge, the beam envelope rapidly increases with axial drift. 83 helium 1+ beam will have an envelope radius 11 times the zero space charge radius after a drift of only 1 M. That is an enormous effect. In the RTECR analysis system, the distance from the extraction electrode to the solenoid center, and the distance from FC#1 to the 90° magnet entrance are both of the order of 1 M. In the case of no space charge force, the beam maximum divergence is a constant and so is xint= rm, that is . . ‘19 £(no sp) = xmaxxint: xintxmaxz lsgl = constant. (5.10) In the case of nonzero space charge force, both the X' and X are max int in) lon er constants and notin that X - r and X' - 'Xfifil .E§_ g 1 3 max' int- vz ‘ pzr ’ the product of X and X! max int ‘19 e(sp) = X' X X' X l-—1 = e(no sp) (5.11) int max= max int: pz is also a constant and equal to the emittance with no space charge force. That means the space charge force does not contribute to the beam emittance. A rigorous proof that the space charge force does not contribute to the beam emittance is given by L. Mills and A. M. Sessler for more general cases [M158]. Although the space charge force does not contribute to the beam emittance, compared to the case of no space charge force, it increases both the maximum beam divergence and the beam envelope along the beam optical axis, and this effect is illustrated in Figure 5.3 (the effective emittance can be 811 XI WITH SPACE CHARGE NO SPACE CHARGE Figure 5.3. A schematic view of the evolution of the emittance envelope after a waist with and without space charge force. The emittance is the same for both cases, but with space charge the tllaxilmm divergence and beam size significantly increase. 85 increased by the indirect effect of space charge causing aberration distortions). We note here another important consequence for the emittance after extraction from a Pierce geometry for high, but still space charge limited currents. Even if'a parallel beam is obtained in a Pierce - 1st extraction gap, the divergence after transit of the extraction electrodes will increase with increasing intensity. In Figure 5.11, BEAM_3D emittance calculations for helium 1+ beams are compared for these different intensities; in all 3 cases the first gap was D = 5 cm; Vex(end plate) = 10 kV, and the voltage on the puller is varied to ensure a space charge limited current. The starting thermal energy is taken to be zero. In each case the emittance after extraction is 77 mm mrad, but the divergence increases with increasing intensity as a result of the radial space charge force. This is a pure space charge effect -- mitigated only if there is some degree of neutralization in the initial beam. The 1 emA case in Figure 5.11 is typical fOr the total extracted current from ECR sources including the RTECR, and we will show that a significant emittance growth may occur in the transit of the focussing solenoid from such high initial divergences. 5.2 Rm Transit of the Solenoid lhgnet As mentioned earlier, the RTECR beamline had been designed under the assumption of a nominal beam emittance (5 x 110 mm mrad), without taking the space charge force into consideration. But the space charge force is not negligible, at least before the analysis magnet, because we have found indirectly that the level of neutralization may 86 BEAM_3D Cal. He”, Vex=1o kV, SCL Currents I III I I I I I I r Ij' I III I I I fr I I I I I I I I I 1- ' 1 r e = 77 mm mrd i 3 ‘ 50 F- ° -‘ 1- -1 L. -1 A I" .. 1.. E o r— ............... .- v 1' 4 5< r ~ ’ -' I (emA) _ ‘ r. - a 1 1 0.2 -50- . - _ . | 2 0J5 - __ | 3 1.0 L I I I L I I L L I. I I Li LI LLLLL I I I L I L L4 -30 -20 -10 0 10 20 30 X(mm) -¢=8mm,Tw=O.D=5cm.Z=4lcm Figure 5.“. A comparison of the divergence versus beam intensity for space charge limited extraction using the BEAM_BD code. Even though a parallel beam profile at the first gap is ensured, the effect of space charge, which increases the divergence, is clearly seen. 87 be quite low, less than ten percent approximately, because BEAM_3D calculations without any neutralization agree quite well with measurements. Thus this space charge force increases the maximum beam divergence well beyond the nominal design beam divergence at the entrance of both the solenoid and the analysis magnets, resulting in an emittance growth due to the lens aberrations. The observed low transmission from PC“ to FC#2, and the high divergence after analysis, are a consequence of this space charge force. The main point is -- since the divergence grows with drift distance due to this space charge force, the beam transport magnets are not in the right locations to correctly image the beam, that is, space charge alters the beam transport system. A beam crossing the solenoid with a large envelope will undergo an effective emittance growth due to the spherical aberration. This can occur for high intensity ECRIS beams because of low neutralization. Figure 5.5 shows emittances predicted by BEAM_3D, after crossing the solenoid for .065, 0.5 and 1.0 emA He1+ extracted from the RTECR. In these calculations Tl. is set to be zero, so the initial emittances of 69 mm mrad are determined by the other source conditions. In all three cases the puller voltage is chosen to achieve a space charge limited extraction in the first gap, and zero space charge neutralization is assumed. The emittances after crossing the solenoid, plotted at the position of FC#1, are seen to significantly increase with intensity. This is simply due to the increase in the beam envelope due to space charge (as shown in Figure 5.3) before the entrance of the solenoid. 88 The effective emittance growth due to the solenoid aberration, originating from a large beam envelope in the solenoid due to the space charge force, will also increase the beam envelope after the solenoid. BEAM_3D predicts that for a 65 euA He1+ extracted at 10 W at the space charge limit, the solenoid should be excited with 81 A to focus the helium beam with a waist at the object of the analysis magnet (FC#1), and will have a beam envelope of 1.6" at the divergence box, and is experimentally seen as shown in Figure 5.6A. Figure 5.68 1+ beam, also extracted at 10 kV at the space shows that a 550 euA He charge limit, has doubled the beam size at the divergence box due to space charge agreeing fairly well with a BEAM_3D calculated width of 3". The corresponding measured emittance at the divergence box for the 65 euA case is shown in Figure 5.7. As can been, the measured emittance of 69 mm mrad agrees with the calculated starting emittance. In the calculation, with T_,_o = O, the emittance is determined by the magnetic field. Good agreement with measurement does suggest that the initial emittance of this 65 euA case is dominated by the magnetic field. BEAM_3D predicts that if an extracted beam is far below the space charge limit in the extraction gap (voltage much greater than space charge limit voltage), the situation is much worse. It will result in very high divergence and large beam profile after extraction due to the excessive focussing strength in the extraction gap. Again such beam will have a very large beam profile at the divergence box due to severe solenoid aberrations and measurements support BEAM_3D's predictions. Shown in Figure 5.8 is a Kapton foil burn for a 65 euA 89 BEAM_3D Cal. He”. Vex=10 kV, SCL Currents I I I I l I I . ~ Initial —: 69 mm mrd D A 1: " i E 0 _ _ ....................... _ v L After Solenoid ‘ - _ 1 N +- I ‘ . _ (emA) (mm turd), 40,. 1 0.065 as _ P 2 0.50 92 y r , 3 1.0 340 . L L I L L I I I L L L I I L I _L I J I -20 -1o 0 10 20 X (mm) ¢=8mm,T,o=O,D=3.3crn,Z=190cm Figure 5.5. focussing solenoid for various beam intensities. The effective emittance of He 1+ after crossing the In each case the extraction is space charge limited, the beam energy is of 10 keV, and the emittance after extraction is 69 mm mrad. The 1.0 emA case shows very large emittance growth due to its large beam profile in the solenoid, thus the aberrations have become very severe. 9O \ mmmu' "11111111” :11 -...W M \ .. B Figure 5.6. A and B are Kapton foil burns at the divergence box with 1+ He beams of 65 and 550 euA respectively. The beam passes through a defining slit plate 8 cm upstream of the foil, giving horizontal marks on the £011. BEAM_3D predicts for 65 euA He“ with space charge limited extraction (Vex = 10 kV, Vp = 8.5 kV), beam profile at the divergence box will be 1.6" and that is experimentally seen. A 550 1+ euA He extracted at space charge limit fills the Kapton foil at the divergence box, also agreeing fairly well with a BEAM_3D calculated profile of 3". 91 He“, 65 epA at. FC#1. Obj. 10 mm. L=7.87 cm 40 I I I I I T I I I r I T r I I I r I III I l T l l .J P d 20 — _. P d A ~ 1 s _ « L. 0 - - e - . v .. q 5< : ‘ -301'- -1 1: e = 69 mm mrd‘ t 1 _w I I I L L I I I L L I I LI L I I I I I I I I I -20 -1o 0 10 20 X (mm) Vex = 10 kV, Vp = 8.5 kV, [sol = 82 A Figure 5.7. The measured emittance for the 65 euA I-Ie1+ beam in Figure 5-6A is e = 69 mm mrad, which agrees very well with the BEAM_3D calculation (see Figure 5.5), in which the ion thermal energy was tzaken to be zero. 92 :"~-_,-~-- mfl~r~r rats-3"???"- ‘ ' " " - .. _ ‘.,-w .- ' _ ‘ ‘ ‘ . ‘ 9.... - ~ . . ...‘ . ,. :.e.—-e..,- a .55.“. ... cw -—.o.r-————. t'.‘ -~.~~-. - . ,s . ' .....- '1; :_- -.. v V W? - ‘ 1~I'I_ 1 ' 1 ‘ 'A , H” - - M; .1 — 0 -_‘_‘_L . . -... .-—.....—-—3 — e—fl' ‘ -"_. :—.—.—— ..f - .. - .w— “ _, ...-“-....- . ....-. O-uoordodfi—I- .. _ ,. ...... - _ _ o— ..-—n“..- - - ...-n 'V ‘ a- _- .4 r” — - . - _ . ' . ~— . .- ...- --:-;—r -——--‘—“_-_q“ - ‘ ‘ v w- “‘ ' o ‘ LI V m-” . - 9' . ‘ v - - -.. ~ ’ '9‘.“ . . 'n-‘ O; Q I ... V _ - --.. ,— ..- — ' .. ‘ 04-3-99 .. 343...... ...... ...- A . U. .... ‘v av...“ ‘**~ «««««« o-O ‘ .., . ~ - ' l._‘ U I ' - 0: w.' ffi ..L—aoh— " o ‘ . _ . 1.:." a ~ 3 , c I .' I “m:;a‘ I‘ W’- ‘1 WJ— w Wu¢ an - . ‘. .... . -¢ - .- 2am“. . $2.3. ....4 . ~. ...~-W‘~L "' . . Figure 5.8. A 65 euA He1+ beam extracted (Vex = 10 kV, Vp = 0) well below the space charge limited (Vex = 10 kV, Vp = 8.5 kV) current results in high divergence and large beam profile. For this case, BEAM_3D predicts a diameter of 5.5" at the divergence box. 93 BEAM_3D Cal. He”. 200 epA. z = 2565 mm I I I I I I I I I T I I I I I I I I I T I I f I . - x . .. 00 - x x _ _ 6 o a o : A E ' i E ‘0 r— — v ,. 1 N - -4 g . . X P Tto = 0 1 20 — , _. _ Calculation: x x ‘ - Measured (at least): 0 o ‘ o L I I I I I I L I I I I L I I I I I I I L L I L 0 10 16 20 26 100 - I I f I r I IiT I I 1’ I I I fI I I I I I I I I ‘ r- d P x x . x 1 00 — .. r- x 4 C 0 D U U :1 A LE- 60 — — V P' .4 >4 I . 3 4° ’ “ 5< ; I ’ Tt0 = 0 ‘ 2° :— Calculation: x x g - Measured (at least): :1 o 1 o I I _I I I L L I I I l I I I I I I I I I I ,I d 0 5 10 is 20 25 Vex (kV) Figure 5.9. BEAM_3D predicts that a 200 euA He1+ extracted at 7, 10, 15 and 20 W with an extraction gap of 3.3 cm will have very high divergence and large beam profile at the divergence box, because the extraction is far below the space charge limit. Measurements, limited by the measuring apparatus to a maximum divergence 65 mrad, show that the actual divergence is higher, in fair agreement with the calculations. 911 He1+ beam extracted well below the space charge limited current. As can be seen, this 65 euA He1+ beam profile fills the whole measuring frame, and as BEAM_3D predicts, has a diameter lager than the 550 euA space charge limited case. Figure 5.9 shows the BEAM_3D predictions and measurements (the measurements are limited by the apparatus) of the maximum divergences and beam profiles for a 200 euA He1+ beam extracted at 7, 10, 15 and 18 W with a gap of 3.3 cm. All of these extraction conditions were well below the space charge limit extraction, and result in high divergence in the beamline due to over focussing in the first gap. 5.3 Transit of the Analysis Magnet Because of the unneutralized space charge force, the divergence at the entrance of the analysis magnet can be significantly higher than that assumed in the beam transport design calculations. The transit of the analysis magnet may then result in substantial beam aberrations. We have graphic evidence of this effect for the other operating ECRIS at NSCL, the CPECR [An86b]. The analysis system for the CPECR differs from that for the RTECR, in that there is no focussing magnet -— the source extraction electrode is placed directly at the object of the 90° magnet (FCH in the RTECR system). During the first year of operation of the CPECR, primarily lithium beams were produced for injection into the [(500 cyclotron. For lithium production the source is operated at high pressure on helium support gas with lithium vapor coming from an oven. The total extracted current is about 1 emA with about 50% helium 1+. After about 1 year of operation in this manner the source was moved to a different 95 beamline, and the image Faraday cup assembly (equivalent to FC#2 in Figure 1.2) happened to be removed as a part of this operation. We found a large triangular beam mark on the face of the A Jaw collimator mounted just before this Faraday cup, as shown in Figure 5.10. The bulk of our object side foil burns on the RTECR do not show triangular beams, for example as those shown in Figures 5.6 and 5.8, so this mark on the CPECR FC#2 assembly is more likely related tn) the transit of the analysis magnet than to beam effects at the source. Beam transport calculations at the design emittance (5 x 140 mm mrad) for this dipole design do not show evidence for triangular beams after transit of the analysis magnet [N087]. In addition, extensive magnet studies do not show magnetic field errors that might result in triangular beams [N089]. If however we consider the transit of the analysis magnet with an unneutralized 1.0 emA beam having the design starting emittance at the object point, we are able to generate the triangular beam marks observed. Figure 5.11 shows an intensity contour plot and transverse coordinate beam profiles at the image of our dipole magnet with a 1.0 emA He+ beam having a starting emittance of 200 mm mrad. The intensity is uniformly distributed across the initial beam profile. This calculation was made with the 6105 beam transport code [H087]. The calculated profile has the same shape as the observed slit plate mark in Figure 5.10, and would be due to the second order aberrations that result from excessive divergence at the magnet entrance. The excessive divergence is due to the space charge growth. Furthermore, the y-profile in this calculation is strikingly like the scanner profile for an Ar10+ beam made after the RTECR analysis magnet that was shown in Figure 3.8. 96 .msflwmwumnm vawo 9N mfimsmo dam mung p959: man EH3 5 53mm“ 60555 98%.: on» owowmn 88g? Emma 93 so pommwm 0mg 08% d5 8 B 85% we mama cage» mg no waste was .mumau 05 now mane—cums gum mo wopmfifloo 93 mo 00mm on» so comm ma gram: Emma 3.3 m .36 mag 97 PLOT 0F 1x VS a) x - RANGE -O.200E' a - RANGE -O.100E°( PLOT 0F 0( VS Y) X - RANGE -O.3OOE° Y - RANGE -O.3OOE- I I j I I If I I I I I 90 DEGREE MAGNET : Figure 5.11. A 6108 beam transport calculation for the case in Figure 5.10. The transit of the analysis magnet with an unneutralized 1.0 emA helium 1+ beam of starting emittance 200 mm mrad will result in a triangular shaped beam after analysis. 98 5.11 Matching the 90° Analysis Dipole under the Effect of Space Charge As mentioned above, the space charge force alters the effect of the beam transport system. So even if the beam is extracted at the space charge limit and properly focussed by the solenoid, with little emittance growth crossing the solenoid, the space charge force still can increase the beam divergence and beam envelope beyond the analysis magnet design limit, and a poor transmission of the analysis magnet will result. The lens will treat the beam, regardless of the prior history of the beam, if it has the right divergence and beam profile at the dipole entrance, as if it comes from the design object location, and image the beam at the design image point. If the space force is zero after the dipole entrance, it will not affect the beam imaging process. If the space charge force after the dipole entrance is not negligible, then this force will still affect the beam transport after the transit of the dipole, and the beam may not be imaged at desired location with the right size. In addition, an emittance growth may occur in the dipole transit because of aberrations. Based on the above arguments, one may improve the transmission of the 90° dipole by deceiving the magnet. The deception is to move the beam waist closer to the magnet entrance than in the design, as schematically illustrated in Figure 5.12. Because of the shorter drift distance to the dipole when the waist is moved closer, the increase in the beam divergence and the beam envelope due to the effect of space charge will be less than if the beam waist was at the design object. If this results in beam characteristics that are closer to matching the design optics at the dipole entrance, then the 99 .omamco woman o: no ammo on» o... @8358 omamno woman :33 283 com 383 .8 2: .8 9.332. .533 ..c 83932:: 33528 a .m..m 93m: muuoco oooaw ouuoco oooam ct; BB; 305:; +20; . Ea +®CUUE +O®_.A_O wfiboco 100 ions will be imaged closer to the design image location. We tried this technique, it works, and further confirms the transport limiting effects of space charge on the drifting beam. As shown in Figure 5.13, a 330 euA He1+ was extracted from the RTECR at the space charge limit, has a waist at the dipole magnet object when the focussing solenoid was excited with 81 Amps, and the maximum transmission for this setting is about 791. If the solenoid excitation decreases to 78 Amps, the beam waist moves about 10 cm closer to the magnet entrance, a maximum transmission of about 871 is obtained. BEAM_BD calculations show that the solenoid spherical aberration is minimum for this beam after the transit of the focussing solenoid either for the solenoid excitation of 81 or 78 Amps, but the second case (78 Amps) gives a beam with much closer divergence and beam profile to the optics design, as shown in Table 5.1. Therefore at 81 Amps, the beam is both bigger and has higher divergence -- both are bad, and the transmission decreases as a result. Thus the dipole magnet matching with a closer beam waist is simply due to the beam space charge. Table 5.1 Beam envelope at the 90° dipole entrance Design at BEAM_3D (He1+ 330 euA) 90° entrance Solenoid: 78 (A) 81 (A) xmax (am) no 37 All Xéax (mrad) MO “3 52 Note: A beam of 5 x 110 um mrad is assumed at the object in the optics design. The drift distance is 1 meter to the 90° entrance. 101 He“, 330 epA (FC#1), Vex = 10 kV, Vp = 2.6 kV 10° ’- Ifi T I I l I I T I r I T I l’ I I I I I I I I I l I I I I I 1 - 4 0.0 :- 28 x 28 slit -: 7: I 1 2;: (L6 P- -: rat. I 17 X 17 slit . \ _ . .. 0*2 "' -4 o 0.4 I . . E; ; 20 x 10 snt 3 0:: 0.2 L 1 i . 00 r. l 1 l I I I I I l I I 1L1 I I l I LI I L I l J I I I I I d ' 70 72.5 75 77.5 00 82.5 as 1301 (A) ¢ex = 8 mm, ‘I’pul = 12 mm. D = 5 cm Figure 5.13. A 330 euA He1+ is extracted with space charge limit and transported through the 90° dipole, this beam has a waist at the dipole object when the focussing solenoid is excited with 81 A. However the optimized transmission occurs at I(sole) = 78 A, for which the beam waist is about 10 cm closer to the dipole. 102 Chapter 6 Summary and Conclusions 6.1 Extrapolation to mltiply-Cl'arged Ion Deals The original motivation for the development of BEAM_3D, and the beam measurements on the RTECR, was to study the emittance and beam transport matching of multiply-charged ions. This has led to the He1+ technique, simplifying both the calculations and the experimental studies. We have found indirect evidence for low neutralization of the initial beams, with several important consequences. It is necessary for the extraction to be space charge limited in the first gap, leading to the use of a complete spherical Pierce lens system, to minimize the initial divergence for any total extracted current. The space charge force is proportional to the square root of M/Q, which 1 means the space charge force from 100 euA Ar + is equivalent to 316 euA He1+ at the same extraction voltage. Thus for heavier ion beam transport, the space charge force before the analysis, if not neutralized, will become much stronger than for a helium ion beam at the same extraction voltage and with about the same total extracted current. Although the space charge force does not increase the beam phase area, there may be lens aberrations due to substantially larger than design divergence at the magnet entrances. The high divergence tails and triangular shapes of ECRIS beams after transit of the analysis magnet are likely due to this effect. The RTECR tunes for multiply-charged ions require much higher 1 microwave power than for the He + beams, and gas mixing, and we have 103 measured thermal energies of about 6.5 eV x q for higher charged argon ions [An88]. As a consequence the starting conditions are likely to be some what different for multiply-charged ions than for the He1+ studies reported here. Preliminary BEAM_3D calculations for an Ar8+ beam extracted from the RTECR have been made, using T4,, 5 5 eV x q, and an actual charge state distribution of intensities among argon ions and oxygen support gas ions. These calculations showed that the Ar8+ ions are sensitive to the full unneutralized beam current before the solenoid entrance. A spherical aberration occurs in the solenoid crossing, increasing the emittance about a factor of two, as shown in Figure 6.1. The solenoid does some pre-analysis, but the lost ions are mostly of higher charge than 8+ and do not constitute a significant percentage of the total extracted current. Therefore for such Ar8+ beams, we have then essentially the same problem as for the He1+ beams -- the divergence growth before lenses would be expected to be a critical limiting phenomenon. We have already seen in Figure 3.7 that high divergence tails are observed on highly charge argon ions measured after the analysis magnet, and there is an expectation that this will prove to be due to aberrations as a consequence of high divergence at the analysis magnet entrance, when further measurements are made. 6.2 Sumary and Conclusions In this thesis, some aspects of the RTECR ion beams have been studied both theoretically and experimentally. The new 3 dimensional code BEAM_3D, with a straightforward space charge model for beams of multiple ion species, has proved to be a successful analysis tool at 1011 BEALBD Cal. Ar“. 15 em (FCflZ). Vex=13.44/—2.15 xv 60 I I I 20 X'(rnr) O r'filT'ITIUUUIII'IT]'IIU[IIII I I I ¢=8/ 12 mm, '1‘,°<5 qu, D=5 cm, I(sol)=94.3 A Figure 6.1. BEAM_3D code predicts that after crossing the focussing solenoid the effective emittance of’Ar8+ (S shaped, due to the solenoid spherical aberrations) is doubled compared to its effective emittance before the solenoid. The CSD.and focussing solenoid excitation are based on actual operating values. 105 least for the helium beams. A better extraction geometry to ensure a parallel beam with minimum divergence at the extraction gap has been introduced. The aberration of the focussing magnet lens due to a large beam envelope has been demonstrated, and subsequently a better transmission through the analysis magnet resulted from the realization that the space charge force was driving the focussing lens aberration. The good agreement between BEAM_3D calculations and equivalent measurements suggests additionally that the plasma boundary and starting thermal energies do not play a significant role in determining the emittances when the source is tuned for these He1+ beams. Based on the studies presented above, it seems not too unreasonable that an emittance upper limit of 200 mm mrad is achievable, if no aberration occurs during source extraction, for an aperture of 8 mm, an extraction voltage of 10 kV, and a magnetic field of 0.25 T, since there no evidence that the ion temperature is higher than 10 eV x q. For cool ion beams, the transverse emittance is simply dominated by the magnetic field which converts a small amount of momentum into the angular direction. While if the ions are warm, at a few eV per charge state, both the ion temperature and magnetic field are comparable in contributing to the beam emittance. Space charge neutralization is very low in the RTECR beam line and therefore the space charge dominates the pre-analysis beam transport. The RTECR beamline is capable of transmitting a beam of 5 x 140 mm mrad emittance, but space charge alters the beam transport by increasing the beam divergence, so the main task is to compensate the space charge force to avoid lens aberrations. 106 Shortening the beam drift distance is onecaf the means to compensate for this space charge effect. Since the beam envelope is quadratically proportional to the drift distance, reducing half of the drift distance can reduce a factor of u of the beam envelope, and the aberration will become very small. Other alternatives would be to (1). generate a parallel electron beam within the ion beam to fully neutralize the space charge [Kr87], and one could then return to the designed beam transport system based on zero intensity transport calculations, or (2). assume a maximum space charge in the design of the beamline, and weaker beams would be properly transported by retuning the beamline. All of these techniques can be subjects for future study on ECRIS ion beam characteristics to fully understand this young technology for future development of ECRIS. 107 Appendix Introduction to ECRIS An ECRIS is a confined plasma device from which it is possible to extract useful beams of highly-charged ions. Microwaves are launched into the plasma, resonantly accelerating confined electrons. These hot electrons ionize atoms in a process loosely described as electron impact ionization. Ions lost from the magnetic confinement zone fall into the extraction zone where beams are formed. The key components of this kind of positive ion source and the main operation characteristics will now be briefly discussed. A.1 'Unit' ECR Cell All ECRIS have at least one unit ECR cell, which will now be defined. A unit ECR cell consists of a vacuum vessel, a minimum-B magnetic bottle [N183], a microwave generator and an extraction system, as illustrated schematically in Figure A.1. The vacuum vessel 6 to 10"7 T), and serves as a is maintained at low pressure (~10- microwave resonance cavity. The minimum-B field provides the plasma confinement and nested closed magnetic surfaces for resonant electron heating. This minimum-B field is fOrmed by superposition of a pair of solenoid coils and a multipole magnet. The solenoid coils (room temperature or superconducting coils) produce a tandem magnetic mirror field, as shown for the NSCL CPECR [An86b] in Figure A.2. Tandem mirrors would provide the well known axial confinement for a collisionless plasma, but do not contribute to good radial confinement 108 GAS WE VACUUM VESSEL (PLASMA CHAMBER) MINIMUM B MAGNET/C FIELD HEXAPOLE / RF / \\ ———-—-7————-—-—— - -___<::~—-- COILS .\ \ EXT RACT ION Figure A.1. A 'Unit' ECR Cell consists Of a vacuum vessel, microwave generator, a minimum-B field and an extraction system. 109 .mHmom ammo» mamcfim a you madoo ufiocoaom «o own a an boos—coca 3:93 33.“ 038mm... 3:8 183»... < .~.< 9.33m T... v N Ofl O0 ON 0— ¢ r q ‘14 u 4 . file 4 a 4 A 1 4 . O r IL— . I fil In I 4 P In f i w .. 1.. 11v f _ p F . p p p — P p . r — . L b P 1 ”ME—LOW: mam: 43x6. moan—1&0 (ox In) as 110 due to ion - ion collisions and bad field curvature in between the mirror coils. The addition of a multipole magnet, which produces a magnetic field that increases with radius (quadrupole or higher multipole), provides improved radial confinement. For historical reasons, most ECRIS have used a hexapole magnet for this purpose. Ir) ECRIS, most hexapole magnets are made of Rare Earth Cobalt permanent magnets (for example, SmCo, or Sm2Co,,) because equivalent strength coils would have very high power consumption, we choose permanent magnets at the price of a loss of field adjustability. As can be seen in Figure A.3, the field strength of a typical ECRIS hexapole magnet varies approximately with the square of the radius over most of the magnet bore [An83]. The superposition of a tandem mirror (solenoid field) with a hexapole field is then one way to produce a minimum—B field, In such a superposition, the magnetic field will increase in all directions away from the center. It has been established experimentally that a minimum-B field provides better plasma confinement compared to the case of only a tandem mirror field [1062], the resulting minimum-B field topology produce by a.set of mirror solenoid coils and a hexapole magnet is schematically shown ixll?igure A.“ [An87b]. The longer ion and electron confinement times in a minimum-B field has significant consequences for high charge state ion production. First, the step-by-step ionization dominates the ionization process [Ge85], so the longer the ions stay in the plasma, the more probable higher charge states become. Second, electrons will have higher energy in the plasma if their confinement time increases. 111 .amm m :H can modem on» no one mcoam madam; «o couuocsh m mm Bongo... m «o saucepan on... msonm 0.3m: m2; .m.< 0.3m:— .Sno.;.~.m.:um..~u< AEVu m as s a... o II I I l I I III—III I [III I III A an». V mvmwnm .8. hanstm .mm a so; m (9x In) «Ia 112 Ffieui lane 71 I L AVIS Igrzx ‘\fiV\ifi\_;l I‘F‘1Ij1 H / l I I 7 L 164‘; Figure A.“. A "minimum-B field" topology as a result of the superposition of a hexapole and a set of solenoid fields. 113 Charged particles moving at a magnetic field will experience a Lorentz force §=QGX§ (A.1) where Q is the charge that the particle carries, 3 is the particle velocity and 8 is the local magnetic field. For historical reasons, we call the frequency of such particle rotation the "cyclotron frequency", which is related to the local magnetic strength B, the charge Q and the mass M of the charged particle by the following expression :I‘B (A.2) If the charged particle is an electron, the above cyclotron frequency is called the "electron cyclotron frequency". - 93 (A.3) w - co m e where e and me are the charge and mass of the electron respectively. When a plane wave of frequency w is launched into a plasma having electrons confined by a magnetic field, acceleration is possible where w 2: wec' Energy can then be transferred into the electrons from the incoming electromagnetic wave. This energy transfer process is called "Electron Cyclotron Resonance Heating". As a consequence of the heating, the energetic electrons then can bombard the atoms and ions 11A to a certain degree of ionization. In ECRIS the electron energy gained by ECRH heating can be up to hundreds keV, but the peak of the distribution is at tens of keV [Be8li], which improves the probability for ionizing a variety of atoms and ions as can be seen from the ionization potentials, taken from Carlson et a1 [Ca70], of various atoms and ions shown in Figure A.5. Some ECRIS make use of two ECR cells, for example, the RTECR is a two stage room temperature ECRIS [An86a]. In two stage ECRIS, the first stage produces a predominantly 1+ dense plasma which diffuses into the second stage (main ionization stage). The advantage of two stage operation is the coupling of two stages greatly enhances the high charge state ion production, because the main stage operating pressure is substantially reduced while maintaining a high plasma density. Comparison of one stage versus two stage operation for nitrogen ion production in the RTECR is shown in Figure A.6. A.2 ECR Operating Characteristics Here we briefly summarize important operating characteristics of DC mode ECRIS. The reader is referred to the literature, especially [6e79, Jo8fl], for additional information on this subject. 1. ECRIS reach charge equilibrium. In equilibrium, net charge gain in the ECRIS plasma should be zero. Thus we require that, 5e = {1q(¢;+¢:+....) (A.u) Q 115 Ionization Potential ‘0‘ IIIIlfirrII,TIIfIIIITIITIII 103 , 9 103 _ s I /’ E a" , He H Ar H )03 Obi! 100 1 L LJ I l l 1 l l l I L I L l l L l L i L 1 O 5 10 16 30 Figure A.5. Single ionization potentials of some atoms and ions. 116 STRONG 2 STAGE OPERATION VS. 2ND ONLY BO .- I I I I I I I l I I I I I I I I I I I I f I I I I T I fi : He“ N3 + He Feed j .. ....-- 2 STAGE - 60 L— __ 2ND ONLY ""‘ i : N‘+ N1+ I; f " N5+ N3+ 51 - g _ N2+ ;: .1 12‘ - fl 1 D '- q 0 Q ” .. a — — 5 . g ' -1 '- 1 1 I I I 1 I L I I I I I I 1 1 1 1 I I I I I I L 1 I 1 J 50 75 100 125 150 175 ANALYSIS MAGNET CURRENT Figure A.6. Performance comparison between 2-stage and second stage only RTECR operation for the production of nitrogen ions. Helium is used as a support gas. Each next higher charge state shows a large percentage increase in current with the first stage on. 117 where Qe is the electron flux density, 5; stands for the flux density of ions with q electrons removed, and there may be as many as i of ions of different elements with the same charge state q in the plasma. Since the net gain of electrons and ions in the plasma should be zero, we must also have dNe dNi a;— = Adi: = 0 (A5) where Ne is the electron density and N is the ion density of charge iq state q. 2. The probability of producing multiply-charged ions in a single electron impact collision falls off rapidly with increasing ion charge Q. The production of highly-charged ions in ECRIS is dominated by step-by-step ionizations [Ge85]. The single step ionization rate, for an ion going from state q to q+1, is a function of the electron energy E and is given by R (E) ion q,Q+, (2)-ve(E)~ue(E) (A.61 : oion q+q+1 where o is the electron impact single ionization cross ion qoq+1 section which falls off rapidly with increasing charge state q for a given electron temperature [Mu80], ve is the electron velocity and Ne is the electron density. The ionizing electrons in an ECRIS are not monoenergetic, but have an energy distribution. An integration must 118 be performed on all possible energies to calculate the ionization rate R [JoBM]. The exact form of the electron distribution in ECRIS is not yet clearly known. For simplicity, a Maxwell distribution is generally used in order to estimate the ionization rate. Shown in Figure A.7 are calculations of ionization rate coefficients S = (Rion q+q+1/ Ne) for stepwise ionization of argon atoms and ions, using electron-impact cross section due to Muller et al [111180], and the atomic subshell binding energies from Carlson et al [Ca70]. 3. Charge exchange between ions and neutrals occurs in plasma and this is an important limiting process. Single charge capture from neutrals dominates the charge exchange process. The cross section for single charge capture, proposed by Muller and Salzborn [Mu77], is = 1.u3 10-12-q1'170P6’;76 cm2 (A.7) oexch q+q-1 where P, in eV, is the first ionization potential of the atom. Muller and Salzborn also give formulae 0 through 0 exch q+q-2 exch Q¢q-u° However, as q increases, the double and higher order charge exchange processes can be ignored when compared to the single charge exchange process. Typically, these single charge capture cross sections are three to four orders of magnitude larger than ionization cross sections. The corresponding rate of single charge capture between ions and neutrals is 119 Ioniztion Rate Coefficients 10-6 :- I I IIIIIII I I IIIIII] I I IIIIIII I IIIIII‘ E " q 1.0-7 §_ 1 E 7 2 ..8 h / 10 .E. 3 E 5‘ _. 45 “in - 67 B 1.0—9 r- 3 E "’ E o h 1213/ ...1 .1 10 E— 14 g E 15 j " 16 - 10"11 4 IIIIIIII 1 UIIIIII 1 I4IJILII J 1 IJIJIJ ... 102 103 104 105 Te (eV) 10 Figure A.7. Ionization rate coefficients S for single ionization of argon atoms and ions from the ground state by electron-impact in plasma (Maxwellian distribution, no collision limit). 120 Rexch q+q-1= oexch q+q-1.vin.N° (A'B) where vin is the relative velocity between ions and neutrals and No is the neutral density. The ions in ECRIS plasma are rather cold compared to the electrons, at most a few tens to a hundred eV for ions of charge state q S. 20 [K086, Me86, An88], and the ion velocities are much slower than the electrons. Thus there is a competition between ionization and charge exchange in ECRIS plasma. Since we do not have much control over the charge exchange cross sections and the relative velocity Vin, the most effective way to reduce such charge exchange is to reduce the neutral density N., and ECRIS generally do operate at low pressure, to ensure the best performance of the source. Typical operation pressures in the ECRIS ionization (main) stage is 10.6%7 T, for two stage ECRIS, the operation pressure in the first stage is 10‘3~'“ T. 4. The electron density is limited. The maximum electron density in plasma is tied to the microwave frequency by the following relation N = 1.2ux10’8r2 (A.9) ec which is a consequence of a limit for electromagnetic wave injection for a given plasma density. Here Nec is the critical electron density and f is the microwave frequency. According to Eq. (A.6), increasing the electron density will increase the ionization rate, therefore to 121 improve the high charge state ion production we should raise the density, but Eq. (A.9) sets an upper limit on how high we can raise electron density in ECRIS plasma for a given microwave frequency f. Thus one wants to increase the electron density further in ECRIS, the microwave frequency and the magnetic field should be increased accordingly. 5. Low gas consumption. The source of plasma in an ECRIS is neutral gas. The gas consumption is in the order of one standard cc/hr, due to the low operating pressure and good ionization efficiency. For example, the gas consumption of the RTECR has been measured to be $1 standard cc/hr [An87a]. A 1 standard cc/hr consumption of helium is equivalent to ~7.5x1o15 particle/sec, while the total extraction current from the RTECR (mainly He1+ beam) is 0.5 emA, or 3x1015 particle/sec. The ionization efficiency is then IE z N /N,, = 110%. Metallic ions can be 1 produced by the use of an oven that makes metal vapor, as shown for the NSCL CPECR in Figure A.8, or by direct feed of the material into the main stage plasma [Sa87]. 6. A mixture of a lighter gas as support gas usually boosts the yields of the intermediate and high charge state ions of a heavy gas. Figure A.9 shows a comparison of pure Argon feed to the effect of mixture of Argon with lighter gases obtained from the RTECR, and similar results were also been observed in other ECRIS [Br811, Ly811]. This effect has been observed in most ECRIS, readers are referred to the literature of ECRIS for the details. The effect of gas mixing 122 WINDOH jfi TURBO PUMP xsruxs {You “c": d_. arcsowsvs xzxuots 1—. ._..- use . —Ill _' :L Figure A.8. A high temperature oven for producing metal vapor is equipped with the CPECR Ion Source at NSCL/MSU. 123 .comnm no“: mommm Loanmda no mcfixfia on» a“ zoom 3 mama :0 33.36 mats... new no mucoucoqoo noon: of. .o.< 6.33m Qw>ozma wzomhumqm O "IIII I s . E o. m s . e s . s . . . q . 4 Ts.“ n a, n 9 .z m xa komuum oszHz men as . . 7 n M? , ...; \ch zoom... zoomc mumnE I . I II ./ ... /.,. .1. m x”. ..®1\\\\0I + . s." . .. «I I r Hz.» .4. / I ./;1 I". I W ,1“! 1.1/,/. D n NO+\ «Bur/DI ./.H.: 7.06 .(fx I .1”! .1. m .uuy. Jr.) .... nnfim.‘ m ~2+\ . ”Hz” . 3.33.358! In la n. .lonoloto-0151510lvlanal-lé Os.“ 12“ could be explained by an ion cooling model proposed by Antaya --energy transfer from the heavy ion species to the light ones [An88]. Such thermalization results in longer confinement time of the heavy ion species. 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