LIBRARY Michigan State University PLACE IN RETURN BOX to remove this checkout from your record. TO AVOID FINES return on or before date due. ' DATE DUE DATE DUE DATE our: 1/98 COMM.“ ASYMNIETRIC FLOWS OF NEWTONIAN AND NON - NEWTONIAN LIQUIDS IN SYMNIETRIC PLANAR EXPANSIONS By Sanjay B. Mishra A DISSERTATION Submitted to Michigan State University in partial fiilfillment of the requirements for the degree of DOCTOR OF PHILOSOPHY , Department of Chemical Engineering 1997 ABSTRACT ASYMMETRIC FLOWS OF NEWTONIAN AND NON - NEWTONIAN LIQUIDS IN SYMMETRIC PLANAR EXPANSIONS By Sanjay B. Mishra The flow bifurcation of Newtonian and inelastic, shear thinning liquids through an abrupt planar expansion with an area expansion ratio of 16 has been investigated. Model Newtonian and non - Newtonian liquids with power - law shear thinning indices spanning 0.5 to 1 were prepared and were carefully characterized. Streak photography and laser Doppler velocimetry were used to explore the effect of fluid rheology and inertia on the flow transitions. In particular, the detailed flow patterns and the onset of asymmetric flows in the symmetric geometry were compared for the difl‘erent fluids. A continuation method which used geometric perturbations was developed to analyze the flow bifurcation for different expansion ratios and fluid rheology. Experimental results with the 1:16 channel revealed that in Newtonian liquids, the onset of asymmetric flow occurred at a critical Reynolds number of 0.8, which is significantly lower than that reported for Newtonian flow through planar channels with expansion ratio of 2 and 3. Increasing pseudOplasticity delayed the onset of the flow transitions but resulted in a higher degree of asymmetry and a longer flow length up to which asymmetry persisted. An unexpected flow transition involving the simultaneous presence of three vortices close to the plane of expansion was observed with the shear thinning liquid. Sanjay B. Mishra Computations predicted the trends of delayed bifurcation with increased shear thinning. Results of computations also showed that the onset of asymmetry occurred at much lower Reynolds number with a high expansion ratio. The Newtonian vortex length prior to the onset of asymmetry was related to the expansion ratio and the Reynolds number. The present study will find applications in many processes which involve flow of shear thinning fluids through expansions such as the extrusion of food materials through dies. ACKNOWLEDGMENTS I am very thankful to my advisor, Dr. K. Jayaraman, for his steadfast support, continuous guidance, patience and understanding, particularly during some of my rougher times. I also thank my committee members - Drs. Charles Petty, John McGrath and William Pratt - who devoted considerable time toward my dissertation. Mike and Terry at the DER machine shop ofien went out of their way to help me complete the seemingly endless task of perfecting the flow configuration that I used so exhaustively in my experiments. The ever - smiling, never - refirsing stafl‘ in the omce - Julie, Candy and Faith really made administrative matters very simple. Thank you all! I thank all my co - workers especially Ashim, Doug and Himanshu, who lent me support whenever I needed it. Friends in my personal life - Venky, Shanti, Uma, Naresh and many others helped me in numerous ways. It will be very difficult to find such a good bunch of buddies. My parents were a constant source of inspiration and motivation. They inspired me to put my best efforts in everything I do in life. I have a lot to thank them for. Finally, this work would never have been completed without the strong support and encouragement of my wife Lata. She made life at home so relaxing that I was always fresh to tackle the problems in grad school. Her contribution to my dissertation is really invaluable. iv TABLE OF CONTENTS LIST OF TABLES ............................................................................................................ viii LIST OF FIGURES ............................................................................................................. ix CHAPTER 1 INTRODUCTION ............................................................................... : ............................... 1 1. Definitions ............................................................................................................ 1 2. Interaction of inertia, elasticity, extensional viscosity and pseudoplastic behavior .......................................................................................................... 3 3. Review of previous work done .............................................................................. S 3.1 Contraction flows .................................................................................... 6 3.2 Expansion flows .................................................................................... 1 1 3.2.1 Experimental results ................................................................ 11 3.2.1.1 Flow transitions due to inertia in Newtonian flow through planar expansions ............................ 11 3.2.1.2 Non - Newtonian flow through expansions ................ 16 3.2.2 Computational results in planar expansions .............................. 19 4. Objectives ........................................................................................................... 23 CHAPTER 2 FLOW VISUALIZATION OF THE ASYlvflWETRIC FLOW TRANSITIONS IN AN ABRUPT PLANAR EXPANSION ........................................................................ 26 1. Introduction ........................................................................................................ 26 2. Backgron ........................................................................................................ 27 2.1 Contraction flows vs Expansion flows .................................................... 27 2.2 Efl‘ect of geometry - Axisymmetric vs Planar .......................................... 29 2.3 Flow transitions due to inertia in Newtonian flow through planar expansions .............................................................................. 30 2.4 Experimental work on Non - Newtonian flows through expansions ........ 32 2.5 Vortex grth prior to the onset of asymmetry ...................................... 34 3. Objectives ........................................................................................................... 34 4. Experimental ....................................................................................................... 36 4.1 Model flow cell ...................................................................................... 36 4.2 Model fluids .......................................................................................... 39 4.3 Flow visualization setup ......................................................................... 47 V 5. Results and Discussion ........................................................................................ 50 5.1 Flow patterns in the Newtonian liquid (Experimental) ............................ 50 5.2 Computations of the flow bifirrcation in Newtonian liquids ..................... 55 5.3 Newtonian vortex growth prior to the onset of asymmetry ..................... 64 5.4 Flow patterns in the shear thinning liquids (Experimental) ...................... 72 5.5 Flow bifurcation in the non - Newtonian liquids ..................................... 77 5.6 Computed vortex growth in non - Newtonian liquids prior to the onset of asymmetry ........................................................................... 80 6. Conclusions ........................................................................................................ 85 CHAPTER 3 LDV MEASUREMENTS OF NEWTONIAN AND NON- NEWTONIAN LIQUIDS 1N ABRUPT PLANAR EXPANSIONS ............................................................. 88 1. Experimental ....................................................................................................... 88 1.1 Laser Doppler velocimetry ..................................................................... 88 1.2 Optical setup ......................................................................................... 90 2. Results and Discussion ........................................................................................ 93 2.1 Velocity profiles of the Newtonian liquids ............................................... 95 2.2 Velocity measurements of the shear thinning liquids (n = 0.7 and n = 0.5) .......................................................................................... 105 2.3 Quantification of the degree of asymmetry ........................................... 124 2.4 Bifirrcation curves fi'om the experiments .............................................. 125 3. Computations of flow bifirrcations ..................................................................... 130 3.1 Computed predictions ofthe decay offlow asymmetry 133 3.2 Velocity profiles from the perturbation - continuation approach ........... 136 3.3 Comparison of experimental and computed bifurcation curves ............. 139 4. Conclusions ....................................................................................................... 142 CHAPTER 4 COMPUTATIONS OF SYMMETRY BREAKING FLOW BIFURCATIONS IN ABRUPT PLANAR EXPANSIONS ........................................................................... 147 1. Introduction ...................................................................................................... 147 2. Background ...................................................................................................... 147 2.1 Newtonian flow transitions in an abmpt planar expansion ..................... 147 2.1.1 Existing experimental results ................................................. 147 2.1.2 Prediction of Newtonian flow bifiircation using computations .................................................................... 150 2.2 Non - Newtonian flow through expansions ........................................... 154 3. Objectives ......................................................................................................... 156 4. Numerical scheme ............................................................................................. 157 4.1 Problem definition ................................................................................ 157 4.1.1 Scaled variables ..................................................................... 159 4.1.2. Boundary conditions ............................................................ 159 4.2 Perturbation - Continuation approach .................................................. 160 vi 4.3 finite elements grids ............................................................................ 164 5. Results and Discussion ...................................................................................... 165 5.1 Flow bifurcation in expansion flows ..................................................... 165 5.1.1 Validation of the perturbation - continuation approach .......... 165 5.1.2 Use of the perturbation approach to study Newtonian flow bifirrcationsina 1:16 channel ................................... 171 5.1.3 Effect of non - Newtonian behavior on flow bifurcation in a 1:16 planar expansion .............................. 174 5.2 Flow patterns during transitions in planar expansions ........................... 178 5.2.1 Newtonian liquids .................................................................. 178 5.2.2 Shear thinning liquid .............................................................. 180 5.3 Velocity profiles in planar expansions ................................................... 183 5.3.1 Velocity profiles in the Newtonian liquid before and after the onset of asymmetry ............................................ 183 5.3.2 Velocity profiles in shear thinning liquid P1 through a 1:16 planar expansion ................................................... 188 5.4 Efl‘ect of expansion ratio and rheology on the excess pressure difi‘erence during flow through expansions ...................................... 188 5.5 Effect of expansion ratio and rheology on the flow resistance ............... 198 6. Conclusions ....................................................................................................... 202 CHAPTER 5 CONCLUSIONS AND RECONflVIENDATIONS FOR'FUTURE STUDY ..................... 207 l. 1 Conclusions ......................................................................................... 207 1.2 Recommendations for fixture work ....................................................... 213 APPENDIX A COMPARISON OF ABRUPT EXPANSION FLOW WITH JEFFERY - HAMEL FLOW .............................................................................................................................. 214 LIST OF REFERENCES ................................................................................................. 221 vii LIST OF TABLES Table 2.1 - Model fluids used ............................................................................................... 40 Table 2.2-Parametersusedintheshearviscositymodels .................................................... 43 Table 2.3 -Fitting constantsusedinFigures 2.15, 2.16 and 2.17 .......................................... 72 Table 3.1 - Description of the components depicted in Figure 3.1 ........................................ 92 Table 4.1 Parameters used in the viscosity models .............................................................. 175 viii LIST OF FIGURES Figure 1.1 Schematic of flow through expansions or contractions ..................................... 2 Figure 1.2a Vortices in contraction / expansion flows ............................................................ 4 Figure 1.2b Asymmetrical flow profile in a planar expansion .................................................. 4 Figure 1.3 Vortex length in a 4:1 axisymrnetric contraction (Boger et al., 1986) ..................... 8 Figure 1.4 Flow patterns with water through a 1:3 planar expansion (Sobey, 1985). (a)Re=55(b)Re=115 ..................................................................................................... 12 Figure 1.5 Vortex asymmetry in a Newtonian liquid through a 1:3 planar expansion (Sobey, 1985) ...................................................................................................... 13 Figure 1.6 Effect of aspect ratio and expansion ratio on the flow transition in Newtonian flow (Cherdron et al., 1978) ............................................................................... 15 Figure 1.7 Flow configuration used by Townsend and Walters (1994) .................................. 18 Figure 2.1 Design of the model flow cell .............................................................................. 37 Figure 2.2 Characteristic dimensions of the model flow cell .................................................. 38 Figure 2.3 Efi'ect of Methocel concentration on the viscosity of the polymer solutions ......... 42 Figure 2.4 Shear viscosity of the polymer solutions .............................................................. 44 Figure 2.5 Loss modulus and storage modulus of the polymer solutions ............................... 46 Figure 2.6 Flow visualization setup ..................................................................................... 48 Figure 2.7a Scanning mirror assembly for creating a laser sheet ............................................ 49 figure2.7bLasersheetcreationwithaglassrod ................................................................. 49 ix Figure 2.8 Flow patterns of the Newtonian liquid. (a) Re = 0.001 (b) Re = 0 ........................ 52 Figure 2.8 Flow patterns of the Newtonian liquid (continued). (c)Re=0.5 (d)Re=0.8 ..................................................................................................... 53 Figure 2.8 Flow patterns of the Newtonian liquid (continued). (e)Re=1.5(t)Re=4 ..................................................................................................... 54 Figure 2.9 Experimental vortex growth in the Newtonian liquid ........................................... 56 Figure 2.10 Schematic of the flow channel used in calculations ........................................... 57 Figure 2.11 Results from the perturbation - continuation approach for Newtonian flow through a 1:3 planar expansion ................................................................... 60 Figure 2.12 Effect of grid refinement on bifirrcation curve. Newtonian flow, Expansion ratio = 3 ............................................................................................................. 62 Figure 2.13 Bifirrcation curve for the 1: 16 expansion ........................................................... 63 Figure 2.14 Positive halfof the bifurcation curve for Newtonian flow .................................. 65 Figure 2.15 Experimental Newtonian vortex growth prior to the onset of asymmetry. Solid line is from computation ........................................................................... 66 Figure 2.16 Newtonian vortex growth prior to the onset of asymmetry at high Reynolds numbers. Lines are fits using equation (2.9) .......................................................... 70 Figure 2.17 Newtonian ortex growth prior to the onset of asymmetry at low Reynolds numbers. Lines are fits using equation (2.9) ................................................... 71 Figure 2.18 Flow patterns of the polymer solution P1. (a) Re" = 1.25 (b) Re“ = 1.9 ................................................................................................ 73 Figure 2.18 Flow patterns of the polymer solution P1 (continued). (c) Re“ = 1.25 ((1) Re“ = 1.9 ............................................................................................... 74 Figure 2.19 Experimental vortex growth in the polymer solutions ........................................ 76 Figure 2.20 Predicted bifurcation curve for shear thinning liquid P1 ..................................... 79 Figure 2.21 Vortex growth in polymer solution P1. Solid line is fi'om computation .............. 81 Figure 2.22 Vortex growth observed in P2. Solid line is from computation .......................... 82 Figure 2.23 Vortex growth before the onset of asymmetry, n = 0.7 ...................................... 83 Figure 2.24 Vortex growth before the onset of asymmetry, n = 0.5 ...................................... 84 Figure 2.25 Efi'ect of shear thinning on the creeping flow vortex length ................................ 86 Figure 3.1 Schematic of the LDV setup ............................................................................... 91 Figure 3.2 Nomenclature used to describe the LDV experiments .......................................... 94 Figure 3.3 Fully developed velocity profile of the Newtonian liquid at X = 15. Solid line is the plane Poiseuille flow .................................................................................... 97 Figure 3.4 Symmetrical axial velocity profiles of the Newtonian liquid at Re = 0.6 ............. 98 Figure 3.5 Newtonian velocity profiles after the onset of asymmetry, Re = 1.5 ..................... 99 Figure 3.6 Newtonian velocity profiles afier the onset of asymmetry, Re = 2. 5 ................... 101 Figure 3.7 Newtonian velocity profiles alter the onset of asymmetry, Re = 3 .5 .................. 102 Figure 3.8 Newtonian velocity profiles close to the expansion plane; X = 1 ........................ 103 Figure 3.9 Newtonian velocity profiles at X = 8 ............ ' .................................................... 1 04 Figure 3.10 Infared transverse flow of the Newtonian liquid ............................................ 106 Figure 3.11 Fully developed velocity profile of the 1% shear thinning liquid at X = 45 ........................................................................................................................... 108 Figure 3.12 Velocity profiles of P1 at various axial locations before the transition Re“ = l ............................................................................................................. 109 Figure 3.13 Velocity profiles ofPl afierthe onset ofasymmetry. Re“ =2.0 ....................... 110 Figure 3.14 Velocity profiles ofPl afierthe onset ofasymmetry. Re“ =2.5 ....................... 112 Figure 3.15 VelocityprofilesofPl afiertheonset ofasymmetry.Re* =3.0 ....................... 113 Figure 3.16 Presence of two vortices in the shear thinning liquid close to Y=-l.Re*=2.5,X=1 ................................................................................................... 114 Figure 3.17 Effect of shear thinning on the velocity profiles at Reynolds number = 2.5; X = l .......................................................................................................... 1 16 Figure 3.18 Effect of shear thinning on the velocity profiles at Reynolds number = 2.5; X = 8 .......................................................................................................... 1 17 Figure 3.19 Velocity profiles ofshearthinningliquid P1 atX= 1 ...................................... 119 Figure 3.20 Velocity profiles of shear thinning liquid Pl at X = 8 ....................................... 120 Figure 3.21 Velocity profiles ofshear thinning liquid P1 atX= l6 ..................................... 121 Figure 3.22 Inferred transverse flow in shear thinning liquid P1 ......................................... 122 Figure 3.23 Symmetric velocity profiles of P2 at Re“ = 1.5 ............................................... 123 Figure 3 .24 Growth of asymmetry with the Reynolds number in the Newtonian liquid ............................................................................................................... 126 Figure 3.25 Growth of asymmetry with the Reynolds number in the shear thinning liquid P1 ...................................................................................................... 127 Figure 3.26 Decay of asymmetry in the Newtonian liquid, with increasing flow length ....................................................................................................................... 128 Figure 3.27 Decay of asymmetry in the shear thinning liquid, with increasing flow length ........................................................................................................................ 129 Figure 3.28 Bifirrcation curve for the Newtonian liquid N .................................................. 131 Figure 3.29 Bifurcation curve for the shear thinning liquid P1 ............................................ 132 Figure 3.30 Computed decay of asymmetry in the Newtonian liquid ................................... 134 Figure 3.31 Computed decay ofasymmetryinthe shearthirming liquid .............................. 135 Figure 3.32 Computed velocity profiles of the Newtonian liquid at Re = 8 ......................... 137 Figure 3.33 Computed velocity profiles of the Newtonian liquid at Re = 25.3 ..................... 138 Figure 3.34 Computed velocity profiles of the shear thinning liquid P1 at Re“ = 20 ............ 140 Figure 3.35 Computed velocity profiles of the shear thinning liquid P1 at Re“ = 44.3 ......... 141 Figure 3.36 Comparison of the degree of asymmetry from LDV experiments with that from the FEM computations for Newtonian flow ................................................. 143 Figure 3.37 Degree of asymmetry for the polymer solution Pl ........................................... 144 xii Figure 4.1 Schematic of the flow channel used in calculations ............................................ 158 Figure 4.2a Schematic of the continuation - perturbation approach ..................................... 161 Figure 4.2b Steps involved in the continuation approach .................................................... 163 Figure 4.3 Efl‘ect of grid refinement on bifirrcation curve. Newtonian flow, Expansion ratio = 3 ............................................................................................................ 166 Figure 4.4 Demonstration of the results using the perturbation - continuation approach for Newtonian flow through a l :3 planar expansion ............................................ 167 Figure 4.5 Bifurcation curve for a Newtonian liquid in a 1:2 expansion .............................. 169 Figure 4.6 Bifurcation curve using center - line velocity as the degree of asymmetry for a Newtonian liquid through a 1:2 expansion ............................................ 170 Figure 4.7 Bifurcation curve for Newtonian flow in a 1:16 expansion ................................ 172 Figure 4.8 Effect of geometrical asymmetry on Newtonian flow bifirrcationinalzl6channel .............................................................................................. 173 Figure 4.9 Bifirrcation curve for n = 0.7, B = 16 ................................................................. 176 Figure 4.10 Bifurcation curve forn=0.5, B =16 ............................................................. 177 Figure 4.11 Flow transitions of a Newtonian liquid in a l :2 expansion ................................ 179 Figure 4.12 Flow transitions of the Newtonian liquid in a 1 :16 expansion ........................... 181 Figure4.13 Flowtransitionsofthe shearthinning liquid P1 ina 1:16 channel .................... 182 Figure 4.14 Velocity profiles prior to the onset ofasymmetry. B = 3, Re = 26 ................... 184 Figure4.15Velocityprofilesafiertheonsetofasymmetry. B=3,Re=34 ........................ 185 Figure 4.16 Computed velocity profiles with Newtonian liquid at Re = 8 ............................ 186 Figure 4.17 Computed velocity profiles with Newtonian liquid at Re = 25.3 ....................... 187 Figure 4.18 Computed velocity profiles of the shear thinning liquid P1 at Re" = 20 ........................................................................................................................ 189 xiii Figure 4.19 Computed velocity profiles of the shear thinning liquid P1 at Re" = 44.3 ..................................................................................................................... 190 Figure 4.20 Efl‘ect of expansion on excess pressure difference in Newtonian flow ............... 192 Figure 4.21 Normalized excess pressure difference in Newtonian flow ............................... 195 Figure 4.22 Efl‘ect of pseudoplasticity on excess pressure difference, B = 16 ..................... 196 Figure 4.23 Excess pressure difl‘erence in shear thinning liquid, n = 0.7 .............................. 197 Figure4.24lncreaseinflowresistanceatcritical Re. B=3, n=1 ..................................... 199 Figure 4.25 Increase in flow resistance at critical Re. B = 16, n = 1 ................................... 200 Figure 4.26 Drop in flow resistance due to expansion; Newtonian flow .............................. 201 Figure 4.27 Efl’ect of pseudoplasticity on flow resistance. B = 16 ...................................... 203 Figure 4.28 Efl‘ect of pseudoplasticity on flow resistance in a 1:2 channel ........................... 204 Figure 4.29 Flow resistance in a 1:3 channel ...................................................................... 205 Figure 5.1 Three parameter plot summarizing the efl‘ect of inertia, rheology and expansion ratio on the occurrence of flow transitions ................................................... 212 Figure A.1 Comparison ofvelocity profilewithJHflow. X= 1,Re=1 .............................. 217 Figure A2 Comparison of channel velocity with JH flow, Re = 1 ....................................... 218 FigureA3 Comparisonofvelocityprofilesatx= 1,Re=2 .............................................. 219 Figure A4 Comparison of channel velocity with 1H flow, Re = 2 ..................................... 220 xiv Chapter 1 INTRODUCTION Flow of fluids through converging and/or diverging geometries is very commonly encountered in various engineering operations. Flow through orifices, valves and pipe joints involves flow separations and local recirculations, which have an important impact on the transfer of heat, mass and momentum. Separation flows in expansions result in advantages such as reduction in pressure losses and disadvantages like reduction in the transfer rate. Other examples of diverging / converging flows include the flow of a resin through a fiber bed, which is a complex network of contraction and expansion regions, flow of body fluids through veins and arteries, etc. Very often the flow is made even more complicated by the fluids shear thinning viscosity, visooelasticity or extensional viscosity. Extrusion of shear thinning foods through dies of various shapes is one such operation. 1. Definitions Flow through contractions or expansions is schematically shown in Figure 1.1. Flow occurs around two corners - the salient (or 90°) comer and the non re—entrant (or lip or 270°) comer. Unless otherwise mentioned, the term “vortex" will be used to address the salient corner vortex in this document. The vortex is measured in terms of the reattachment length or vortex length (L,,). The ratio of the cross sectional areas of the two sections (B) is termed as the expansion (or contraction) ratio. If the sections are circular, I I... Salient corner ‘\ ¢< \ > “I Lip corner \ 7 Figure 1.1 Schematic of flow through expansions or contractions 3 the geometry is referred to as axisymmetric whereas rectangular sections (channels) make the geometry planar. 2. Interaction of inertia, elasticity, extensional viscosity and pseudoplastic behavior In the study of flow through contractions and expansions, the flow features of interest include (a) salient comer vortices (b) lip corner vortices and O symmetric to asymmetric flow transitions. Figure 1.2 illustrates these schematically. The salient corner vortices have been the most commonly reported flow feature in any study involving converging or diverging flows. It has now been conclusively proved, at least for Newtonian fluids, that these vortices do exist even at very low Reynolds numbers (Mofi‘att, 1964). Visualization of these depend on the resolution of the experiment. Lip vortices are believed to arise in viscoelastic solutions only, although the computations of Baloch et a]. (1995) predict their presence in Newtonian liquids flowing through a 1:80 planar expansion. In Newtonian liquids flowing through abrupt planar expansions, the transition fi'om a symmetric to an asymmetric flow pattern has been shown to occur at high Reynolds numbers (Cherdron et al., 1978, Sobey, 1985, Fearn et al., 1990 and Durst et al., 1993, flowing through abrupt planar expansions. The factors affecting these flow features include inertia, elasticity, extensional viscosity and pseudoplasticity. Results from experiments with Newtonian liquids can isolate the contribution of inertia to these flow features. Elasticity and pseudoplasticity have similar effects on the grth of the salient corner vortices, both in expansions and contractions. Hence, experiments with inelastic shear thinning polymer solutions and elastic non-shear thinning polymer solutions are needed to clearly identify the efl'ects of pseudoplasticity and elasticity on the growth of the salient corner vortices. Salient cornervortex i / Lip corner vortex 7 Figure 1.2a Vortices in contraction l expansion flows /\\\ Figure 1.2b Asymmetrical flow profile in a planar expansion 5 The importance of extensional viscosity on the occurrence of lip vortices has been shown by Boger and co-workers (1986, 1994) in a 4:1 axisymmetric contraction, where a solution with higher extensional viscosity was observed to produce lip vortices, a feature not seen in the polymer solution with lower extensional viscosity but similar shear and dynamic properties. Thus, solutions clearly delineating the efl‘ects of inertia, elasticity, pseudoplasticity and extensional viscosity need to be carefully prepared and characterized to evaluate the flow patterns through contractions or expansions. The present work attempts to study the effect of inertia and pseudoplasticity on the flow patterns through planar expansions with high expansion ratios. 3. Review of previous work done During the last two decades, considerable attention has been focused on the flow of polymer solutions and melts through geometries with abrupt changes in cross section, with more emphasis on contraction flows. A variety of interesting flow characteristics have been observed in converging flows (Nguyen and Boger, 1978, Walters and Rawlinson, 1982, Boger et a1, 1986, Lawson et al., 1986, Evans and Walters, 1986, McKinley et al., 1991, Chiba et al., 1992,1995, Quinzani et al., 1995) leading researchers to devote more attention to contraction flows than to expansion flows. It should be pointed out that only in the case of creeping flow of Newtonian liquids will the flow features in an expansion be a mirror-image of that in a contraction flow. This is so because flow of polymers is governed by non-linear equations with the nonlinearities appearing due to presence of inertial terms, a shear rate dependent viscosity or polymeric contributions to the stress 6 tensor. Hence, no direct inference for polymers flowing through expansions can be made based on corresponding contraction flow results. 3.1 Contraction flows Although the focus of the present work is on planar expansion flows, a description of contraction flows has been included here for completeness. Axisymmetric contractions have so far been the favored configuration to be studied, both in experiments and computations. Experiments with Newtonian liquids through such geometries have indicated that inertia decreases the salient comer vortex size (i.e. reduces L,,) irrespective of the contraction ratio (Boger et al., 1986, Abdul-Karem et al., 1993). When the vortex length is normalized by the upstream section diameter, the value obtained for creeping flow (Reynolds number < 0.1) is 0.18. This has been verified computationally by Christiansen et a1. (1972) and Vrentas and Duda (1973). The effect of elasticity on the flow in axisymmetric contractions has been studied extensively by Boger and co-workers and Armstrong and co-workers. Boger et a1. (1986) have concluded that characterization of the polymer solutions based on the steady and the dynamic shear properties is not sufficient to explain the differences in flow behaviors of elastic solutions through axisymmetric contractions. They have reported that differences in the extensional viscosity of the polymer solutions may lead to completely difl‘erent flow features. To demonstrate this, they chose two polymer solutions (now called Boger fluids) - a 0.4% solution of polyacrylarnide (PAA) in water and corn syrup and a 0.1% polyisobutylene (PIB) solution in kerosene and polybutene. These fluids are constant, high-viscosity fluids with a high 7 degree of elasticity. The efl’ect of elasticity in absence of inertia and shear thinning in any type of flow may be evaluated using the Boger fluids. Although both these solutions have similar steady and dynamic shear properties, the PIB solution has a higher extensional viscosity than the PAA solution. While flowing through a 4:1 axisymmetric contraction, the PAA solution showed a vortex enhancement beyond a Deborah number (De) of 1, where Deborah number is defined as the ratio of a characteristic fluid time to a characteristic flow time. De=ly Here A is the relaxation time of the fluid and y is the wall shear rate in the downstream section. De is a measure of the elasticity of the solution and is increased by increasing the flow rate in experiments. For an increase in De fi'om 1 to 5, the normalized vortex length with the PAA solution increased from 0.2 to 0.65. The PIB solution through the very same geometry, showed a vortex of length 0.2 (the Newtonian, creeping flow value) until a De of about 1.6 and then reduced to almost zero at higher De. At around De of 2, vortices were observed on the lip corners. These grew in size as the flow rate was increased. For De between 2 and 2.2 both the vortices coexisted. This efl‘ect is summarized in Figure 1.3. As the contraction ratio was increased from 4 to 16, it was observed that both the fluids behaved in the same fashion i.e. like the PAA solution in a 4:1 contraction. These observations proved that the contraction ratio was also an important parameter in evaluating the flow patterns. More importantly, this work also brought out (probably for the first time) the importance of extensional properties of the fluids in entry flows. The solution with the higher extensional viscosity (PIB) showed a 0 PAA/Corners» (n - 0'96) 08 . 4 P18! Poiybutens (n I 099) ‘ I I I I - Lip vortex growth. or . O 05 - «l o-si- J! 0.4.. i 0' 0'3 - / 62- /°/ \ l Figure 1.3 Vortex length in a 4:1 axisymmetric contraction (Boger et al., 1986). 9 reduction in the salient corner vortex length and an enhancement in the lip corner vortices with elasticity. The PAA solution exhibited an enhancement of salient comer vortices with no lip vortices at all. Boger and Binnington (1994) have mentioned that a "true" comparison of elastic efi‘ects needs the Deborah numbers to be evaluated using a shear rate dependent relaxation time and not a constant, zero-shear relaxation time as used by Boger et a1. (1986). Thus, to study elastic effects regardless of the geometry used, both shear and extensional properties of the fluids are essential. Further, a priori assumption about the effect of the area ratio on the vortices based on results obtained using difl‘erent fluids might lead to incorrect conclusions. Similar results with the PIB Boger fluids have been presented by Lawson et al. (1986). McKinley et a1. (1991) have reproduced the lip vortices in the PIB Boger solution through a 4:1 contraction. In addition, they have shown that as De is increased beyond 2, the lip vortices expand outward toward the 90° comer, until flow instability leads to periodic oscillations of the large vortices. This time- dependent, 3-dimensional flow near the contraction lip is observed only between contraction ratios of 2 to 5 and flow remains steady for higher contraction ratios. At very high De (~ 15), flow becomes aperiodic. A shear thinning, elastic liquid (1.5% PAA in aqueous corn syrup solution) has been observed to enhance vortex growth (Boger et al., 1986) in a 4:1 contraction. The range of De beyond which flow becomes unstable is also increased. Shear thinning, thus, seems to have a stabilizing effect on the flow patterns produced in an axisymmetric contraction. 10 The fluid rheology and contraction ratio are not the only important parameters in determining the flow behavior in complex geometries. The mode of contraction, i.e. planar or axisymmetric assumes significance too. Walters and Rawlinson (1982) have shown that the vortex size decreases with increasing inertia in a 13.3:1 planar contraction (from a square channel to a slit) for a Newtonian liquid. Boger fluids (aqueous PAA solutions) which show vortex enhancement in axisymmetric contraction, show very small or no vortices even at very high flow rates. A 80:1 planar contraction was needed by Evans and Walters (1986) to observe lip vortices. With 1-2% aqueous PAA solutions (shear thinning, elastic), a considerable increase in the vortex size was observed with increase in the flow rate. These solutions exhibited lip vortices in a 16:1 planar contraction. Recently Chiba et a1. (1992,1995) have reported flow instabilities in a 0.1% PAA solution through a 5:1 planar contraction. At high flow rates, the salient corner vortices were observed to grow and decay alternately, giving an impression of a moving bundle along the width of the flow cell. Effect of shear thinning on such flow instabilities has not been reported. Based on all the existing data on contraction flows, White et al. (1987) in their review on entry flows mention that vortex growth in general, is more readily observed in axisymmetric contractions than in planar contractions. A possible explanation of this may be obtained from the work by James and Saringer (1980, 1982) wherein they measured the pressure drop for flow of polyethylene oxide solution through axisymmetric and planar orifices. Since flow through an orifice is essentially shear-flee, the pressure dr0p gives a relative measure of the extensional stress in the contraction region. The pressure drop in the axisymmetric case was several times higher than in the planar case leading to the 11 conclusion that large extensional stresses are developed in axisymmetric flow as compared to planar flow. Since vortices are a means for the fluid to relieve stress, it would be expected that larger vortices would be formed in axisymmetric configurations at essentially similar flow conditions. 3.2 Expansion flows 3.2.1 Experimental results 3.2.1.1 Flow transitions due to inertia in Newtonian flow through planar expansions Sobey (1985) has studied the flow patterns developed in a Newtonian liquid (water) flowing steadily through a 1:3 two-dimensional planar expansion. He observed that at low flow rates (or low Reynolds number, Re, defined using the smaller channel half height and the average velocity in the upstream channel), the corner vortices were symmetric and that they increased in size as Re was increased. Beyond a certain critical Re (around 25 for an abruptly expanding channel), flow became asymmetric and one vortex grew more rapidly than the other. This is shown in Figures 1.4 and 1.5. As Re was raised firrther, a third recirculation region far downstream of the expansion plane and on the wall with the smaller corner vortex was observed too. The critical Reynolds. number for the onset of the flow transitions was observed to be higher for channels with gradual expansions. By using long rectangular channels of large aspect ratios (5 and above) Sobey and others have ensured that the flow far away from the expansion plane is one dimensional. Experiments showing similar flow transitions in Newtonian fluids through abrupt expansions in 1:2 and 1:3 channels have been reported by Durst et al. (1974) and Cherdron et al. (1978) and confirmed later by Feam et al. (1990) and Durst et al. (1993). The phenomenon wherein 12 Figure 1.4 Flow patterns with water through a 1:3 planar expansion (Sobey, 1985). (a) Re = 55 (b) Re = 115. 13 5.6 LJD 0.8 Figure 1.5 Vortex asymmetry in a Newtonian liquid through a 1:3 planar expansion (Sobey, 1985). l4 flow transitions lead to difl‘erences in the flow patterns beyond a certain critical Reynolds number is commonly referred to as “flow bifurcation” and the critical Reynolds number is ofien called the bifurcation point. Cherdron et al. (1978) have investigated the efl‘ect of the expansion ratio and the aspect ratio (ratio of the ‘width of the channel to its height) on the flow patterns developed in a Newtonian liquid flowing through a planar expansion. They have reported that the critical Re at which flow transitions occur goes down with an increase in the expansion ratio as well as an increase in the aspect ratio (see Figure 1.6). For example, with a channel of aspect ratio 8, the critical Re goes down from about 150 to 30 in going from an area expansion ratio of 1 :2 to 1 :3. The mechanism of initiation of such flow transitions, even for Newtonian liquids, is not well understood. However, the Coanda effect does seem to explain how it is sustained. Flow asymmetry is a result of the momentum transfer in the direction normal to flow between the shear layers. As a result, the boundary layer adjacent to one wall is richer in momentum and consequently at a lower pressure as compared to the other. A transverse pressure gradient in the channel is created and as more liquid enters, flow of the liquid from the wall at higher pressure to that at the lower pressure takes place. This increases the momentum at the already richer wall even more, resulting in a more pronounced effect of the flow asymmetry. Interestingly, no flow asymmetry has been reported in axisymmetric expansions. In such configurations, flow induces concentric shear layers, as opposed to the stacked shear layers in planar flow. This provides a continuity all along the plane of expansion in the former, preventing any occurrence of asymmetrical flow patterns. .32: :1 a 3:55. E... 2.8.52 a. .3225. 33. a... .3 eta.— ..eiiafi can eta.— 325. he tuba w; 8:»...— ou— 5. an 3. a Av/ _ 5.34 5.3 5.344 Q/Ezm Q T .. v /1... .. S 3. 23— .23... 33. nae...— _ @— open roodsv 16 Although trends between the flow transitions occurring in expansion channels are available now, all the existing results are limited to low expansion ratios of 2 and 3. Experiments with large expansion ratios will help to answer questions like what happens to the flow patterns at much higher expansion ratios and what is the rate of fall of the critical flow rate (or an equivalent critical Reynolds number) when extreme expansion ratios are involved? 3.2.1.2 Non - Newtonian flow through expansions Abdul-Karem et al., (1993) have investigated flow behavior of 0.05% polyacrylarnide solution in glucose syrup (Boger fluid) through a 1:6.8 axisymmetric expansion and a 6.8:] axisymmetric contraction. Although the vortex size observed in expansions was lower than that in contractions, the trend of vortex enhancement with increasing flow rate was observed in the expansion flow too. No lip vortices or instabilities were observed in either configuration. Halmos et al. (1975) have conducted experiments using aqueous carboxymethyl cellulose solution (inelastic, shear thinning power-law index of 0.73) in a 1:2 abrupt axisymmetric expansion. They have measured the radial and axial velocity profiles downstream of the expansion plane using flash photography. Their experimental results on velocity profiles and reattachment lengths agree well with their calculations for Reynolds numbers between 11 to 125. The authors do not observe any flow asymmetries, oscillations or lip vortices. 17 Townsend and Walters (1994) have studied the flow of a 0.15% aqueous solution of polyacrylamide (slightly shear thinning, strongly elastic) through an expansion from a square section to a rectangular slit (area expansion of 13.3) and fi'om the rectangular slit to another square section (area expansion of 13.3). A schematic of the geometry used by them is shown in Figure 1.7. With a Newtonian liquid, significant vortex activity was observed due to fluid inertia. The vortex size increased with the flow rate. The polymer solution, on the other hand, produced small comer vortices, the size of which decreased with the flow rate. Fluid elasticity thus, was observed to inhibit vortex growth. It should be pointed out that their study with Newtonian liquids has not shown any evidence of flow asymmetry, in contrast to those reported by Durst et al. (1974), Cherdron et al. (1978), Sobey (1985) and Feam et al. (1990), despite a wide range of Reynolds numbers used. The square channels used by Townsend and Walters (1994) approximate axisymmetric flow which has never been known to show the flow asymmetry mentioned above. In addition, based on the findings of Cherdron et al. (1978) that the critical Reynolds number for the onset of flow asymmetry increases with decreasing channel aspect ratio, one might conclude that at an aspect ratio of 1, flow asymmetry might be observed, if at all, only at very high Reynolds numbers. One notable contribution of the Townsend and Walters work was to clearly bring out the effect of fluid elasticity on the vortex growth in planar expansions. The observed trends in the effects of fluid inertia and elasticity on secondary flows was in contrast to what had been observed in various contraction geometries, where fluid inertia reduced the vortex size while elasticity led to vortex enhancement. This reversal of roles may be the reason for lack of further investigation of viscoelastic efl‘ects in expansion flows. 18 Flow A\ Ky \/ Figure 1.7 Flow configuration used by Townsend and Walters (1994). l9 Conspicuous by its absence from literature is any indication whether non - Newtonian flows will show flow bifurcation at high Reynolds numbers. If they indeed do so, the effect of fluid rheology on the bifurcation point and on the flow patterns created needs to be studied. 3.2.2. Computational results in planar expansions Various numerical procedures have been used to predict the flow bifiircation in a planar sudden expansion. Computations involving finite elements have always needed some kind of perturbation - either to the geometry or to the boundary conditions - to yield a bifirrcated flow structure. Durst et al. (1993) have made transient calculations to predict the onset of flow transitions for a Newtonian liquid. They followed a perturbation approach which involved the following steps: At time t = 0, a fully developed velocity profile was imposed at the inlet of the smaller channel. After n time iterations and during m time iterations, the inlet velocity conditions were modified such that the axial velocity component (U) was a firnction of time and the normal velocity component (V) was a firnction of both time and space. Subsequently, the original symmetric firlly developed velocity profile was restored as the inlet boundary condition. The solution was allowed to achieve steady state. Using this approach a critical Reynolds number of 42 was predicted for flow through a 1:2 expansion. 20 F earn et al. (1990) used numerical bifirrcation techniques applied to a finite element discretization of the two - dimensional Navier - Stokes equations and predicted flow bifurcation in a 1:3 planar expansion at Re,l of 27. Their work sheds more light on the sensitivity of the bifurcation point to experimental uncertainties. They suggest that the critical transition point is structurally unstable. The slightest imperfection in the experiment may lead to a discontinuity in the bifurcation curve, with a shift in the original bifirrcation point. They showed that a vertical shift in the grid of the larger channel by 0.42% with respect to the axis of symmetry provided much closer match with the experimental data. Their work seems to explain the possible reason for the scatter observed in the experimental results on flow bifirrcations through planar expansions. Indeed , experimental imperfections could have many sources such as geometrical asymmetry, upstream flow asymmetry, momentary mechanical shock, temperature variation, etc. Teschauer (1994) employed an asymmetric upstream channel to compute the bifurcated branch of the solution for various expansion ratios between 1.5 to 3. A commercial finite element code was used. She predicted critical Reynolds numbers of 72 and 27 for expansion ratios of 2 and 3 respectively. In a difl‘erent flow configuration involving Newtonian flow into a rectangular channel through two symmetric openings, Goodwin and Schowalter (1996) have shown the possibility of the simultaneous existence of numerous solutions beyond a critical Reynolds number. To access the asymmetric solutions, they have followed a continuation approach 21 coupled with a perturbation in the flow rates in the two channels. Using a finite element discretization, solutions with the asymmetrical flow rates were computed for increasing Reynolds numbers. Results at the lower Reynolds numbers were used as initial iterates for computations at higher Reynolds numbers. At significantly high Reynolds numbers, the flow was rebalanced and the same continuation approach was used for successively decreasing Reynolds numbers. Such an approach detected the various asymmetric branches of the solutions. A similar approach using continuation and a perturbation in the geometry to compute the flow bifurcation in planar expansions with a single inlet has been devised in the present work. This will be discussed later in Chapter 4. Very recently numerical results using a finite volume approach for flow through planar expansions have been presented. A striking feature of such an approach is that flow bifirrcation has been computed without providing any kind of perturbation to the flow conditions. Drikakis (1997) has presented bifirrcation curves from several schemes for expansion ratios up to 6. Various numerical schemes based on an overall finite volume approach have been tested. His results for the onset of asymmetry with expansion ratios of 2 and 3 match the corresponding results of Teschauer (1994) and the results fi'om the linear stability analysis of Shapira et al. (1990). Foumeny et al. (1996) have shown that a commercial code, FLUENT, can be effectively utilized to study the flow bifurcations. This code employs a finite volume discretization procedure, in which linear approximation firnctions are used to interpolate values of the flow variables throughout the solution domain. Their focus is on obtaining results ~on channels with more than one inlet opening. 22 A characteristic observation fiom the computational results is that flow bifirrcation calculations almost invariably predict a higher critical Reynolds number than the corresponding value obtained in experiments. This is consistently observed in the work described above on channels with low expansion ratios of 2 and 3. Sobey (1985) and Sobey and Drazin (1986) have attempted to relate the experimentally observed bifirrcation to that in Jeffery - Hamel (JH) flows. In the latter, radial flow occurs between two inclined plates intersecting at an angle 2a. Flow is generated by a source located on the line of intersection. JH flows have been shown to bifurcate subcritically, leading to no stable flow above the critical Reynolds number. Planar expansion flows, on the other hand, display a supercritical bifiircation which is confirmed by several reports of stable asymmetric patterns in planar expansions. Sobey, therefore, concluded that JH flows are not of any significance in explaining expansion flow after bifirrcation. Shapira et al. (1990) have performed a linear stability analysis of flow in symmetric expansions. They have considered a gradual expansion with a constant slope of the channel walls. Although their predictions of Recl = 27.5 for a 1:3 expansion are in agreement with the computational results of F earn et al. (1990), whose computations suggest the onset of asymmetry at Re of 27, they over predict Recl of 72 for a 1:2 expansion. More importantly their computations show that the symmetric branch of the solution obtained above the critical Reynolds number is unstable and therefore unlikely to be ever witnessed in experiments. 23 Alleborn et al. (1997) have performed a linear stability analysis on flows through abrupt expansions. Finite difl'erence approximations of the equations of motion in the stream firnction - vorticity form have been used. The bifirrcation picture is extended by computing the subsequent bifirrcation point (Red) and solution branches. Solutions for infinite expansion ratio have been compared with Jefl'ery - Hamel flow. They conclude that away fiom the expansion plane flow profiles do approach the profiles of JH flow. Computational results on flow bifurcation of Newtonian liquids through planar expansions are limited to low expansion ratios. Further, no results demonstrating the effect of non - Newtonian flow behavior on the flow bifurcations, even for low expansion ratios, are available in literature. 4. Objectives Attempts have been made to fill some of the missing links within the literature for flow through planar expansions. The objectives of the present study are: e To carry out experiments to study the flow transition of Newtonian liquids flowing through planar channels of large expansion ratios. .To compare the flow bifurcation results with those available for low expansion ratios. 24 .To use experimental techniques to explore the efl'ect of non - Newtonian viscosity on the flow bifurcation and on the flow patterns produced by the flow of shear thinning, inelastic liquids through planar expansions with large expansions ratios. .To devise a protocol to compute the flow bifirrcation for Newtonian and non - Newtonian liquids, flowing through planar expansions. .To evaluate the efi‘ect of fluid rheology and expansion ratio on the flow bifurcation of liquids through planar expansions. Model channels have been designed with large aspect and expansion ratios. Newtonian model fluids and inelastic, non-Newtonian model fluids have been prepared and the efl‘ects of fluid rheology and injection rate on the flow patterns have been experimentally investigated using streak photography and laser Doppler velocirnetry. A novel approach to compute the flow bifurcations for Newtonian and non - Newtonian liquids has been devised and then tested for accuracy. Flow bifurcation results using this approach have been presented for Newtonian and non - Newtonian fluids flowing through planar expansions. Following is the organization of the various results in this document: (1) Chapter 2: Critical Reynolds numbers for the onset of flow asymmetry have been identified for the model fluids using streak photography. The detailed flow patterns and 25 flow transitions for the Newtonian and non - Newtonian liquids have been presented. Relationships between the Newtonian vortex length prior to the onset of flow transitions, Reynolds number-and the expansion ratio have been proposed and tested. A brief description of the computations performed to determine the bifurcation curves for Newtonian and non - Newtonian flow through 1:2, 1:3 and 1:16 planar expansions has been included. Flow prior to the onset of asymmetry has been studied in detail for channels with expansion ratios 2, 3 and 16 with Newtonian and inelastic shear - thinning liquids. Experimental and computational results on the trends of vortex growth for non-Newtonian liquids have been compared. (2) Chapter 3: Laser Doppler velocity measurements with both Newtonian and non - Newtonian liquids have been presented. Details of the vortex grth and the decay of asymmetry with axial position have been reported. Flow bifirrcation curves using the center line shear rate as the measure of asymmetry have been generated for the liquids. (4) Chapter 4: The approach developed to compute the flow bifurcation for Newtonian and non - Newtonian liquids has been described in detail. Using this approach, bifirrcation curves, streamlines, velocity profiles, excess pressure difference and flow resistances have been evaluated for fluid shear thinning indices of 0.5, 0.7 and 1 and channel expansion ratios of 2, 3 and 16. (5) Chapter 5: Conclusions from the present study have been listed and recommendations for future work have been made. Chapter 2 FLOW VISUALIZATION OF THE ASYMMETRIC FLOW TRANSITIONS IN AN ABRUPT PLANAR EXPANSION 1. Introduction Flow of fluids through diverging geometries is very commonly encountered in various engineering operations. Flow through orifices, valves and pipe joints involves flow separations and local recirculations, which have an important impact on the transfer of heat, mass and momentum. Separation flows in expansions result in advantages such as reduction in pressure losses and disadvantages like reduction in the transfer rate. Another example of diverging flows includes the flow of a resin through a fiber bed, which is a complicated network of contraction and expansion regions. Very often flow is made even more complicated by the shear thinning viscosity, viscoelasticity or extensional viscosity. Extrusion of shear thinning foods through complex shaped dies is one such operation. Another class of flow through expansions is the unsteady state filling operation observed in injection molding and the exit flow of a polymer extrudate from an extruder die. In injection molding, flow of polymer melts into the mold cavity ofien results in flow transitions above a certain critical injection rate. In extrusion, flow of the extnrdate fiom the die to the ambient results in many instabilities (like wavy, bamboo, shark skin, ripple, severe distortion, etc.) only at higher injection rates and with smaller die sizes (Baird and 26 27 Collias, 1995). A clear understanding of such flow phenomena is very complicated due to three - dimensional flows, non - isothermal melt temperatures, complex flow geometries and non - Newtonian properties of the melt. Continuous, steady flow of Newtonian fluids through abrupt planar expansions has also revealed flow transitions above a critical flow rate of the fluid (Cherdron et al. 1978, Sobey, 1985, Feam et al., 1990 and Durst et al., 1993). This critical flow rate is known to vary with the area expansion ratio ([5) and the aspect ratio (ratio of the width to the height) of the channel. Attention has been restricted to obtain and analyze results for the flow of a Newtonian liquid (water) through abruptly expanding channels with area expansion ratios of 2 and 3. Although trends between the flow transitions occurring in these channels are available now, certain questions still need to be resolved. For example, what happens to the flow patterns at much higher expansion ratios? What is the rate of fall of the critical flow rate when extreme expansion ratios are involved? As far as this author is aware, there has been no attempt - experimental or computational - to gather evidence of such flow transitions with non - Newtonian fluids and to study the effect of fluid rheology on the occurrence of flow transitions, assuming that non - Newtonian liquids also behave similarly. The present study has been devoted to answering these queries related to the steady flow of Newtonian and non - Newtonian liquids through planar expansions. 2. Background 2.1 Contraction vs Expansion flows To understand the flow transitions of Newtonian liquids through planar expansions, a systematic, fundamental study is needed to understand more clearly the effects of fluid 28 nature, flow geometry and inertia on the flow characteristics. Unfortunately, there has been relatively less focus on expansion flows compared to the considerable attention that has been devoted to the flow of polymer solutions and melts through converging geometries. One possible reason for this could be the occurrence of various interesting flow characteristics in steady converging flows reported by Nguyen and Boger, 1979, Walters and Rawlinson, 1982, Boger et a1, 1986, Lawson et al., 1986, Evans and Walters, 1986, McKinley et al., 1991, Chiba et al., 1992,1995, Quinzani et al., 1995, etc. These features include the presence of lip vortices, enhanced comer vortex growth due to fluid viscoelasticity, oscillating flow and Goertler vortices. White et al. (1987) and Boger (1987, 1997) have presented a detailed review of such entry flows, while a few relevant ones have been discussed in Chapter 1. It is now accepted that in contractions, inertia decreases the size of the salient corner vortex (Boger et al., 1986, Abdul - Karem et al., 1993) whereas viscoelasticity enhances the vortex growth (Boger et al., 1986, Lawson et al., 1986 and McKinley et al., 1991). Fluid viscoelasticity and inertia produce the opposite effect in expansions (Abdul - Karem et al., 1993). Shear thinning seems to have a stabilizing effect on the flow patterns produced in an axisymmetric contraction by delaying the onset of flow instabilities (Boger et al., 1986). The effect of shear thinning on expansion flows has not been reported yet. The flow transitions of Newtonian liquids through planar expansions reported by Cherdron et al., 1978 and others have not been observed in contraction flows. It should be pointed out that only in the case of creeping flow of Newtonian liquids will the flow features in an expansion be a mirror-image of that in a contraction flow because only in 29 this case is the problem governed by linear equations. Inertial efl‘ects with any liquid would lead to differences in flow patterns. With non - Newtonian liquids, additional nonlinearities fiom the liquid properties such as shear thinning viscosity, viscoelasticity, extensional viscosity and yield stress would make the flow patterns in expansions difi‘erent from that in contractions. Hence, no direct inference for polymers flowing through expansions can be made based on corresponding contraction flow results. 2.2 Effect of geometry - Axisymmetric vs Planar Boger fluids (viscoelastic fluids with a constant viscosity) which show vortex enhancement in axisymmetric contractions, show very small or no vortices in planar contractions, even at high flow rates (Walters and Rawlinson, 1982). Lip vortices observed commonly in viscoelastic liquids flowing through axisymmetric contractions, are seen in planar contractions only at very high contraction ratios (Evans and Walters, 1986). Halmos et al. (1975) have shown that increasing shear thinning leads to increasing size of the vortices in a 1:2 axisymmetric expansion. Corresponding results for planar expansions are non - existent. White et al. (1987) in their review on all the existing data on contraction flows mention that vortex growth in general, is more readily observed in axisymmetric contractions than in planar. Differences in the flow features of Boger fluids between axisymmetric and planar contractions have been explained by White et al. on the basis of the work by James and Saringer (1980, 1982). In their work, James and Saringer have examined planar and axisymmetric sink flow of polyethylene oxide solutions. Sink flow may be approximated essentially as a shear-free flow and therefore the pressure drop through the orifice is a relative measure of the extensional stress in the contraction region. 30 It was observed that the pressure drop in the axisymmetric case was several times higher than in the planar case. This behavior was numerically predicted by Chakraborty and Metzrrer (1986). A similar analogy could be derived for expansion flows too, to explain difl‘erences between axisymmetric and planar expansion flows. 2.3 Flow transitions due to inertia in Newtonian flow through planar expansions Sobey (1985) has. studied the flow patterns developed in a Newtonian liquid (water) flowing steadily through a 1:3 two-dimensional planar expansion. He observed that at low flow rates (or low Reynolds number, Re, defined using the smaller channel half height and the average velocity in the upstream channel), the corner vortices were symmetric and that they increased in size as Re was increased. Beyond a certain critical Re (around 25 for an abruptly expanding channel), flow became asymmetric and one vortex grew more rapidly than the other. As Re was raised further, a third vortex was observed downstream of the expansion plane on the wall with the smaller corner vortex. The critical Reynolds number was observed to be higher when channel with gradual expansions were used. By using long rectangular channels of large aspect ratios (5 and above) Sobey and others have ensured that the flow far away fi'om the expansion plane is one dimensional. Experiments showing similar flow transitions in Newtonian fluids through abrupt expansions in 1 :2 and 1:3 charmels have been reported by Durst et al. (1974) and by Cherdron et al. (1978) and confirmed later by Fearn et al. (1990) and by Durst et al. (1993). The phenomenon wherein flow transitions lead to difl‘erences in the flow patterns beyond a certain critical Reynolds number is commonly referred to as “flow bifurcation” and the critical Reynolds number is called the bifirrcation point. 31 Cherdron et al. (1978) have investigated the efi‘ect of the expansion ratio and the channel aspect ratio (ratio of the width of the channel to its height) on the flow patterns developed in a Newtonian liquid flowing through a planar expansion. They have reported that the critical Re at which flow transitions occur goes down with an increase in the expansion ratio as well as an increase in the aspect ratio. For example, with a channel of aspect ratio 8, the critical Re goes down from about 150 to 30 in going from an area expansion ratio of 1:2 to 1:3. The mechanism of initiation of such flow transitions, even for Newtonian liquids, is not well understood. However, the Coanda efi‘ect does seem to explain how it is sustained. Flow asymmetry is a result of the momentum transfer in the direction normal to flow between the shear layers. As a result, the boundary layer adjacent to one wall is richer in momentum and consequently at a lower pressure as compared to the other. A transverse pressure gradient in the channel is created and as more liquid enters, flow of the liquid from the wall at higher pressure to that at the lower pressure takes place. This increases the momentum at the already richer wall even more, resulting in a more pronounced effect of the flow asymmetry. Interestingly, no flow asymmetry has been reported in axisymmetric expansions, where the flow induces concentric shear layers, as opposed to the stacked shear layers in planar flow. A continuity all along the plane of expansion in the former, prevents any occurrence of asymmetrical flow patterns. Although results on the flow transitions of Newtonian flows through expansion channels are available now, all the existing results are limited to low expansion ratios of 2 and 3. Experiments with large expansion ratios will help to answer 32 questions like what happens to the flow patterns at much higher expansion ratios and what is the rate of fall of the critical flow rate (or an equivalent critical Reynolds number) when extreme expansion ratios are involved? 2.4 Experimental work on Non - Newtonian flows through expansions Abdul-Karem et al., (1993) have investigated flow behavior of 0.05% polyacrylanride solution in glucose syrup (Boger fluid) through a 1:6.8 axisymmetric expansion and a 6.8:1 axisymmetric contraction. Although the vortex size observed in expansions was lower than that in contractions, the trend of vortex enhancement with increasing flow rate was observed in the expansion flow too. No lip vortices or instabilities were observed in either configuration. Halmos et al. (1975) have conducted experiments using aqueous carboxyrnethyl cellulose solution (inelastic, shear thinning power-law index of 0.73) in a 1:2 abrupt axisymmetric expansion. They have measured the radial and axial velocity profiles downstream of the expansion plane using flash photography and have compared those with their calculations for Reynolds numbers between 11 to 125. A good agreement was observed between their experimental and computational results. The authors do not observe any flow asymmetries, oscillations or lip vortices. Townsend and Walters (1994) have studied the flow of a 0.15% aqueous solution of polyacrylarnide (slightly shear thinning, strongly elastic) through an expansion fi'om a square section to a rectangular slit (area expansion of 13.3) and fi'om the rectangular slit to another square section (area expansion of 13.3). With a Newtonian liquid, significant vortex activity was observed due to fluid inertia. The vortex size increased with the flow 33 rate. The polymer solution, on the other hand, produced small comer vortices, the size of which decreased with the flow rate. Fluid elasticity thus, was observed to inhibit vortex growth. It should be pointed out that their study with Newtonian liquids has not shown any evidence of flow asymmetry, in contrast to those reported by Durst et al. (1974), Cherdron et al. (1978), Sobey (1985) and Fearn et al. (1990), despite a wide range of Reynolds numbers used. The square channels used by Townsend and Walters (1994) approximate axisymmetric flow which has never been known to show the flow asymmetry mentioned above. In addition, based on the findings of Cherdron et al. (197 8) that the critical Reynolds number for the onset of flow asymmetry increases with decreasing channel aspect ratio, one might conclude that at an aspect ratio of 1, flow asymmetry might be observed, if at all, only at very high Reynolds numbers. One notable contribution of the Townsend and Walters work was to clearly bring out the efl‘ect of fluid elasticity on the vortex growth in planar expansions. The observed trends in the effects of fluid inertia and elasticity on secondary flows was in contrast to what had been observed in various contraction geometries, where fluid inertia reduced the vortex size while elasticity led to vortex enhancement. This reversal of roles may be the reason for lack of further investigation of viscoelastic effects in expansion flows. Conspicuous by its absence from literature is any indication whether non - Newtonian flows will show flow bifurcation at high Reynolds numbers. Ifthey indeed do so, the effect of fluid rheology on the bifurcation point and on the flow patterns created needs to be studied. 34 2.5 Vortex growth prior to the onset of asymmetry Acrivos and Schrader (1982) have shown that prior to the onset of asymmetry, a linear relation exists between the reattachment length, the expansion ratio and the Reynolds number. They have derived an analytical expression that successfirlly predicts the symmetric vortex length at high Reynolds numbers for Newtonian flow in 1:2 and 1:3 planar expansions. Their expression, however, is valid only at high Reynolds numbers and does not account for the Mofl‘att eddies (Mofl‘att, 1964), which exist even under creeping flow conditions. Baloch et al. (1995) have numerically computed the reattachment length and have reported vortex growth curves for a wide range of Re for 1:4, 1:133 and 1:80 planar expansions. They indicate that the vortex growth is not linearly related to Reynolds number, particularly for channels with higher expansion ratios. As far as this author is aware, no study has addressed this issue of trying to relate the vortex length and the expansion ratio at both low and high Reynolds numbers in planar channels, before the onset of asymmetry. 3. Objectives The present work attempts to fill some of the missing links within the literature for flow through planar expansions. The objectives of the present chapter are: c To study the flow transition of Newtonian liquids flowing through planar channels of large expansion ratios. .To compare the flow bifurcation results with those available for low expansion ratios. 35 e To relate the Newtonian vortex grth before the onset of the flow transitions to expansion ratio and the Reynolds number. .To explore the effect of non - Newtonian viscosity on the flow bifurcation and on the flow patterns produced by the flow of shear thinning, inelastic liquids through planar expansions with large expansions ratios. Model channels have been designed with large aspect and expansion ratios. Newtonian model fluids and inelastic, non-Newtonian model fluids have been chosen and the effects of fluid rheology and injection rate on the flow patterns have been experimentally investigated using streak photography. Critical Reynolds numbers for the onset of flow asymmetry have been identified for the model fluids. Brief descriptions of the computations performed on 1:2, 1:3 and 1:16 planar expansions have been included. The details are reported in Chapter 4. Flow prior to the onset of asymmetry has been studied in detail for channels with expansion ratios 2, 3 and 16 with Newtonian and inelastic shear- thinning liquids. Relationships between the Newtonian vortex length and Re for the whole range of Reynolds number have been proposed. Experimental and computational results on the trends of vortex growth for non-Newtonian liquids have also been presented. Laser Doppler velocity (LDV) measurements have been presented in Chapter 3. Detailed computations of the bifurcation curves have been performed and are reported in Chapter 4. 36 4. Experimental 4.1 Model flow cell A model flow cell. with an abrupt area expansion of 16 has been constructed by using inserts to join two rectangular channels of the same width. An area expansion ratio of 16 is much higher than the ratios of 2 and 3, results for which are available in literature. A schematic of this transparent flow cell is sketched in Figure 2.1. Figure 2.2 shows the characteristic dimensions involved. An aspect ratio of 10 or more in either channel ensures that the upstream and downstream flows far from the expansion plane are one dimensional. Flow at the entry of the smaller channel is spread uniformly in the width of the channel by using a distributor plate. The inner inserts may be easily modified to incorporate a gradual expansion between the two channels. The height of the larger channel may be varied to change the area expansion ratio. Thus, the present "model configuration" permits flow observations on both abruptly and gradually expanding channels for more than one expansion ratio. Since the flow cell is constructed fi'om plexiglass, optical studies may be performed all along the length. During the assembly of the cell, care was taken to monitor the deflection of the plates while tightening the screws. This was achieved by using a Mag Base Indicator (NDI - MX50), which could detect deflections as small as 0.001 ". The thickness of each of the plates was measured by a screw gauge at least 12 locations. The maximum variation that was inherent to these plexiglass plates was about 7-8%. During filling of the cell, the vents were kept open to facilitate the flow of entrapped air. The cell was positioned such that the flow direction was aligned vertically against gravity. 37 Outer Plate (15” x 19” x 1”) Window (15” x 1.6” x 0.5” ) A / \\\\\\\V\\\\\\\\ \ j A ’(6135 36” x 0.75”) I< 19,, >1 Figure 2.1 Design of the model flow cell. 38 l6” ’ F >1 i”: 1... Left Side View Front View Figure 2.2 Characteristic dimensions of the model flow cell. 39 After the removal of the trapped air, the vents were shut ofi‘ and a valve connecting the central circular exit on the end-plate to a flow meter was turned on and steady state was allowed to be established. It must be pointed out that the weight of the flow cell (due to an exceptionally large size) and its contents did hinder easy movement of the assembly. 4.2. Model fluids Any model fluid used in the present study needs to be optically clear, non-toxic and non- degradable due to shear. Table 2.1 lists the model fluids and some of the relevant properties. Aqueous solutions of glycerol were used as Newtonian fluids. They were suitably diluted to yield solutions of viscosities between 12 to 1350 mPa-s. Viscosity measurements were performed on a Brookfield Viscometer (Model LVF-DVIII). A spindle with a diameter of 1.2 cm (Model SC-31) was used in the tests. The temperature of the sample was controlled by a heater in which the cup containing the sample was placed. Different fluid viscosities were needed to span a wide range of Reynolds number, which was defined as h U Re = A3 (2.1) Here h is the separation between the walls of the upstream channel, p and p are the fluid density and viscosity respectively and U”. is the average velocity in the upstream channel. 40 The latter was evaluated fi'om the flow rate of the liquid collected at the exit of the downstream end. The Reynolds number of flow may be varied from 0.001 to 6, covering regimes of creeping flow as well as low Re flows with non-negligible inertia. Table 2.1: Model fluids used Solution Designation Viscosity (mPa-s) n Relaxation (zero shear) time (s) Aqueous glycerol N 12 - 1350 1 - 1 wt% aqueous hydroxypropyl cellulose P1 350 0.7 5.4 x 10" ether 2 wt% aqueous hydroxypropyl cellulose P2 63 00 0.5 7.8 x 10'3 ether Inelastic polymer solutions have been prepared and used in the study. These shear thinning solutions used are aqueous solutions of hydroxypropyl cellulose ether (Methocel K4M, Dow). The shear thinning index (or pseudoplasticity) of the solution may be varied from 0.5 to 1 depending on the concentration of Methocel. The shear viscosity of the solutions was measured at 25 °C on a Fluids Rheometer (Rheometrics, RFS 8400). These steady 41 tests were performed at shear rates ranging between 0.1 to 100 s-l. A 0.02 rad cone and a 5 cm diameter plate were used for this purpose. A water-bath was used to maintain isothermal conditions in the sample holder. Figure 2.3 shows the efl‘ect of concentration on the shear viscosity of the solution. As the amount of the polymer was increased fiom 0.5 wt% to 2 wt%, the zero shear viscosity increased by 2 orders of magnitude. The shear thinning index went down fi'om 0.86 to 0.5. To prepare the solutions, about a quarter of the total water required was heated to 90° C. Methocel was then added to it with continuous stirring. When the temperature of this paste reached 40° C, the remainder of the water (in the form of water at room temperature and ice) was added and the mixture was stirred for about 30 minutes. The solution was allowed to stand for at least 24 hours with intermittent stirring. For lower stirring times, it was observed that the consistency of the prepared solution was very inhomogeneous and its appearance was cloudy and misty. This rendered the solution useless. The present study uses 1% (wt/wt) and 2% (wt/wt) Methocel solutions yielding shear thinning indices of 0.7 and 0.5 respectively. No significant difl‘erences in properties were observed due to repeated shearing of the fluids. The shear viscosity of the polymer solutions was fitted to a Carreau - Yasuda model of the form (2.2) 111 = [1+(bY)"]("'”/° (2,2) 0 and to the generalized Oswald-dc Waele power-law model (2.3). Shear viscosity, mPa-s 42 104 ' ' "r'rl v fi vvwwvv' 1 . 1,,fVT; AAAA AAA 3 AAA A 1 AAA w A 0000 000 4 000 00 00A A 103: 0 t 0 (boooooooooocpc,0000 L O 101: M0% 1 i 01.5% : 013% nunuunnnnnuu‘ no.5% T 101 a .r.r . . ....r.r . . ...,..7 lo-1 10° 101 101 Shearrate,s'l Figure 2.3 Effect of Methocel concentration on the viscosity of the polymer solutions. 43 n = k (r)‘""’ (2.3) Here n, is the viscosity at zero shear rate and a, b and k, n are fitting constants. The constant n is called the degree of shear thinning or the pseudoplastic index. Figure 2.4 compares the measured shear viscosity and the values predicted by using equations (2.2) and (2.3). Table 2.2 lists the fitting constants used. Equation (2.2) provides a better fit of the viscosity since it incorporates the Newtonian viscosity behavior at low shear rates. Table 2.2: Parameters used in the shear viscosity models Model Solution 1],, (Pa-s) a b (s) n k (Pa-s“) Carreau 1% 0.35 2 0.05 0.7 - Carreau 2% 6.4 2 0.24 0.5 - Power-law 1% - - - 0.7 0.751 Power-law 2% - - - 0.5 12.784 Since the viscosity of the polymer solution is dependent on the shear rate, equation (2.4) was used to define the Reynolds number of the shear thinning solutions. This took into Shear viscosity, mPa-s 104 103 , — Carreau model O 2% solution 0 l % solution °°°°° Power - law model A A I I ‘4 A J L A A I 100 101 Shear rate, 5'1 Figure 2.4 Shear viscosity of the polymer solutions. 45 account the power-law efl‘ect of shear thinning. n 2-n h Um p Re. - 2(1l2n)],,.l (2.4) 2H The wall shear rate in the upstream channel was used as the characteristic shear rate for the computation of the viscosity. The ranges of Re“ achievable for P1 and P2 were 0.1 to 4 and 0.1 to 1.6 respectively. The upper bound was related to the pressure that the apparatus could withstand. The polymer solutions were characterized by using a Fluids Spectrometer (Rheometrics RFS 8400) for both steady and dynamic shear properties. Dynamic measurements were made at fiequencies between 0.1 to 100 rad/s by using a 0.02 radian cone and a 5 cm diameter plate. The sample temperature was maintained at 25 °C by placing it in a thermally controlled water-bath. Figure 2.5 shows the storage modulus (G’) and the loss modulus (G”) curves for both the polymer solutions. For the 1% solution, the modulus could be reproducibly detected only at frequencies above 6 rad/s. The relaxation time of the polymer solutions was calculated fi'om the zero-fiequency limit of the G’ curve as GI 71009 A = (lim mm) (2.5) Relaxation times for the 1% and 2% solutions were 0.54 and 7.8 milliseconds respectively. The fluid elasticity was evaluated from the Deborah number. This product of the relaxation time and the wall shear rate at the highest flow rate indicated that the 1% G'(Pa), G" (Pa) 101. - m . "r": 'r'"! ' ' ' I A; l A r 06' P1 ago" ’ A‘e ‘ p .G' P2 . q p AAA . 4 AG”P1 ‘ . 100- AG”P2 A“ ' (i D ‘ . 6 1 : ‘A .. 88 f . ‘A . AA . A A O I . A 1 O A . AA 1 O A O '1. q 10 E e 0 3 I ' 0 I s . o _ O O O 10.2 A . .r...r . r x .mrIrr A r . .L... 10:1 10° 101 102 Frequency, rad/s Figure 2.5 Loss modulus and storage modulus of the polymer solutions. 47 solution was inelastic (Dem < 10"). The 2% solution, however, had a Dem of ~ 0.3 and was believed to exhibit elasticity under the conditions of the present study. 4.3 Flow visualization setup In order to carry out flow visualization experiments, the model fluids were seeded with 0.03 gm of neutrally buoyant Silicon Carbide particles (45 - 70 microns, Aldrich Chemicals). Using a sheet of light, a plane encompassing the expansion plane was illuminated. Particles passing through this sheet reflected light which was collected by a CCD camera (Nikon, F3). Using long exposure times (4 seconds to a few minutes) the path of these particles was traced. The size and the shape of the corner vortices and the flow patterns in the rest of the cavity could be picked up by this technique. The setup used for the flow visualization experiments is portrayed in Figure 2.6. Compressed nitrogen was used to force the model fluid fiom the reservoir to the flow cell and then back to the reservoir. A regulator was used to maintain constant flow rate conditions in the flow cell. By increasing the pressure in the reservoir, flow rates up to 400 ml/s were achievable in the flow cell. Two techniques were used to create a laser sheet fiom a laser beam. Figure 2.7 schematically demonstrates these methods. In the first technique, a laser sheet was created by passing a laser beam fi'om a 20 mW He-Ne laser source (Newport ULM ) through a cylindrical glass rod. By altering the position and to some extent the size of the rod, it was possible to get sheets of various widths and intensities. Although this procedure was simpler to set up and to manipulate than the other one, it resulted in significant intensity losses. Also, the sheet was non-uniform in intensity, with the center being much brighter than the periphery. Another indigenously developed technique that s33. 5:33.? .6...— en 2&3 horses“ 3 3.933— .925 .83 £338“ hoe—Emu mac‘— couch: Z .8555 ooh—em nemes— ozem cede—sue: 3.52 49 Rotating shaft pseudo-sheet Figure 2.7a Scanning mirror assembly for creating a laser sheet. Refracted laser sheet Cylindrical glass rod Figure 2.7b Laser sheet creation with a glass rod. 50 was used involved reflecting the laser beam ofl‘ a well-polished mirror rotating at around 2000 rpm such that the reflected beams scanned through a cross section of the flow cell. The latter approach created a sheet of higher intensity since it minimized loss of power. The former technique was the choice at lower flow rates and the latter yielded better results at higher flow rates. Flow visualization studies were then carried out using the 35 mm CCD camera mounted on a tripod close to the illuminated plane. Photographs of the seed particles were taken with exposure times varying between 4 seconds to a few minutes and apertures between f/ll to f/2.8. Use was made of a timer that allowed up to 16 minutes of exposure time. 5. Results and Discussion 5.1 Flow patterns in the Newtonian liquid (Experimental) Flow patterns at low Reynolds numbers of 0.01, 0.1 and 0.5 are shown in Figure 2.8a, b and c. Streak lines symmetric about the channel center-line are observed, with the reattachment lengths on both walls being equal. The angle of entry of the liquid is very close to 90°. This is expected because of the low Reynolds number and a large degree of expansion. With increasing inertia, the vortices were observed to grow in size. The flow profiles were always symmetric for Re between 0.001 and 0.6. Reproducibility was confirmed by repeating the experiment twice. To obtain the reattachment length, the negatives of the photographs were projected onto a screen and measurements were made using a meter ruler. These were then normalized with the step height. This non- dimensional reattachment length will be referred to as L,. 51 At Re = 0.8 (Figure 2.8d), a flow transition is observed. Close to the expansion plane, the streak lines in the center of the larger channel droop toward one wall and then firrther downstream shoot toward the other wall. This leads to an asymmetry in the flow patterns with a large vortex reattaching itself to one wall and a small one to the other. Sobey (1985) observed a flow transition with water through a 1:3 planar expansion at a Reynolds number of 25. Experiments performed by Durst et al. (1974) on a 1:2 planar expansion showed that the flow turned asymmetric at a Reynolds number of around 42. Thus, the interesting feature of the flow through a channel with expansion ratio 16 is the occurrence of flow transition at Reynolds numbers 2 orders of magnitude lower than those observed with the smaller expansion ratios of 2 and 3. This extends the findings of Cherdron et al. (197 8) who reported that increasing expansion ratios from 2 to 3 resulted in lowering the critical Reynolds number at which the flow asymmetry started. As Re is increased firrther, the larger vortex grows quite rapidly. The smaller vortex length decays slightly or remains constant. Figure 2.8e and f show the flow patterns at Re of 1.5 and 4 respectively. Some of the photographs showed the crossing of some streaklines close to the walls. These were initially assumed to be due to unsteadiness in the flow but later confirmed to be a result of slight movement of the camera timer. Laser Doppler velocirnetry measurements in the larger channel confirmed no flow unsteadiness at these Reynolds numbers. The LDV results have been reported in Chapter 3. The presence of a large vortex in Figure 2.8e and f results in a very narrow jet of the fluid in the core between the vortices. The swiveling motion of this jet is very similar to the jetting phenomenon observed in injection molding at high injection rates and low gate land 52 (b) Figure 2.8 Flow patterns of the Newtonian liquid. (a) Re = 0.001 (b) Re = 0. 53 v i t‘mfifl,‘ »...~T . ' 5- v {Mu-"Q! ' ((1) Figure 2.8 Flow patterns of the Newtonian liquid (continued). (c) Re = 0.5 (d) Re = 0.8. 54 Figure 2.8 Flow patterns of the Newtonian liquid (continued). (e) Re = 1.5 (f) Re = 4. 55 lengths (White and Dec, 1974 and Oda et al., 1976). In the experiments conducted by Sobey (1985), Durst et al. (1978, 1993) and Feam et al. (1990) for expansion ratios of 2 and 3, a second fl0w transition showing the presence of a third vortex has been reported at Reynolds numbers higher than the critical Reynolds number for the onset of the first flow transition. Unfortunately, due to a much larger channel size being used in the present experiments, practical limitations prevented the achieving of flow rates corresponding to higher Reynolds numbers. The second transition for the Newtonian liquid was therefore not observed. Figure 2.9 shows the vortex growth as a firnction of the Reynolds number. At Re of 0.8 and above, the salient vortices are difl‘erent in size. The difi‘erence grows as the Reynolds number is increased. The larger corner vortex grows more rapidly than the smaller corner vortex. 5.2 Computations of the flow bifurcation in Newtonian liquids Steady, two.dimensional finite element calculations were performed to predict the critical Reynolds number for the onset of asymmetry. A commercial code FIDAP (Fiuent, Inc.) was employed for this purpose. Only a brief description of the technique used and the numerical grids is included in this section. The details follow in Chapter 4. Figure 2.10 shows a schematic of the flow channel used. No slip velocity on the walls and a firlly developed velocity profile at x = -l, were imposed. l1 and I2 chosen were 5 and 65 step heights respectively. Reducing their values by 50% changed the solution only by 0.01%. The upstream channel height and the half height of the downstream channel were used to non - dimensionalize the axial and normal distance respectively. Reattachment length 56 O _ O O O O . o o 0 0 no 0 °° ° 0 1 2 3 4 Reynolds number Figure 2.9 Experimental vortex growth in the Newtonian liquid. 57 Figure 2.10 Schematic of the flow channel used in calculations. 58 The first goal was to validate the computational findings on Newtonian flow in a 1:3 channel by comparing them with the experimental and computational results of Feam et al. (1990) for a similar flow configuration. Their experiments and calculations have shown the onset of asymmetry at Reynolds numbers of around 23 and 27 respectively. Steady state computations on a symmetric grid failed to show any flow asymmetry fi'om Re = 0 to 40. The calculation protocol was then modified by incorporating a perturbation to the grid. An asymmetry was introduced in the geometry of the configuration by shortening one of the steps by about 10%. Stokes solution was then computed for this asymmetric channel. Using the Stokes solution as the initial iterate for the next run, the equations of motion were solved for a higher Reynolds number. For every subsequent Re, the result of the previous computation was used as the initial guess. This procedure was continued until Re of 40. At this point, the computational domain was made symmetric again and computations were now performed on this symmetric grid. For each subsequent run, Re was lowered gradually and the results of the previous runs were used as the initial iterate. This procedure was followed until a Reynolds number much lower than the bifirrcation point was reached. This approach will be called a perturbation - continuation approach. The step size of Re was anywhere fi'om 0.1 to 1. To evaluate the reattachment length, the sign of the axial velocity was monitored at the nodal layer closest to the walls and two successive points with negative and positive u- velocity were identified. A simple linear interpolation of the form of equation (2.6) then yielded the reattachment length. This was then normalized with the step height and was referred to as L, 59 (Jr+1(xrrl - xi) x = x , - 2.6 f I (1",! _ (It ( ) Figure 2.1 1 demonstrates the three branches of the bifurcation curve which result fiom the perturbation -‘ continuation approach for a channel with expansion ratio 3. The difl'erence in the reattachment lengths on the two walls normalized by the step height is used as the index of the degree of asymmetry in Figure 2.11 (and in subsequent bifurcation curves). Up to Re = 27, no asymmetry exists (i.e. the difference in the reattachment length is zero). This stable branch (1) is the one that is picked up experimentally. At Re greater than 27, the vortex lengths become unequal. The degree of asymmetry increases with increasing Reynolds number. Either of the branches 2 or 3 may be followed at Re > 27. At a critical Reynolds number of 27, the unique solution (1) is said to have bifirrcated into multiple solutions (2 and 3). The branch of the solution representing symmetry beyond the critical Re (branch 4) is the one that will be picked up by computations without using the perturbation - continuation approach. Durst et al. (1997) have recently performed a stability analysis and have shown that the branches 1, 2 and 3 are indeed stable solutions and branch 4 is the unstable solution and therefore would not be observed experimentally. The predicted onset Reynolds number of 27 for Newtonian flow through a 1:3 planar expansion using the perturbation - continuation approach is in very close agreement with the computations of Feam et al. (1990), which also predict the onset of flow asymmetry at the same Reynolds number. Difference in reattachment length 8 U ' l I ' x Asymmetric grid 3 4 ' OSymmetric grid 3 -. ' 0 ..... 4 4 . -8 . r r r r r r 0 10 20 30 Reynolds number Figure 2.11 Results from the perturbation - continuation approach for Newtonian flow through a 1:3 planar expansion. 61 To investigate the efl‘ect of grid resolution on the outcome of our calculations, three grids - Gl, GZ and G3 were designed with 2351, 5871 and 11431 nodes respectively. The mesh was graded finely in all the corners and was less dense away from the comers. Figure 2.10 schematically shows the variation of the grid density in the channel. In the axial direction (i.e., along the x axis), the mesh density was the maximum close to the x = 0 plane. In the transverse direction, the mesh was more dense near both the 90° corners (y= t 1) and the 270° corners (y = :h 1/ B) and was less dense in between. The bifurcation point for a channel with an area expansion ratio of 3 was used to compare the performance of the three grids. Figure 2.12 illustrates the result. GI and G2 produced results to within 0.1%. The performance of G2 and G3 was nearly identical. Further results have been computed on the grid G3. The computations for a Newtonian liquid flowing through a 1:16 planar channel revealed that the critical Reynolds number was around Re = 6.3. The corresponding bifirrcation curve is shown in Figure 2.13. The computations predicted a higher critical Reynolds number than that observed in the experiments. Such an over prediction has also been observed by other workers with 1 :2 and 1:3 channels. The lowering in the experimental critical Reynolds number for the onset of flow bifirrcations could be brought about by uncertainties in the experimental configurations. Computations for a 1:16 channel are also significantly difl‘erent from the corresponding 1:2 or 1:3 channel in the far severe corner singularity and the required more dense mesh grading close to the corners in the former. Difference in reattachment length 62 AG] 0G2 X G3 1" ,1 . 7 ' . .‘\ \C . d -i 1 4 I - 30 35 Reynolds number Figure 2.12 Effect of grid refinement on bifurcation curve. Newtonian flow, Expansion ratio = 3. Difference in reattachment length fl s y-s 63 b an 6 8 Reynolds number Figure 2.13 Bifurcation curve for the 1:16 expansion. 10 64 Since the critical Reynolds numbers obtained fi'om experiments and computations are difl'erent, a modified Reynolds number is defined to facilitate a comparison between the experiments and computations. Rem, = Re - Rem, The experimental critical Reynolds number is used to evaluate the experimental modified Reynolds number and the computational critical Reynolds number is used to evaluate the computational modified Reynolds number. Figure 2.14 compares the bifirrcation curves using the difl‘erence in the reattachment lengths on the two walls as the index of flow asymmetry. Only the positive half of the bifirrcation curve has been illustrated for purposes of clarity. At Re close to the critical Re, computations predict a lower degree of asymmetry than the experiments. This trend is reversed at Re much higher than the critical Reynolds number. 5.3 Newtonian vortex growth prior to the onset of asymmetry Figure 2.15 shows the trend of vortex grth with inertia, up to Re of 0.6. The data points used are fiom the flow visualization experiments. The solid line is from the computations described earlier. Equation (2.7) provided a good fit between LV and Re. L» = aRe + b (27) Values of 0. 18 and 0.425 were used for a and b respectively. Baloch et al. (1995) have computed the Newtonian creeping flow reattachment length (i.e., b in equation 2.7) for a 1:4 planar expansion to be 0.385, which is close to our value for the 1:16 expansion. They Difference in reattachment length 65 3 r U V I V fi' 1 0 Experiment V —- Computation O Remod = Re - Rec,“ Figure 2.14 Positive half of the bifurcation curvefor Newtonian flow. Reattachment length 0.6 u u u e in 0.40.0 0.2 0.4 0.6 0.8 Reynolds number Figure 2.15 Experimental Newtonian vortex growth prior to the onset of asymmetry. Solid line is from computation. 67 have also presented the reattachment lengths normalized with the downstream channel height for 1:133 and 1:80 planar expansions. The asymptotic reattachment length in the creeping flow limit for the 1213.3 channel is slightly higher than that for the 1:4 expansion. The vortex growth curves reveal two distinct regions, thus rendering a simple relation like equation (2.7) unsuitable to model the reattachment length for the entire range of Reynolds number used in their study (0 to 50). Acrivos and Schrader (1982) have proposed a linear relation between the vortex length and the Reynolds number based on the momentum flux. This leads to the following proportionality relating the reattachment length, expansion ratio ([3) and the Reynolds number. Re LV (1 (B -1)"2 (2.3) This expression is valid for large Reynolds numbers and predicts a zero vortex length for creeping flows. The presence of a finite corner vortex (Moffatt eddy) even under creeping flow conditions has been conclusively demonstrated in Mofl'att’s analysis (1964). To account for this anomaly and also to model the vortex length at low Reynolds numbers, the following is proposed: At low Re (the definition of low will be left ambiguous for the present), the growth of the normalized vortex length from creeping flow is proportional to the average inlet velocity of the channel, i.e., Lv-LoaRe 68 or L, = mRe + L0 (2.9) L, is the creeping flow reattachment length and m is the vortex growth coeficient. At higher inertia levels, flow behaves like a “jet” entering a stagnant fluid fiom a small orifice. This would require the reattachment length to depend on the flux of the momentum of this jet. Acrivos and Schrader (1982) have used this line of logic to come up with the model in equation (2.8) which is now modified to kRe kRe L, - L, = (0-1)!” = (l) (2.10) At high Reynolds numbers the assumption that L, << I.v leads to the equation (2.11). L = kRe = kRe v (ii-1)” (l) (2.11) Acrivos & Schrader have showed that their model is very effective with k = 0.137 (L, = 0 in their model) predicting the Newtonian reattachment lengths in a 1:2 and 1:3 planar expansion respectively. At the high Reynolds numbers at which this model has been tested, L, is indeed << L, For the data obtained at low Reynolds number in a 1:16 channel, such a relationship fails, as is obvious fi'om Figure 2.15. Clearly L, - L, is not negligible here and our earlier equation (2.9) is a better relationship to be used at low Reynolds numbers. To test this hypothesis, the reattachment lengths were computed for 1:2, 1:3 and 1:16 expansions for a wide range of Reynolds numbers, below the critical Reynolds numbers. 69 For B = 2, 3 and 16, the computations were carried out between Re of 0 - 65, 0 - 25 and 0 - 5.5 respectively. The upper bound is slightly lower than the critical Reynolds number for the onset of asymmetry for the channels. To compare the computed results with those of Acrivos and Schrader, L, was plotted as a function of Re / d), for B = 2 & 3. Only the reattachment lengths at high Reynolds numbers were considered. Figure 2.16 predicts slopes of 0. 135 and 0.137 respectively which are in very close agreement with 0.137, the prediction of Acrivos and Schrader (1982). The y-intercepts of 0. 14 and 0.2 for B = 2 and 3 respectively support the hypothesis that at high Reynolds numbers, L, << L, and that it may be neglected to yield equation 2.11. Such a relation, however, fails to predict the reattachment lengths accurately at lower Re, at which equation (2.9) is a more accurate representation of I.,,. Figure 2.17 shows the corresponding fits for the reattachment lengths in 1:2 and 1:3 channels at low Reynolds numbers. Table 2.3 reveals the fitting constants used in Figures 2.15, 2.16 and 2.17. Interestingly, the creeping flow reattachment length predicted for all the channels lies between a narrow range of 0.425 - 0.465. The vortex growth in the 1 :16 channel was already illustrated in Figure 2.15 for Re between 0 to 0.6 . L, predicted is 0.43 and is close to the values obtained for the 1:2 and 1:3 channels, thereby confirming the general applicability of equation (2.9) at low inertia levels. Excellent agreement between the computational results and the experimental data collected through streak photography is also evident in Figure 2.15. 70 12 ' I ' l ' I ' I ' U ' I OB=2 XB=3 .. too. a. s- .. - r: .e' .2 . ‘ Fl , .0" , g ,0" g c a 3 4. ' ' I 00 10 20 30 40 50 60 70 Rel(B-1)m Figure 2.16 Newtonian vortex growth prior to the onset of asymmetry at high Reynolds numbers. Lines represent'fits using equation (2.11). Reattachment length 71 4 ' I ' I j w I OB = 2 . ,s>"' . x B = 3 "0" 55'? 0‘0 2 - 0o . 00 O O O 10 15 20 25 Reynolds number Figure 2.17 Newtonian vortex growth prior to the onset of asymmetry at low Reynolds numbers. Lines are fits using equation (2.9). 72 Table 2.3: Fitting constants used in Figures 2.15, 2.16 & 2.17 B Re range k m L, 2 0 - 22 - 0.12 0.45 2 22 - 65 0.135 - - 3 0 - 7 - 0.15 0.465 3 7 - 25 0.137 - - 16 O - 0.6 - 0.18 0.425 5.4 Flow patterns in the shear thinning liquids (Experimental) Figures 2.18a - d show the effect of increasing inertia on the flow patterns developed in the 1% shear thinning fluid (n = 0.7). Symmetric streak lines are observed at Reynolds numbers of 1.25. The flow patterns at lower Reynolds numbers were qualitatively similar to that shown in Figure 2.18a. The corner vortices increased in size with increasing Reynolds numbers. At Re“ = 1.9, a flow transition leading to asymmetrical flow patterns is observed. Thus, the critical Reynolds number for the onset of flow transition for the 1% shear thinning liquid is between 1.25 and 1.9 and is higher than the corresponding value for the Newtonian case (between 0.5 and 0.8). Shear thinning, therefore, seems to delay the flow transition. An interesting feature observed in Figures 2.18b through 2.18d is the presence of a bunch of closely-spaced streak lines, starting from the center of the expansion plane and curving toward one of the walls. These bent streak lines resemble the 73 (b) Figure 2.18 Flow patterns of the polymer solution P1. (a) Re* = 1.25 (b) Re“ = 1.9. 74 Figure 2.18 Flow patterns of the polymer solution P1 (continued). (c) Re' = 2.4 (d) Re" = 3.1. 75 asymmetric filling patterns observed in injection molding at a high filling rate (Re* = 0.02, Dee and White, 1974), wherein the melt instead of radially filling the mold near the gate tends to shoot toward the opposite wall and then piles upon itself. This phenomenon of jetting was not observed by Dee and White at a low injection rate (Re‘ ~ 104 ). It would seem that both of these “difl‘erent” flow conditions i.e., the unsteady state mold filling during injection molding and the steady state channel flow in our present experiments show similar flow transitions beyond a critical injection rate. Another interesting observation above the critical Reynolds number is the simultaneous presence of three vortices. The largest vortex attaches itself to the transverse wall, close to the lip corner and it grows the fastest with increasing inertia. The first flow transition from the symmetric two-vortices state to the asymmetric two-vortices condition is not captured in the present experiments. Pseudoplasticity hastens the second transition which was observed by Durst et al. (1993) and Fearn et al. (1990) at much higher Reynolds numbers in their Newtonian experiments (214 and 85 for 1:2 and 1:3 expansions respectively). The simultaneous presence of three vortices has been confirmed by laser Doppler velocimetry measurements (results are reported in Chapter 3). Figure 2.19 shows the vortex growth with increasing Re“ for the 1% solution. Only the two 90° corner vortices have been presented in the figure because it was very difficult to get all of the three vortices on to one single photograph. While the smallest vortex length remains essentially constant, the larger vortex is seen to grow much faster at Re‘ > 1.9. Streak photography experiments carried out with the more shear thinning liquid (2% Methocel, n = 0.5) did not reveal any flow asymmetry until the highest achievable Re“ of Reattachment length 76 1.0 ' j r 1 ' 0 P1 0.8 " 0 p2 0.6 " o O 0.4 r o o o 0 O O O 0.2 '- [ 0 O O O 0'0 o 1 2 Reynolds number Figure 2.19 Experimental vortex growth in the polymer solutions. 77 1.6. The only conclusion that may be made is that the critical Reynolds number for this liquid is above 1.6. This is consistent with the trend of increasing critical Reynolds number (from 0.8 to 1.9) with increasing shear thinning (for n = l to n = 0.7) observed in our earlier experiments. In addition, characterization of the 2% polymer solution did reveal that it possessed a finite elasticity at the higher flow rates. Studies performed on elastic polymer solutions by Townsend et al. (1995) have shown that elasticity decreases the vortex activity in a 1:133 planar expansion. The efl‘ects of higher shear thinning and higher elasticity would thus translate to an even higher critical Re“ for the 2% Methocel solution. The reattachment lengths for the 2% solution have been included in Figure 2.19. 5.5 Flow bifurcation in the non - Newtonian liquids A power - law model was used to describe the viscosity of the polymer solutions. The same perturbation - continuation approach described earlier for the Newtonian liquids was used and flow bifurcation curves were obtained for the shear thinning liquids. A critical Reynolds number of about 18 was predicted for the shear thinning liquid with n = 0.7. As with the Newtonian liquid, computations for the shear thinning liquid also over - predicted the critical Reynolds number. The non-idealities that are inherent to the experiments are probably responsible for an earlier transition. The computations did reveal both the flow transitions for the pseudoplastic liquid. Interestingly, the ratio of the experimental critical Reynolds number for n = 1 and n = 0.7 and the computational critical Reynolds number are very close in magnitudes. 78 = 0.39 [Re‘ lap! C and [——‘—],0 = 0.35 Re a c "'P For a shear thinning index of 0.5, a higher critical Reynolds number of about 27 was obtained. This confirmed that shear thinning delays the onset of flow transitions in a 1:16 channel. The bifurcation curves and other associated details for the shear thinning liquid have been presented in Chapter 4. To facilitate a comparison between the experimental and the computed bifirrcation curves for the shear thinning liquid with n = 0.7, a modified Reynolds number was defined as Rum = Re* — Re-rcm For the experiments and the computations, the respective critical Reynolds numbers were used to evaluate the modified Reynolds numbers. Figure 2.20 compares the positive half of the bifurcation curves. The trends observed are essentially similar to those described earlier for the Newtonian liquid. Computations seem to deviate much more fi'om the experiments as the Reynolds number is increased. Difference in reattachment length 79 1.5 u 0 Experiment — Computation 1.0 0.5 0.00.0 0.5 Figure 2.20 Predicted bifurcation curve for shear thinning liquid Pl. 1.0 1.5 Re*m,d = Re“ - R6,,“ 2.0 80 5.6 Computed vortex growth in non-Newtonian liquids, prior to the onset of asymmetry Figure 2.21 compares the experimental and the calculated vortex lengths for P1 before the onset of asymmetry. The solid line represents a linear fit of the computed vortex lengths. A good agreement between the calculated and the experimental values is observed. A zero-Re vortex length of 0.23 is predicted, which is almost halfof that for the Newtonian liquid. A similar comparison for the 2% solution is done in Figure 2.22. Here the computational predictions are within 5.5% of the experimental L, data. The predicted vortex length under creeping flow conditions is around 0.136, which is lower than that for both the other liquids. Thus shear thinning consistently suppresses the growth of the corner vortices. The efi‘ect of expansion ratio on the vortex lengths before the onset of asymmetry for n = 0.7 is brought out in Figure 2.23. Here the results for B = 3 have been compared with those for B = 16. At low Reynolds numbers, L, for B = 16 is lower than that for B = 3. In both the channels, L, rises monotonously with Re', with the grth being higher in the larger expansion channel. At Re' of around 7, a cross-over occurs. This cross - over is merely an artifact of the higher scaling term (step height) used for L, at B = 16 as compared to that at B = 3. The step height in the former is 7.5 times that in the latter. The dimensional vortex lengths will, therefore, be much larger for the higher expansion ratio. For the more shear thinning liquid with n = 0. 5, no cross-over is observed for the entire range of Reynolds numbers studied (Figure 2.24). The non - dimensional L, for the channel with B = 16 is always less than that for the one with B = 3. The vortex lengths for Reattachment length 81 0.4 . . . . os - . 0.2 i .. 0.1 - . Moo T 0:5 A 1:0 Reynolds number Figure 2.21 Vortex growth in polymer solution P1. Solid line is from computation. 1.5 Reattachment length 82 0016 ' I ' r ' U V , 0 d 0.15 0.14 (moo A 0.5 A 1.0 ‘ 15 A 2.0 Reynolds number Figure 2.22 Vortex growth observed in P2. Solid line ,is from computation. Reattachment length 3 O 0B ' "[3:16 0 o 5 A 10 15 Reynolds number Figure 2.23 Vortex growth before the onset of asymmetry, n = 0.7. Reattachment length 006 ' f j I ' I I OB=3 0 "13:16 0.4 ~ ° - O O x x 0.2 " x x x x x - x x x X x x x 0'00 2 4 6 8 Reynoldsnumber Figure 2.24 Vortex growth before the onset of asymmetry, n = 0.5. 10 85 n = 0.5 are shorter than those obtained for n = 0.7. Figure 2.25 reveals the efl‘ect of shear thinning and expansion ratio on the creeping flow vortex length, L,. With an increase in the expansion ratio from 3 to 16, the normalized vortex length goes down at any shear thinning index. Attempts made to model the reattachment lengths for the shear thinning liquids at high Reynolds numbers using equation (2.11) met with little success. The values of k for the best linear fit ranged from 0.01 to 0.08 for the 1:3 and 1:16 channels. There is definitely a need to address this issue further and to propose new relationships between L, and Re“ for the shear thinning liquids. 6. Conclusions Flow visualization was used to study the onset of asymmetry in a 1:16 planar channel. One Newtonian and two shear thinning solutions were employed as the test fluids. Flow transition in the Newtonian liquid occurred at Red of 0.8, which is significantly lower than the critical Reynolds numbers reported previously for 1:2 and 1:3 planar channels. This extends the findings of Cherdron et al. (1978) who reported that increasing expansion ratios from 2 to 3 resulted in the lowering of the critical Reynolds number at which flow transitions were witnessed. With the shear thinning liquid P1 (n = 0.7), flow transition was observed between 1.25 - 1.9. Shear thinning, therefore, delayed the onset of asymmetry. No flow transition was observed with the more shear thinning liquid P2 (n = 0.5), for the entire range of Reynolds numbers studied. Higher shear thinning and/or higher elasticity could be responsible for the absence of the expected flow transitions. With P1, the flow transition occurred from a state of two symmetrical vortices to a state of three asymmetrical vortices. The intermediate step of two asymmetrical vortices was not Creeping flow reattachment length 86 0.5 r ' j 0 O x 0.4 r ' 0.3 ' ' O x 0.2 - " X 0 B = 3 0.1 r x B = 16 ‘ 0.00.4 0.6 0.8 1.0 1.2 Shear thinning index Figure 2.25 Effect of shear thinning on the creeping flow vortex length. 87 observed. Others have reported a similar second flow transition fi'om two asymmetrical vortices to three asymmetrical vortices with Newtonian liquids, at much higher Reynolds numbers. Therefore, it may be said that pseudoplasticity hastens the second transition with a 1:16 planar expansion. It may be summarized that a combination of high enough expansion ratio, a fairly non-shear thinning liquid and high injection rates will lead to early flow transitions in planar expansions. A perturbation - continuation approach was developed to compute the bifurcation curves for the liquids. The predictions of the critical Reynolds numbers were higher than the experimentally obtained values. This could be due to the uncertainties inherent to the experimental configuration. The computations of the vortex lengths prior to the onset of asymmetry showed excellent agreement with the experimental data. Relations between the Newtonian reattachment lengths, Reynolds number and the expansion ratio were proposed for the entire range of Re prior to the onset of asymmetry. These were confirmed by our computations with 1:2, 1:3 and 1:16 planar channels. A Newtonian non-dimensional vortex length of about 0.44 step heights was predicted for creeping flow, for all the three channels investigated. The creeping flow reattachment length increased with B and with n. More work needs to be done to obtain a modified relationship that successfirlly predicts the non-Newtonian reattachment lengths. Chapter 3 LDV MEASUREMENTS OF NEWTONIAN AND NON - NEWTONIAN LIQUIDS IN ABRUPT PLANAR EXPANSIONS This chapter discusses the laser Doppler velocimetry experiments performed to acquire detailed velocity profiles in Newtonian and non - Newtonian solutions, particularly afier the onset of flow asymmetry, in a 1:16 planar channel. The occurrence of flow transitions in the Newtonian and the non - Newtonian model fluids flowing through a 1:16 planar expansion were revealed in Chapter 2. The objectives of this chapter are to make detailed velocity measurements with particular emphasis on the velocity profiles at Reynolds numbers much higher than the critical Reynolds number for the onset of flow transitions. These measurements will confirm some of the findings reported in the earlier chapter. They will then be used to determine the rate of decay of the flow asymmetry with axial location and also to evaluate the flow bifurcation curves using the center line shear rate as a measure of asymmetry. These trends will be compared with the predictions developed in the present study. 1. Experimental 1.1 Laser Doppler velocimetry A single component laser Doppler velocimetry (LDV) system was used to measure the velocity along the direction of bulk flow. A detailed description of the principles of LDV is 88 89 given in texts by Drain (1980), Durst et al. (1976), Watrasiewics and Rudd (1976), etc. LDV (or LDA, laser Doppler Anemometry) is a non-obtrusive technique which measures the velocity of non-buoyant particles suspended in a flow. Ifthese particles are small, they behave like flow tracers and their velocity is equal to the velocity of the medium. When the suspended particles are illuminated with a laser beam, the particles scatter light at a particular fiequency, difl‘erent fi'om that of the incident beam. This difference in the fi'equencies, called the Doppler shift, is linearly proportional to the particle velocity. In the commonly employed fiinge mode, LDV is implemented by splitting a laser beam and making the resultant beams intersect at the focal point of a transmitting lens, thus forming interference fiinges. As the suspended particles cross these fiinges, they scatter light which is intensity modulated. The scattered light is collected and focused onto a photodetector, whose output is a Doppler signal with frequency independent of the collection angle. Ifthe transmitting lens itself is used to collect the scattered light, the scattering is called backward mode. The scattering is forward mode if a separate lens is used to focus the scattered light onto the receiving optics. The Doppler frequency is estimated using a signal processor and the velocity is obtained from the following relation: A U=u -f)d =(f-f) D S f D S 2Sin(%) (31) where U is the component of velocity in the plane of the two laser beams and perpendicular to their bisector, fD and f9, are the Doppler and the shifi frequencies respectively, df is the fiinge spacing, A is the wavelength of the laser light and 6 is the beam intersection angle. 90 When the fiinges are stationary in the measurement volume, particles moving in opposite directions result in identical photodetector signals. Difl‘erentiation of the direction of motion then becomes impossible. This problem is commonly encountered in the measurement of reversal of flows, which form part of the present study. Difl'erentiation is accomplished by introducing a fiequency shifi to one of the laser beams using an acousto- optic modulator called Bragg cell. This results in a bias motion of the fiinges, which makes the resulting signals direction sensitive. Another distinct advantage of using frequency shifting is its ability to measure the small magnitudes of the velocities, often encountered close to the walls. 1.2 Optical setup Figure 3.1 shows a schematic of the setup used in the present study. Table 3.1 details the various components. A 35 mW He-Ne laser emitting light at a wavelength of 632.8 nm was used to make measurements of the axial velocities in the forward scatter mode. The unusually long width of the flow cell and the extremely small magnitudes of the velocity component normal to the bulk flow, prevented their acquisition. The major optical components consist of a beam splitter, which divides the incident beam in two equal intensity beams separated by 50 mm, and transmitting and receiving lenses, each having a focal length of 250 mm. This lens system produces a beam halfangle of 5. 17° and an ellipsoidal measuring volume ofO. 18 x 0.18 x 1.9 mm’. The fiinge spacing is 3.18 pm, resulting in 64 fiinges across the measuring volume. The velocities measured in this study typically are in the range of 0.005 to 20 cm s", which correspond to Doppler frequencies 01“ approximately 0.16 to 640 kHz. To measure the flow reversal and the slower velocities 91 .953 >A: a... ._e BEES—um fin 95!..— 2 U U On. E 2 92 Table 3.1 Description of the components depicted in Figure 3.1 No Model Description ' Number 1 9126-105A 35 mW He-Ne laser, Wavelength = 632.8 nm 2 9126—255 Laser power supply 3 TSI 9115-2 Beam Splitter, 50 mm separation 4 TSI 9182 Bragg Cell 5 TSI 9186 Frequency Shifter Electronics 6 TSI 9118 Transmitting lens, focal length = 25 cm 7 TSI 9118 Receiving lens, focal length = 25 cm 8 TSI 9126, Optical rails 9121 9 TSI 9160A Photomultiplier 10 TS] 9165 Photomultiplier power supply 1 l Compudyne Computer 486 DX2 12 DANTEC N Signal Processor Burst Spectnrm Analyzer 13 465 M Oscilloscope 93 near the wall, frequency shifting was employed by using a Bragg cell. The power supply to the Bragg cell contains circuitry for downmixing the detector signal, so that the effective ' shift fi'equency may be adjusted to yield the optimum Doppler signal fiequencies. After the signal fi'om the photodiode detector is downmixed by the frequency shift electronics, it passes to a signal processor, which obtains essentially real time results for the Doppler fiequency by using a dedicated FFT processor and a four-bit quantization of the real and imaginary parts of the complex Doppler signal. The DANTEC software BURST was used to perform statistical analysis on the measurements. The standard deviations were always less than 0.5% of the mean values in the measurements reported here. The transmitting and the receiving optics were mounted on mechanical traverses which had a range of 10 cm in all the three dimensions and a resolution of 0.025 mm. Care was taken to ensure that no mechanical shocks were imparted to the setup during data acquisition. 2. Results and Discussion LDV experiments were performed in the larger channel of the flow cell. Figure 3.2 defines the nomenclature to be followed in the next few sections. The central plane of the flow channel along the z - axis (the axis normal to the x-y plane) was chosen to be investigated. This ensured that end-effects were avoided. The axial velocity component, U, was measured at various x - locations, traversing the laser beams along the y - direction from one wall to the other. The upstream channel height, h, and the downstream channel half - height, I-I/2 were used to normalize x and y respectively. The velocity was normalized by Um, the maximum inlet velocity in the upstream channel. This was estimated from the measured flow rate and by assuming a fully developed velocity profile 94 I I I I I I Y=I r A I I I I I I I H I I I I I I I I I I I I I V r Y=_1 X=0 I I r r X=l X=5 Figure 3.2 Nomenclature used to describe the LDV experiments. 95 at the inlet of the smaller channel. In the present setup, measurement of the normal velocity component (V) along y = 0 could not be accomplished due to two reasons - the unusually long length of the channel in the direction normal to the x-y plane and the very small magnitudes of V which resulted from the low Reynolds numbers investigated (maximum Reynolds number was 3.5). The presence of thick plexiglass walls and extremely small magnitudes of U close to the wall resulted in zero - velocities about 2 mm from either wall. These measurements have not been considered in the present work. Reproducibility was confirmed by repeating each experiment twice. 2.1 Velocity profiles of the Newtonian liquids Velocity was measured at X =1, 8 and 15 at various points between Y = -1 to +1, and at Reynolds numbers of 0.6, 1.5, 2.5 and 3.5 for the Newtonian liquid N. Recall that the streak photography experiments reported in Chapter 2, revealed that the critical Reynolds number for the onset of flow asymmetry was between 0. 5 - 0.8. The Reynolds number referred to here is defined in Chapter 2 and is reproduced below in equation (3 .2). _ ”Um? 211 Re (3.2) Here h is the upstream channel height, U,,,ll is the average velocity of the fluid in the upstream channel and p and u are the fluid density and viscosity respectively. 96 To validate the LDV measurements, velocity profiles were measured far downstream of the plane of expansion and compared with the plane Poiseuille flow. Figure 3.3 shows the comparison of the velocity profiles at X = 15 for various Reynolds numbers. The solid line represents the known analytical solution. By X = 15, flow is fully developed for all the Reynolds numbers investigated. The maximum deviation is about 3%. Figure 3.4 illustrates the axial velocity profiles at Re = 0.6. The solid lines were obtained from computations, which will be described later. Symmetry in the flow is obvious at all the three locations. At X = 1, the expansion efi‘ect is clearly seen when the incoming momentum fi'om the upstream channel results in a peak velocity of only about 40% of Um. At X =1, negative velocities are observed between Y = i 0.8 to i 1. The point at which the negative velocity crosses over to positive values, indicates the center of the recirculating vortex. This flow reversal region spans more than 20% of the channel. As the monitoring plane is moved downstream, the peak velocity is reduced drastically from about 0.09 at X = 5 to the fully developed value of 0.0625 at X = 15. No negative velocities were detected at X = 5 and 15. The overall flow profile flattens out as the axial distance is increased. The fluid excluding the portion in the recirculation zones will be called the core. This core continuously expands from X = 1 to X = 15. Considerable difi‘erenoes in the velocity profiles are observed (Figure 3.5) when the Reynolds number is increased to 1.5, i.e., above the onset of asymmetry. At X = 1, a peak velocity of about 0.43 occurs at Y = 0.2, which is clearly far away fi'om the center line Y = 0. The asymmetry is also seen in the recirculation zones, with one being almost thrice the other. Significant motion in the corner vortices is detected, with the peak negative velocity Axial Velocity 0.0a - . - . . . . . 0.06 - , ; ‘ - .. 0.04 - 3 Z . 0 cm = 0.6 i 0 Re = 15 ' ‘ 0.02 - : ' ‘Re = 25 ; r a Re = 35 0 s r s r L I a A .1 -0.6 .0.2 0 2 0 6 r Y Figure 3.3 Fully developed velocity profile of the Newtonian liquid at X = 15. Solid line is the plane Poiseuille flow. Axial Velocity 98 0.5 . r . I n r Ax=l 0.4 " OX=5 I'-|X=15 0.3 r Solid line - Calculations 0.2 0.1 0 '0'1-1 A 0 o .02 03 0.6 Figure 3.4 Symmetrical axial velocity profiles of the Newtonian liquid at Re = 0.6.. Axial Velocity 0.5 ' U V 1 U T F j A Ax=l 0.4 " ' OX=8 0.3 _ I3X=15 ‘ A 0.2 " a O O A 01 l- O A o A d n n D D II a an a D a a O a a I g 8 0.0-qoooo<>°AA 8!. A A A A A A A A '0°1-l.0 -0.6 -0.2 0.2 0.6 1.0 Figure 3.5 Newtonian velocity profiles after the onset of asymmetry, Re = 1.5. 100 being about -0.07. At X = 8, the smaller vortex has disappeared but the efl'ect of the larger one can still be seen. The flow becomes symmetric again, with a fillly developed profile observed at X = 15. With an increase in the Reynolds number to 2.5 and then to 3.5, similar trends are observed. These are shown in Figures 3.6 and 3.7. The peak velocities at X = 1 and X = 8 increase only slightly with increasing Reynolds numbers. For the range of Reynolds numbers used in the present study, the second flow transition that has been reported in Newtonian flows through 1:2 and 1:3 planar channels (by Cherdron et al., 1978, Sobey, 1985, Fearn et al., 1990 and Durst et al., 1993) was not observed in the 1:16 channel. Higher Reynolds numbers would be required to witness such a transition. Figure 3.8 compares the velocity profiles at X = 1. At Re = 0.6, a symmetrical profile with a peak at Y = 0 and with weak recirculation zones is observed. A drastic change in the profile occurs at Re = 1.5. Velocity now peaks at Y = 0.2. As Re is increased to 3.5, the peak shifts slightly toward Y = l and the motion in the vortices also increases. Some experiments revealed the larger vortex clinging to Y = 1 during a run and then showed the same vortex attaching itself to Y = -1, when the experiment was repeated. The vortices did not seem to have preference to attach to any particular wall. In our presentation, however, we have always retained the smaller vortex at Y = 1, as a matter of convention. At X = 8 (Figure 3.9), the smaller vortex has disappeared at all the Reynolds numbers. The profile is still asymmetric at Re = 1.5 and 3.5 but has started approaching the symmetric profile. This may be concluded by the observation that the peaking of the velocity now occurs closer to the center line than at X = 1. Axial Velocity 101 0.5 v u w w I u v 04 A AX=1 ' ox=s 0.3 _ A DX=15 0.2 ’ " A X o 0.1 a a I: n o a a u u a u an O a O O 2 B a 0.0rllnooooO A A3... A A A A: A A 9 A .0.1 s 4 l l a l A -l.0 -0.6 -0.2 0.2 0.6 1.0 Y Figure 3.6 Newtonian velocity profiles after the onset of asymmetry, Re = 2.5. 102 0.5 I I I II A AX = l 0.4 ' " A OX = 8 03 . a x = 15 . 5’ .3. 9 .. A J z 0.2 A O 3 o 0.1 ' o O o A d a D D u D u D a an a u u o 8 B B 3&3 A A A A A M .0 1 LA A l l a l A . -l.0 -0.6 -0.2 0.2 0.6 1.0 Figure 3.7 Newtonian velocity profiles after the onset of asymmetry, Re = 3.5. Axial Velocity 103 0.5 + u u r fl 1 D °Re=0.6 O 0.4 ' ‘ 0Re=l.5 a DR =3.5 0.3 - e « o 0.2 - o D - o 0.1 L a - o 0 o o 9 . o o . 0.0 W°°°°°003 099883 B 9 0 ° 0 n a I!" .01 P a P l 4 a l A ° -l.0 -0.6 -0.2 0.2 0.6 1.0 Figure 3.8 Newtonian velocity profiles close to the expansion plane; X = 1. Axial Velocity 104 0018 I V I I V I °Re=0.6 g 0.14 - ORe=1.5 " B URB=3.5 q 5 a J 0.10 - o o o o o '3 ‘ o o o p 0 cl 0.06 o o o o o 8 ‘ . o 0 o 0.02 o a 0 0 § 1 9 Ia. * to 0 ° 9 8 1 a U u .o.oz_w .0 6 -o.2 0.2 o 6 Figure 3.9 Newtonian velocity profiles at X = 8. 1.0 105 The area under the flow curve from our experimental data was evaluated using Simpson’s rule. A parameter A using the difi‘erence between this area and the measured flow rate per unit width in the z - direction is defined in equation (3.3). This parameter may be considered as a measure of the inferred transverse flow. (%)actual " (‘9wa 0%,»ch A x 100 (3.3) Here (Q/W),cum is the measured flow rate per unit width in the z - direction, (Q/W),_Dv is the area under the curves shown in Figures 3.4 through 3.7. The inferred transverse flows at various X - locations and for all the Reynolds numbers are shown in Figure 3.10. These range from 0.2% to 9%. Significantly high values of A close to the expansion plane indicate that the transverse flow is maximum close to X = O and that it reduces with increasing axial distance. 2.2 Velocity measurements of the shear thinning liquids (n = 0.7 and n = 0.5) LDV measurements were performed with the shear thinning solution, Pl at four locations - X = l, 8, l6 and 45, and at Reynolds numbers of 1, 2, 2.5 and 3. Since the viscosity of the polymer solution is dependent on the shear rate, equation (3.4) was used to define the Reynolds number (denoted by Re“) of the shear thinning solutions. This took into account the power-law effect of shear thinning. The half height of the upstream channel, the upstream average velocity and the wall shear rate in the upstream channel were taken as the characteristic parameters to define the Reynolds number. 106 10 - u - . - . . . . ' o °Re=0.6 8 ~ ‘ ORe=1.5 ’ ARe=2.5 6 . flRe=3.5 U A,% 6 4.. O D A 2' c O A 0 - n J a 1 a 4 4 0 4 8 12 16 Figure 3.10 Inferred transverse flow of the Newtonian liquid. 107 n 2-n h Um,g p 2"[2(1;2n)],,.1 (3-4) Re" = Flow visualization experiments (Chapter 2) had indicated that the flow transition from symmetric to asymmetric flow occurred at Re“ between 1.25 and 1.9. With the shear thinning liquid the development of the flow profiles was observed to be much slower than in the Newtonian liquid. At the higher Reynolds numbers, flow became fully developed at X = 45, as Opposed to X = 15 for the Newtonian liquid. Figure 3.11 shows the velocity profiles at X = 45. The solid line is the analytical solution for flow between parallel plates of a power - law liquid. An excellent agreement indicates the reliability of the measurements and the fact that the flow at X = 45 is not afi‘ected by the abrupt changes in the geometry at X = 0. The velocity profiles at Re“ = 1 (before the onset of asymmetry) are shown in Figure 3.12. The solid lines are fiom computations which are described later. Velocity at all X - locations is maximum at Y = 0. At X = 1, the peak velocity is about 0.375, which is less than the peak of the Newtonian liquid, even at Re = 0.6. At X = 8, the velocity profile has approached the fully developed flow observed at X = 45. The velocity profile above the onset of asymmetry is illustrated in Figure 3.13 at Re" = 2. At X = 1, strong vortex activity is observed in both the corners. The peak velocity in the recirculation zone is about -0.04. A narrow core indicative of the presence of large recirculation eddies is clearly seen. Difl‘erences in the sizes of the recirculation zones are not very obvious. The peak velocity appears to be only slightly off - centered, a behavior Axial Velocity 108 0008 ' I ' 1 ‘ I V U 0.06 " ‘ °Re* = 1.0 0.04 " t 0 Re“ = 2.0 ARe“ = 2.5 i 0.02 _ D Re"I = 3.0 .. Solid line - FEM computation I l A l 4.0 A -0.6 -o.2 ‘ 0.2 0.6 A 1.0 Figure 3.11 Fully developed velocity profile of the 1 % shear thinning liquid at X = 45. Axial Velocity 109 0.5 V I ' T U ‘7 I A X = l 0.4 ' ' O X = 8 fl = 03 _ x 45 Solid line - FEM computation 0.2 " . Figure 3.12 Velocity profiles of P1 at various axial locations before the transition. Re“ = 1. 1.0 Axial Velocity 110 05F I I . I I I I fl °X=l 04' OX=8 ‘ AX=16 0.3 ’ ‘ 0 0.2 b o O ' o o A A 0.1 r 9 " AA 0 A A 80° ‘ 9 A A A 0 ° 0 6 A 0.0 " 0 O o A " I: : : r c . a 0.1.1.0 -0.6 -0.2 0.2 0.6 1.0 Figure 3.13 Velocity profiles of P1 after the onset of asymmetry. Re“ = 2.0. 111 in contrast to what was observed with the Newtonian liquid. At X = 8, the maximum velocity occurs significantly away from the center line at Y = 0.3. The core also expands considerably, demonstrating the decay of the corner vortices at X = 8. Portions of the recirculation zones are still visible. At X = 16, the peak has moved slightly toward the center and the profile has started acquiring symmetry. The velocity profile is firlly symmetric at X = 45. Figures 3.14 and 3.15 show essentially the same behavior at Re“ = 2. 5 and 3, with the peak velocities increasing marginally with an increase in the Reynolds number. In Chapter 2, the presence of three simultaneous vortices was reported in the shear thinning liquid, at Re“ above the critical Reynolds number. The intermediate stage wherein flow transition occurs from a state of two symmetric vortices to a state of two asymmetric vortices in the Newtonian liquids was not detected in the flow visualization experiments with the shear thinning liquid. The present LDV measurements also do not show a flow transition to a state of two asymmetrical vortices. Instead the existence of three vortices is confirmed from Figure 3.16, which shows the presence of two comer vortices in the portion of the channel close to Y = -l, at Re" = 2.5. The dimensional velocities corresponding to those shown in Figure 3.16 are in the range of 0.2 to -7 mm s ", which are well above the minimum velocities that can be measured reliably by the laser Doppler equipments used in the present study. Very close to the walls, faint signals with positive velocities were detected. The velocity changes sign and becomes negative at Y = -O.8 and then turns positive again at around Y = -0.25. The occurrence of three cross - overs at X = 1 clearly demonstrates the simultaneous existence of three vortices in the larger channel. Axial Velocity 112 0.5 V I I 7 I w I ' 0X=1 l 04' OX=8 ‘ O AX=16 ° 03 b o .. 0.2 - 0 ° . o O 0 6 A0 0.1 r o ‘ A A A A A A A A 306 o 2 0.0 ’ 68 9 o O 0 9° 0 6 AM . '0'1-1.o -0.6 -o.2 0.2 o 6 1.0 Figure 3.14 Velocity profiles of P1 after the onset of asymmetry. Re“ = 2.5. Axial Velocity 113 0.5 U ' fi U f j 7 °X=1 0.4 ' 0X=8 O ‘ AX=16 o 0.3 P c: 00 O 0.2 ’ O . A 0 A0 A 6 J 0.1 ' A 0 A6 A A A A A go A 2 9 o o 8’ g o o .o'l-L0 -0.6 -0.2 0.2 0.6 1.0 Figure 3.15 Velocity profiles of P1 after the onset of asymmetry. Re“ = 3.0. Axial Velocity 114 0.01 r - . s o 0 our - ° « o ‘ .0.03 - ° - o I 9 '°'°§o.9 .0 7 .0.5 .03 v Figure 3.16 Presence of two vortices in the shear thinning liquid close to Y = -1. Re" = 2.5, X = l. -0.1 115 Such a phenomenon has been reported as a second flow transition in Newtonian liquids at Reynolds numbers much higher than the critical Re for the first flow transition (Durst et al., 1993 and Feam et al., 1990). No other results are known to be reported for any kind of flow transition in inelastic, shear thinning liquids. The presence of three simultaneous vortices close to the expansion plane results in a thin core of the order of the upstream channel height. As a result, a quick look at the velocity profile close to the expansion plane (X = 1 in Figure 3.13) creates an impression of essentially symmetric flow. Figures 3.17 and 3.18 bring out the contrasting behavior between the Newtonian and the non-Newtonian liquid, at Re = Re“ = 2.5. At X = 1 (Figure 3.17), the recirculation zone close to Y = l is much larger in P1, indicating the vortex is more stretched in the y - direction. A wider core is observed in the Newtonian liquid. This is a manifestation of the three vortices in the shear thinning liquid taking up most of the channel height, close to the expansion plane, as is evident fi'om our flow visualization results in Chapter 2 (Figures 2.18 b, c and d). The additional vortex attaches itself to the smaller corner vortex, thereby resulting in a core which is almost symmetrically distributed about Y = 0. Further downstream at X = 8 (Figure 3.18), the largest vortex shrinks in the y - direction as does the vortex close to Y = 1. This results in a wider core in P1. The off - centered peaking is now more obvious because the recirculation zone close to Y = 1 has almost died out but the large central vortex (closer to Y = -l) is still present, resulting in significant asymmetry. Axial Velocity 0.5 0.4 0.3 0.2 0.1 0.0 -0.1 116 fl 0 Non - Newtonian O Newtonian l o Figure 3.17 Effect of shear thinning on the velocity profiles at Reynolds number = 2.5; X =. 1. 1.0 Axial Velocity 117 0.3 . . . . . . . ONewtonian ONon-Newtonian 0.2 - ' ' - e o e 0 ' 0.1 - ° ° .. o O o e. 0 a 0 e °azo 0.0 - ‘9 3 a 8 8 0 r 'v 'o'l-m ‘ -0.6 ‘ -o.2 0.2 0.6 1.0 Y Figure 3.18 Effect of shear thinning on the velocity profiles at Reynolds number = 2.5; X = 8. 118 Figures 3.19 - 3.21 compare the velocity profiles of the shear thinning liquid at X = l, 8 and 16 respectively. The evidence of three simultaneous vortices is seen at Re“ = 2, 2.5 and 3 in Figure 3.19. Based on the ofi‘ - centered peaking, flow appears to be quite symmetric at X = 1. At X = 8 (Figure 3.20) though, peaking at significantly large ofi‘ - centered locations is obvious. The smallest vortex has disappeared and the vortex along Y = 1 has shrunk in the y - direction. Strangely, the peak appears to be more ofi‘ centered at Re" = 2 than at Re“ = 3. This would indicate that the efi‘ect of inertia on the largest vertex is weaker than that on the vortex along Y = 1. At X = 16, all the vortices have disappeared. Flow is still asymmetrical about Y = 0. As shown earlier (Figure 3.11), symmetrical firlly developed flow was confirmed at X = 45. The inferred transverse flow was calculated for the shear thinning liquid using equation 3.3. The results are shown in Figure 3.22. A ranges from 0.5% to 7%. Contrary to what was observed with the Newtonian liquid, A is larger at X = 8 and X = 16 than at X = 1. This could be a manifestation of the three vortices close to the expansion plane hampering flow in the normal direction at X = 1. Results from the streak photography experiments reported in Chapter 2, demonstrated the absence of flow asymmetry in the more shear thinning liquid P2, even up to the highest achievable Reynolds number of 1.6. This was confirmed from our LDV measurements too. The results are shown in Figure 3.23. As mentioned in Chapter 2, the solution P2 is Axial Velocity 119 005 U fi' I I I °Re*=l.0 0.4 ' n - ORe*=2.0 U I"= . 03 Re 30 I: oo . O u 0.2 - a o ‘ 0° 0 a 0.1 " 9 9° ' 08 08 0.0’ 0.800330 .880099. a ° 0 u ° ° ° 8§ a u D I: u .0°l-1.0 -0.6 -0.2 0.2 0.6 Y Figure 3.19 Velocity profiles of shear thinning liquid P1 at X = 1. 1.0 Axial Velocity 120 0.25 ' I 7 U U ' I V D °Re*=l.0 ° F o J ORe*=2.0 a O IllRe"'=3.(l 0.15 - a 0 - D O . o . 3 0 0 o o oo o °°o 0.05 - o o 0 o 3 - o o 0 83° 0 o °¢ O o O O ‘ Q0 0 a u o ‘ a u n a “3 '0'05-1.o A .045 -o.2 0.2 0.6 A Figure 3.20 Velocity profiles of shear thinning liquid P1 at X = 8. 1.0 Axial Velocity 121 0.20 ' 1 V I I f I 1 °Re* = 2.0 A 0 Re" = 2.5 O 0.15 - o . ARe“ = 3.0 a A o o o A 0.10 - 0 o - ° A t o . 6 o t A . 0 § . § § 9 Q . Q l 0.00 J? . . . . . . 2g— -1.0 -0.6 ~0.2 0.2 0.6 1.0 Y Figure 3.21 Velocity profiles of shear thinning liquid P1 at X = 16. A,% 122 » o ORe“ = 1.0 < _ one = 2.0 . ° ARe“ = 25 D * - 1 ll Re - 3.0 l . a o . 0 A b o 1 ’0 ° ‘ .n a a . A o 10 20 so 40 x Figure 3.22 Inferred transverse flow in shear thinning liquid P1. 50 Axial Velocity 123 0.6 U 0.5 0.4 ' 0.3 AX=1 . OX=8 DX=45 Solid line - Calculations . 0.2 0.6 A 1.0 Figure 3.23 Symmetric velocity profiles of P2 at Re“ = 1.5. 124 viscoelastic at high Reynolds numbers. Townsend and Walters (1995) have shown that viscoelasticity dampens the vortex growth in planar expansions. Also based on our experiments, shear thinning too delays the flow transitions. The combined efi‘ect of fluid viscoelasticity and higher pseudoplasticity could explain why flow transitions were not observed in P2. 2.3 Quantification of the degree of asymmetry The normal velocity component at Y = O has been used as an index of the degree of asymmetry by Feam et al. (1990) in their experiments with Newtonian flow through a 1:3 planar expansion. Durst et al. (1993) have used the difl‘erence in the reattachment lengths along the two walls as a suitable measure of asymmetry. Another parameter that may be used is the difi‘erence in the wall shear stresses. As described earlier, practical limitations prevented the measurement of the center line V component of velocity in the present work. The difi‘erence in reattachment lengths requires LDV measurements at very close x - positions to locate the exact reattachment point. The current work uses the center line shear rate as the index to quantify the degree of asymmetry. Non - zero center - line shear rates are indicative of flow asymmetry. Figure 3.24 plots the center - line shear rates for varying Reynolds numbers, for the Newtonian liquid at X = l, 8 and 15. At X = 15 the symmetric flow is obvious from the zero degree of asymmetry observed at all the Reynolds numbers. At Re = 0.6, the center - line shear rate is zero at all axial locations. For Re 2 1.5, a finite asymmetry exists at both the locations X = 1 and X = 8, and it increases with increasing Re. As the fluid moves downstream, the asymmetry reduces. Since the vortices have no preference to attach to any particular wall, there is an equal 125 likelihood of the shear rate being negative. So a mirror - image of the positive shear rates has been used to sketch the whole curve shown in Figure 3.24. A similar plot for the shear thinning liquid at X = 8 and X = 16 is shown in Figure 3.25. The shear rates at X = 1 for P1 have not (been reported because the inflection point of the velocity profiles at X = 1 is very close to Y = O. This has the potential of introducing significant errors. Although the trends observed are similar to those described above for the Newtonian liquid, the magnitudes of the asymmetry in P1 is always higher than that in the liquid N. Figures 3.26 and 3.27 reveal the axial variation of the center - line shear rate for N and P1 respectively. At any x - location, the asymmetry increases with increasing Reynolds number. At Re 2 1.5, Figure 3.26 shows that as the Newtonian liquid flows fi'om X = 1 to X = 8, the center - line shear rate falls down by an order of magnitude before the flow finally becomes symmetric at X = 15. With the shear thinning liquid, the flow is still asymmetric at X = 16 and zero asymmetry is observed only at X = 45. This clearly indicates that the flow length over which asymmetry persists is also higher. 2.4 Bifurcation curves from the experiments Equation (3.5) shows a modified parameter called the degree of asymmetry, D,” which is defined using the center - line shear rate and the axial location. D =—| -X” (3.5) U is the non - dimensional axial velocity and p is a fitting constant selected such that the Center - line shear rate 126 1.0 T 1 V r v I v ' 0N, X = 1 .. _ o d 0.6 ON, X — 8 o > AN, X = 15 o 0.2 r . o O ° -——0 r r t—— O o o -0.2 - '- 0 0 -0.6 " o " ‘1'0 o A 2 3 4 Reynolds number Figure 3.24 Growth of asymmetry with the Reynolds number in the Newtonian liquid. Center - line shear rate 127 1.0 . . - . s . ORX=8 ’ e 0.6 . 0 P, X = 16 . 0 AP, x = 45 ' O 0.2 b a a—+——a -o.2 - O O O -0.6 ~ ' o ’ e '1'" o A 1 2 3 Reynolds number Figure 3.25 Growth of asymmetry with the Reynolds number in the shear thinning liquid P1. Center - line shear rate 0.8 0.6 0.4 0.2 0.0 128 ' oRe=0.6 . ORe= 1.5 A ARe=2.5 . URe=3.5 P O 0"" J 5 W in ‘ *5 X Figure 3.26 Decay of asymmetry in the Newtonian liquid, with increasing flow length. Center - line shear rate 1.0 0.8 0.6 0.4 0.2 0.0 ‘ 129 Figure 3.27 Decay of asymmetry in the shear thinning liquid, with increasing flow length. n ORe“ = 1.0 0Re* = 2.0 P A 4 ARe" = 2.5 ' a Re“ = 3.0 i 0 1 A O ——e—._l—.e.¢ 1 e 1 l -.__ 0 10 20 30 40 50 130 degree of asymmetry at any Reynolds number is the same at both axial positions. Bifurcation curves relating the degree of asymmetry, D,” and the Reynolds number are shown in Figures 3.28 and 3.29 for the Newtonian liquid and the shear thinning liquid respectively. p = 0.9 and 0.6 have been used for N and P1 respectively. Interestingly, p lies very close to the shear thinning index of the liquids used (i.e., 1 and 0.7 respectively). For the Newtonian liquid, flow occurs along branch 1 until Re = 0.6. Flow bifurcates between Reynolds numbers of 0.6 and 1.5 and either of the paths shown by branches 2 and 3 could be followed at higher Re. Branch 4, which is an extension of the symmetric state, is not observed in the experiments. Shapira et al. (1990) and Allebom et al. (1997) have performed a linear stability analysis of Newtonian flows through expansions and have conclusively demonstrated that the branch 4 is indeed unstable and will not be realized in experiments. The polymer solution also exhibits a qualitatively similar bifurcation curve. The bifurcation point is located between Re“ = 1 and 2. At comparable Reynolds numbers, the shear thinning solution exhibits a higher degree of asymmetry than the Newtonian liquid. 3. Computations of flow bifurcation Flow bifurcation curves were computed by using a perturbation - continuation approach. Only a brief description of the method has been included here. Refer Chapter 4 for a description of the technique followed, the details of the solution method and the grid resolution. Finite element calculations were performed on an asymmetric domain for Reynolds numbers spanning O to Re,, where Re, is a Reynolds number greater than the critical Reynolds number. A continuation method was used wherein the results at lower Degree of asymmetry 131 1.0 - u . I u 9N, X = 1 ON, X = 8 o 2 “-5 ’ AN x = 15 ’ c 1 0.0 _t 1 1 JA—— 0 -0.5 " o 3 .1.0 o 1 2 3 Reynolds number Figure 3.28 Bifurcation curve for the Newtonian liquid N. Degree of asymmetry 132 3 ' I 1 j—'— OP, x = s ’ 2 2 OP, X = 16 0 AP, X = 45 l 0 t h—i—i 1 -l O .2 3 0 . 1 . n 4 . 3 0 l 2 3 Reynolds number Figure 3.29 Bifurcation curve for the shear thinning liquid P1. 133 Reynolds numbers were used as initial iterates for computing the solution at higher Re. At Re = Re,, the domain was made symmetric and continuation solutions were computed on the symmetric grid by successively reducing Reynolds numbers. The results from this technique on Newtonian flow through channels with expansion ratios of 2 and 3 showed excellent agreement with the computational results available for such channels. Computations were then performed for planar channels with expansion ratio of 16. A power - law model was used to describe the viscosity of the shear thinning liquid. The computed axial velocity profiles before the onset of asymmetry for the Newtonian and non - Newtonian liquids are compared with the experimental data in Figures 3.4, 3.12 and 3.23. Excellent agreement validates the approach used in the computations. Critical Reynolds numbers of 6 and 18.5 for the onset of flow transitions were obtained for n = l and n = 0.7 respectively. These are higher than the corresponding values observed experimentally. 3.1 Computed predictions of the decay of flow asymmetry Figure 3.30 shows the variation of the center - line shear rate with increasing axial positions, at locations X = 1 and 8 for the Newtonian liquid. The asymmetry decays downstream of the expansion plane for both the Reynolds numbers considered. At the same position, higher Reynolds number results in a higher asymmetry. These trends are consistent with the findings from the LDV experiments reported in Figure 3.26. A similar decay was computed for the shear thinning liquid with n = 0.7. The results at X = 8 and at X = 16 are shown in Figure 3.31, for Re“ = 26, 31 and 48. The computed critical Reynolds number for the first and second flow transitions were 18.5 and 42 respectively. Center line shear rate 134 ’ ORe = 8.3 ARe = 13.3 .. A 4 o b- d ‘ A O 0 2 4 6 8 X Figure 3.30 Computed decay of asymmetry in the Newtonian liquid. 10 Center line shear rate 135 ORe"=26 ARe*=3l uRe*=48 Figure 3.31 Computed decay of asymmetry in the shear thinning liquid. 136 For all the three Reynolds numbers reported in Figure 3.31, the flow asymmetry reduces as X increases. At any location, higher Re“ results in a higher flow asymmetry. As opposed to the Newtonian flow where flow asymmetry had subsided by X = 15, flow of the shear thinning. liquid is considerably asymmetric even at X = 16, confirming the earlier experimental observation that shear thinning results in a slower decay of flow asymmetry and consequently a longer flow length up to which asymmetry in the flow persists. 3.2 Velocity profiles from the perturbation - continuation approach Figure 3.32 shows the computed velocity profiles at various axial positions for the Newtonian liquid at Re = 8. At X = 5, the two recirculation regions are clearly seen. The velocity peaks slightly away from the center line. At X = 20 the smaller vortex is no longer present and the velocity peaks much closer to Y = 1 than at X = 5. Flow is firlly developed at X = 75. The velocity profiles shown in Figure 3.32 is qualitatively similar to the ones obtained experimentally (Figures 3.5 through 3.7). The velocity profiles at Re = 25 are depicted in Figure 3.33. At this Reynolds number, the second flow transition has already occurred and three vortices are present. At X = 5, the two recirculation regions representing the two comer vortices are seen. The smaller corner vortex is no longer present at X = 30 and at X = 60 the third vortex is inferred on the wall on which the smaller comer vortex had attached itself close to the expansion plane. Figure 3.34 illustrates the computed velocity profiles of the shear thinning liquid at Re“ = 20. A flow transition fi'om a state of two symmetrical vortices to two asymmetrical Axial velocity 137 0.5 e in 0.1 * DX=5 OX=fll D AX=75 a D a G u D 1.0 Figure 3.32 Computed velocity profiles of the Newtonian liquid at Re = 8. Axial velocity 138 0.7 . a . . . . . ax=5 #1 OX=30 D 05' AX=60 D ‘ D ”41.0 ‘ -0.6 A -o.2 0.2 ‘ 0.6 1.0 Figure 3.33 Computed velocity profiles of the Newtonian liquid at Re = 25.3. 139 vortices is observed at this Reynolds number. This flow transition was not detected in the corresponding LDV experiments. The flow transition is obvious with the two asymmetric corner vortices coexisting at X = 5. By X = 15 and X = 20, only the larger corner vortex exists. The computed velocity profiles at Re“ = 44 corresponding to the second flow transition in the shear thinning liquid are shown in Figure 3.35. At X = 5, two recirculation regions are observed. Only the larger comer vortex exists at X = 30 and at X = 45 the third vortex is confirmed on the wall on which the smaller corner vortex had attached itself close to the expansion plane. Streamlines from the computations always showed the third vortex to attach itself far downstream of the expansion plane. The LDV measurements (and the flow visualization), however, revealed that the third vortex was located on the walls at X = O. 3.3 Comparison of experimental and computed bifurcation curves The degree of asymmetry was calculated at Re = 8.33 and 13.33 for the Newtonian liquid and at Re" = 26 and 31 for the shear thinning liquid with n = 0.7. The same values of p as that used in the experiments were employed to determine the degree of asymmetry from the computations. To account for the differences in the experimental and the predicted critical Reynolds numbers, a modified Reynolds number was defined as - Remod=Re-Re - Re‘mod=Re‘-Re‘. (3.6) Cf" ’ Cf" The experimental critical Reynolds number was used to evaluate the experimental modified Reynolds number and the computational modified Reynolds number was calculated from the computational critical Reynolds number. Figure 3.36 illustrates the Axial velocity 140 0.5 - 1 . u u - D a X — 5 r0 O X = 15 I: AX = 20 D 0.3 L a D b D 0.1 " .0J-l.0 -0.6 -0.2 0.2 Figure 3.34 Computed velocity profiles of the shear thinning liquid Pl at Re“ = 20. Axial velocity 141 0.8 u D X = 5 0.6 " OX = 30 .. AX = 45 0.4 ' " 0.2 " ‘ AAA ‘ ‘ 0.0 an O a a an . 0° 0 '02-].0 -0.6 '02 0.2 0.6 Y 1.0 Figure 3.35 Computed velocity profiles of the shear thinning liquid Pl at Re“ = 44.3. 142 modified bifiircation curve for the Newtonian liquid. Only the positive half is shown for purposes of clarity. Increasing the Reynolds number increases the degree of asymmetry for both the computations and the experiments. D. evaluated from the experiments seem to level ofl‘ in comparison with that obtained from the computations. In the shear thinning liquid, however, a continuity is apparent between the experimental and the computed degrees of asymmetry (Figure 3.37). 4. Conclusions Laser Doppler velocimetry was used to obtain detailed information on the velocity profiles of Newtonian and non - Newtonian liquids flowing through a 1:16 planar channel. Reynolds numbers between 0.6 to 3 .5 and 1 to 3 were spanned for the Newtonian liquid and the shear thinning polymer solution with a power - law index of 0.7 respectively. The velocity profiles at various axial locations were used to make detailed observations on the dynamics of vortex growth at Reynolds numbers above the onset of flow transitions. The center - line shear rate was used as a measure of the degree of asymmetry and plots were drawn to show the flow bifurcation in these liquids above the critical Reynolds number. The Newtonian liquid experienced flow transition between Re = 0.6 and 1.5. Results from the flow visualization experiments had indicated that at Re = 0.8, flow transition had set in in the Newtonian liquid. At Re 2 1.5, flow was asymmetric close to the expansion plane (X = l) and also at X = 8. All asymmetries decayed by X = 15. The second flow transition to a state of three vortices was not observed for the range of Reynolds numbers studied. 143 7 v u . u w u 0 Experiment 6 - A - A Computation ca 5 I- u E“ a 4- - 8 .5 3 b d A i so a 2 P . l ' .. 0 ° 0 a A l A l A l 0 0 2 4 6 8 Remod = Re - Rec,“ Figure 3.36 Comparison of the degree of asymmetry from LDV experiments with that from the FEM computations for Newtonian flow. Degree of asymmetry, D,ls 144 A _ OExperiment . A Computation b A d D O C 0 ho a a l l 0 5 10 Remod = Re - Rec,“ Figure 3.37 Degree of asymmetry for the polymer solution P1. 15 145 At Re"I = 1, the shear thinning liquid showed symmetric velocity profiles at all the axial locations. It also showed a flow transition to the simultaneous presence of three vortices at Re“ = 2 and above. The flow transition to the state of two asymmetrical vortices occupying the comers of the larger channel was not detected by the experiments with the pseudoplastic liquid. Shear thinning, therefore, seems to hasten the onset of the second flow transition experienced by the Newtonian liquids at very high Reynolds numbers. Asymmetry in the flow in terms of the center line shear rate was observed to decrease downstream of the plane of expansion for both liquids. However, the degree of asymmetry in the shear thinning liquid was greater than that in the Newtonian liquid and it also persisted for a longer flow length. The shear thinning liquid with a power - law index of 0.5 (liquid P2) revealed symmetric profiles up to the maximum achievable Reynolds number of 1.5. Fluid viscoelasticity at high Reynolds numbers and a higher pseudoplasticity could be responsible for the delayed flow transitions. Flow bifiircation curves were computed using a perturbation - continuous approach for liquids with power - law shear thinning indices of l and 0.7. The predicted bifurcation points were higher than those obtained from experiments. However, the computed trends of higher bifurcation points and of a greater degree of asymmetry with increasing shear thinning were the same as that observed experimentally. Also, computations predicted the trends of decaying flow asymmetry with increasing axial positions. The computed velocity profiles demonstrated both the flow transitions for the Newtonian and shear thinning liquids. 146 The efl‘ects of shear thinning may be summarized as: (1)to delay the onset of the first flow transition, (2) to hasten the onset of the second flow transition, (3) to raise the degree of asymmetry at comparable Reynolds numbers and (4) to cause the asymmetry to persist for a longer flow length. Chapter 4 COMPUTATIONS OF SYMMETRY BREAKING FLOW BIFURCATION IN ABRUPT PLANAR EXPANSIONS 1. Introduction Flow of fluids through geometries with abrupt changes in cross section is commonly encountered in various engineering operations. Such flows are firrther complicated by inertia or by fluid nonlinearities such as pseudoplasticity, stretch thickening, yield stress or viscoelasticity. While the literature is replete with the description of converging flows (see reviews by White et al., 1987 and Boger, 1987 and 1997), the corresponding diverging flows have not evoked comparable attention. Only in the case of creeping flow of Newtonian liquids will the flow features in an expansion be a mirror-image of that in a contraction flow. Due to the nonlinearities in other cases, no direct inference for polymers flowing through expansions can be made based on corresponding contraction flow results. 2. Background 2.1. Newtonian flow transitions in an abrupt planar expansion 2.1.1. Existing experimental results Sobey (1985) has studied the flow patterns developed in a Newtonian liquid (water) flowing steadily through a two - dimensional 1:3 planar expansion. He observed that at 147 148 low flow rates (or low Reynolds number, Re, defined using the smaller channel half height and the average velocity in the upstream channel), the corner vortices were symmetric and that they increased in size as Re was increased. The first flow transition was observed beyond a certain critical Reynolds number, Rem (around 25 for an abruptly expanding channel), when flow became asymmetric and one vortex grew more rapidly than the other. In mathematical terms, the flow is said to have bifirrcated at Recl into two possible stable solutions (both exhibiting asymmetric flow), with the pre-bifirrcated symmetric solution now becoming unstable. As Re was raised further, a second flow transition took place at a critical Reynolds number, Red, leading to three vortices, two along one wall and one along the other. The steady flow became periodic at higher Re before finally turning turbulent. The critical Reynolds numbers were observed to be higher for channels with gradual expansions. By using long rectangular channels of large aspect ratios, i.e., the ratio of the width of the channel to its height, Sobey ensured that the flow far away from the expansion plane was one dimensional. Experiments showing similar flow transitions in Newtonian fluids through abrupt expansions have been reported by Durst et al. (1974) and Cherdron et al. (1978) and confirmed later by Feam et al. (1990) and Durst et al. (1993). Cherdron et al. (1978) have investigated the effect of the expansion ratio (B) and the aspect ratio on the flow patterns developed in a Newtonian liquid flowing through a planar expansion. They have reported that the critical Re at which the first flow transition occurs goes down with an increase in the expansion ratio as well as an increase in the aspect ratio. For example, with a channel of aspect ratio 8, the critical Re goes down from about 150 to 30 in going fiom an area expansion ratio of 1 :2 to 1:3. The mechanism of the 149 initiation of such flow transitions, even for Newtonian liquids, is not well understood. However, the Coanda efl‘ect does seem to explain how it is sustained. Flow asymmetry is a result of the momentum transfer between the shear layers in the direction normal to flow. As a result, the boundary layer adjacent to one wall is richer in momentum and consequently at a lower pressure as compared to the other. A transverse pressure gradient in the channel is created and as more liquid enters, flow of the liquid from the wall at higher pressure to that at a lower pressure takes place. This increases the momentum at the richer wall even more resulting in a more pronounced efl‘ect of the flow asymmetry. No flow asymmetry has been reported in axisymmetric expansions, where the flow induces continuous concentric shear layers, as opposed to the stacked shear layers in planar flow. Some scatter in the critical Reynolds numbers reported is evident in the literature. The Reynolds number used in the present work is defined in equation (4.1). =hUmp 2n Re (4.1) Here, h is the upstream channel height, U" is the average velocity in the upstream channel and p and u are the fluid density and viscosity respectively. Cherdron et al. (1978) reported that Recl was around 62 for flow in a channel with a 1:2 expansion ratio and with an aspect ratio of 8 or more in the larger channel. Mth a similar channel, Durst et al. (1993) observed flow asymmetries at Re = 42. In a channel with an area expansion ratio of 3, Durst et al. (1974), Sobey (1985) and Feam et al. (1990) reported that Newtonian flow became asymmetric at Re of 38, 25 and 22 respectively. In our experiments (reported in 150 Chapters 2 and 3) with a much higher expansion ratio of 16, asymmetric flow sets in at Reynolds number of 0.8. 2.1.2. Prediction of Newtonian flow bifurcation using computations Various numerical procedures have been used to predict the flow bifurcation in a planar sudden expansion. Computations involving finite elements have always needed some kind of perturbation - either to the geometry or to the boundary conditions - to yield a bifurcated flow structure. Durst et al. (1993) have made transient calculations to predict the onset of flow transitions for a Newtonian liquid. They followed a perturbation approach which involved the following steps: At time t = O, a firlly developed velocity profile was imposed at the inlet of the smaller channel. After n time iterations and during m time iterations, the inlet velocity conditions were modified such that the axial velocity component (U) was a function of time and the normal velocity component (V) was a function of both time and space. Subsequently, the original symmetric fully developed velocity profile was restored as the inlet boundary condition. The solution was allowed to achieve steady state. Using this approach a critical Reynolds number of 42 was predicted for flow through a 1:2 expansion. F earn et al. (1990) used numerical bifirrcation techniques applied to a finite element discretization of the two - dimensional Navier - Stokes equations and predicted flow bifurcation in a 1:3 planar expansion at Re,1 of 27. Their work sheds more light on the sensitivity of the bifurcation point to experimental uncertainties. They suggest that the critical transition point is structurally unstable. The slightest imperfection in the 15 1 experiment may lead to a discontinuity in the bifurcation curve, with a shift in the original bifurcation point. They showed that a vertical shift in the grid of the larger channel by 0.42% with respect to the axis of symmetry provided much closer match with the experimental data. Their work seems to explain the possible reason for the scatter observed in the experimental results on flow bifiircations through planar expansions. Indeed , experimental imperfections could have many sources such as geometrical asymmetry, upstream flow asymmetry, momentary mechanical shock, temperature variation, etc. Teschauer (1994) employed an asymmetric upstream channel to compute the bifurcated branch of the solution for various expansion ratios between 1.5 to 3. A commercial finite element code was used. She predicted critical Reynolds numbers of 72 and 27 for expansion ratios of 2 and 3 respectively. In a different flow configuration involving Newtonian flow into a rectangular channel through two symmetric openings, Goodwin and Schowalter (1996) have shown the possibility of the simultaneous existence of numerous solutions beyond a critical Reynolds number. To access the asymmetric solutions, they have followed a continuation approach coupled with a perturbation in the flow rates in the two channels. Using a finite element discretization, solutions with the asymmetrical flow rates were computed for increasing Reynolds numbers. Results at the lower Reynolds numbers were used as initial iterates for computations at higher Reynolds numbers. At significantly high Reynolds numbers, the flow was rebalanced and the same continuation approach was used for successively 152 decreasing Reynolds numbers. Such an approach detected the various asymmetric branches of the solutions. A similar approach using continuation and a perturbation in the geometry to compute the flow bifurcation in planar expansions with a single inlet has been devised in the present work. This will be discussed later. Very recently numerical results using a finite volume approach for flow through planar expansions have been presented. A striking feature of such an approach is that flow bifirrcation has been computed without providing any kind of perturbation to the flow conditions. Drikakis (1997) has presented bifirrcation curves fi'om several schemes for expansion ratios up to 6. Various numerical schemes based on an overall finite volume approach have been tested. His results for the onset of asymmetry with expansion ratios of 2 and 3 match the corresponding results of Teschauer (1994) and the results from the linear stability analysis of Shapira et al. (1990). Foumeny et al. (1996) have shown that a commercial code, FLUENT, can be effectively utilized to study the flow bifurcations. This code employs a finite volume discretization procedure, in which linear approximation fiinctions are used to interpolate values of the flow variables throughout the solution domain. Their focus is on obtaining results on channels with more than one inlet opening. A characteristic observation from the computational results is that flow bifirrcation calculations almost invariably predict a higher critical Reynolds number than the corresponding value obtained in experiments. This is consistently observed in the work described above on channels with low expansion ratios of 2 and 3 and also for a channel with a more severe expansion ratio of 16, the computational results for which are reported 153 in the present work. The corresponding experimental findings for the 1:16 channel have been presented earlier in Chapters 2 and 3. Sobey (1985) and Sobey and Drazin (1986) have attempted to relate the experimentally observed bifurcation to that in Jeffery - Hamel (II-I) flows. In the latter, radial flow occurs between two inclined plates intersecting at an angle 2a. Flow is generated by a source located on the line of intersection. JH flows have been shown to bifiircate subcritically, leading to no stable flow above the critical Reynolds number. Planar expansion flows, on the other hand, display a supercritical bifurcation which is confirmed by several reports of stable asymmetric patterns in planar expansions. Sobey, therefore, concluded that 1H flows are not of any significance in explaining expansion flow after bifirrcation. Shapira et al. (1990) have performed a linear stability analysis of flow in symmetric expansions. They have considered a gradual expansion with a constant slope of the channel walls. Although their predictions of Recl = 27.5 for a 1:3 expansion are in agreement with the computational results of Feam et al. (1990), whose computations suggest the onset of asymmetry at Re of 27, they over predict Rec, of 72 for a 1:2 expansion. More importantly their computations show that the symmetric branch of the solution obtained above the critical Reynolds number is unstable and therefore unlikely to be ever witnessed in experiments. Allebom et al. (1997) have performed a linear stability analysis on flows through abrupt expansions. Finite difference approximations of the equations of motion in the stream 154 function - vorticity form have been used. The bifirrcation picture is extended by computing the subsequent bifurcation point (Re,,_) and solution branches. Solutions for infinite expansion ratio have been compared with Jefl‘ery - Hamel flow. They conclude that away fiom the expansion plane flow profiles do approach the profiles of JH flow. 2.2. Non - Newtonian flow through expansions Still much work remains to separate the contributions of inertia, shear thinning and stretch thickening viscosities, elasticity, expansion ratio and the mode of expansion (axisymmetric vs. planar) on the flow patterns in expansions. Abdul-Karem et al., (1993) have investigated flow behavior of 0.05% polyacrylamide solution in glucose syrup (Boger fluid) through a 116.8 axisymmetric expansion and a 6.8:] axisymmetric contraction. Although the vortex size observed in expansions was lower than that in contractions, the trend of vortex enhancement with increasing flow rate was observed in the expansion flow too. No lip vortices or instabilities were observed in either configuration. Halmos et al. (1975) have conducted experiments using aqueous carboxymethyl cellulose solution (inelastic, shear thinning power-law index of 0.73) in a 1:2 abrupt axisymmetric expansion. They have measured the radial and axial velocity profiles downstream of the expansion plane using flash photography. Their experimental results on velocity profiles and reattachment lengths agree well with their calculations for Reynolds numbers between 11 to 125. The authors do not observe any flow asymmetries, oscillations or lip vortices. Townsend and Walters (1994) have studied the flow of a 0.15% aqueous solution of - polyacrylamide (slightly shear thinning, strongly elastic) through an expansion from a 155 square section to a rectangular slit (area expansion of 13 .3) and from the rectangular slit to another square section (area expansion of 13 .3). With a Newtonian liquid, significant vortex activity was observed due to fluid inertia. The vortex size increased with the flow rate. The polymer solution, on the other hand, produced small corner vortices, the size of which decreased with the flow rate. Fluid elasticity thus, was observed to inhibit vortex growth. It should be pointed out that their study with Newtonian liquids has not shown any evidence of flow asymmetry, in contrast to those reported by Durst et al. (1974), Cherdron et al. (1978), Sobey (1985) and Feam et al. (1990), despite a wide range of Reynolds numbers used. The square channels used by Townsend and Walters (1994) approximate axisymmetric flow which has never been known to show the flow asymmetry mentioned above. In addition, based on the findings of Cherdron et al. (1978) that the critical Reynolds number for the onset of flow asymmetry increases with decreasing channel aspect ratio, one might conclude that at an aspect ratio of 1, flow asymmetry might be observed, if at all, only at very high Reynolds numbers. One notable contribution of the Townsend and Walters work was to clearly bring out the effect of fluid elasticity on the vortex growth in planar expansions. The observed trends in the efl‘ects of fluid inertia and elasticity on secondary flows was in contrast to what had been observed in various contraction geometries, where fluid inertia reduced the vortex size while elasticity led to vortex enhancement. This reversal of roles may be the reason for lack of further investigation of viscoelastic effects in expansion flows. No results demonstrating the effect of pseudoplastic flow behavior on the bifurcation phenomenon, even for lower expansion ratios are available in literature. 156 3. Objectives Experimental evidence of Newtonian flow transition at expansion ratios higher than 3 is non - existent. Also conspicuously absent is any indication whether non - Newtonian flows will show flow bifirrcation at high Reynolds numbers. The present study seeks to extend the findings of Cherdron et al. (1978) by experimentally locating the flow bifirrcation in channels of expansion ratio 1:16. Our detailed observations on the flow visualization and laser Doppler velocimetry experiments carried out with Newtonian and non - Newtonian liquids have already been reported in Chapters 2 and 3 respectively. In the present Chapter, the corresponding computational results have been discussed. The unique feature of this work is the determination of the effect of non - Newtonian viscosity on the occurrence of flow bifurcation in planar channels with a high expansion ratio of 16. A power - law model has been chosen to represent the shear thinning viscosity of the fluids. The parameters have been based on the properties of the polymer solutions used in our earlier experiments. Two shear thinning indices of 0.5 and 0.7 have been investigated. A commercial finite element code, FIDAP (Fluent, Inc), has been employed for solving the equations of motion. A perturbation - continuation approach has been developed to study the flow bifirrcation in channels with expansion ratios of 2, 3 and 16. Results showing the effect of pseudoplasticity and expansion ratio on the excess pressure drop and on the flow resistance have been presented. A comparison of flow through a 1:16 expansion with that of Jeffery - Hamel flow has been included in Appendix A. 157 4. Numerical scheme Steady, twoodimensional finite element calculations were performed to predict the critical Reynolds number for the onset of asymmetry. A commercial code FIDAP (Fluent, Inc.) was employed for this purpose. 4.1 Problem definition The steady, two - dimensional, isothermal flow of an incompressible fluid through an abrupt expansion (Figure 4.1) is described by (BUx 6U), O 42 + _ = 6x 8y ( ' ) (U 6U): U aux) [61:10: 61”] 3p 4 3 + = + _ - _ + p ‘ ax ’ 6y 8x 8y 5x pg, ( ' ) 6U 6U 61: at a U—1 + U y = xx + W - P + 4.4 .1. = k1" (4.5) where x and y are the distances along and normal to the direction of bulk flow respectively, U,I and Uy are the axial and normal components of velocity, rii are the components of the stress tensor 1:, y is the shear rate tensor, p is the pressure, p is the 158 X Figure 4.1 Schematic of the flow channel used in calculations. 159 density and g is the gravitational constant. k and n are the consistency index and the shear thinning index used to define the pseudoplastic viscosity of the non - Newtonian fluid. Expansion ratios of 2, 3 and 16 and shear thinning indices of 0.5, 0.7 and 1 were investigated. 4.1.1 Scaled variables U U U: ”,1/= y ,X=£;y=.l_ Um Um h _B_}1 2 Um is the maximum velocity at the inlet of the upstream channel and h is the height of the upstream channel. [3 is the expansion ratio. The domain of the problem is now -11 < X < 12 and -1 < Y < 1. l1 and 12 chosen were 5 and 65 step heights (i.e. (B - 1)/B) respectively. Reducing their values by 50% changed the solution only by 0.01%. 4.1.2 Boundary conditions U(O,:h%sYsil) = O U(X,:L~%) = V(X,:t-[1;) = U(X,i1) = V(X,:+:l) = 0 1+— U(-11,Y) = 1 - Y "; V(-I,,Y) = o 160 4.2 Perturbation - Continuation approach Our steady state computations for Newtonian flow through a 1:3 planar expansion using a symmetric grid failed to show any significant flow asymmetry fi'om Re = 0 to 40. Recall that the critical Reynolds number for this case is around 27. The calculation protocol was then modified by incorporating a grid perturbation method. Figure 4.2a illustrates schematically the procedure followed. An asymmetry was introduced in the geometry of the configuration by shortening one of the steps from .111 to IH. This resulted in IH being about 10% shorter than the step ON. The resulting asymmetrical domain A is shown in Figure 4.2a. The Stokes solution was then computed for this asymmetric channel. Using the Stokes solution as the initial iterate for the next run, the equations of motion were solved for a higher Reynolds number. For every subsequent Re, the result of the previous computation was used as the initial guess. This procedure was continued until point b, where the Reynolds number was much above the expected Red. The resulting path is shown in dashed lines in Figure 4.2a. At point b, the computational grid was made symmetric again (Domain S). The solution was then computed for the symmetric domain using the results at point b on Domain A as the initial iterate. Subsequently the continuation method was repeated on the symmetrical grid with the Reynolds number now being reduced gradually fiom point c to e. A point d, called the bifurcation point (or the critical Reynolds number) was crossed over, below which the flow was essentially symmetric. We call this whole approach a perturbation - continuation approach. The step size of Re was anywhere from 0.25 to 2. The solid lines (edc and edc’) reveal the bifurcation curve obtained by following the continuation - perturbation approach. At low Reynolds numbers, the degree of asymmetry is zero. Above the critical Reynolds number, Degree of Asymmetry 161 J K I II_II_II—II—II-II.L G F o N M Domain A: Asymmetric (FGHILMNOF) Domain S: Symmetric (FGHJKMNOF) A - .. _ .. Asymmetric grid Symmetric grid b Reynolds number (Re) Figure 4.2a Schematic of the continuation - perturbation approach. 162 the degree of asymmetry starts increasing with Reynolds number. The curve edc’ would be obtained if the perturbation in the channel wall were made such that JH would be longer than ON. The final solution was not dependent on the amount of perturbation provided to the grid. Checks made with 2%, 10% and 20% asymmetries resulted in identical bifurcation curves. Figure 4.2b shows the various steps involved within the continuation approach. A continuation approach carried out at Reynolds numbers above points c or c’ on a symmetric grid yielded the second flow transition reported by Feam et al. (1990) and Durst et al. (1993), etc. Interestingly, our flow calculations revealed that the branch of the solution representing this second flow transition which shows the simultaneous presence of three asymmetric vortices could be reached by a steady state, two dimensional computation on a symmetric grid alone, without using the perturbation approach and by starting from Stokes solution on a symmetric grid. The degree of asymmetry may be represented by several indices. These include the difference in the reattachment lengths on the two walls, the difference in the wall shear stresses, the center line normal velocity component or the shear rate in the center of the channel. The difference in the reattachment lengths at the two walls normalized by the step height was used as the measure of asymmetry in the present work. To evaluate the reattachment length, the sign of the axial velocity was monitored at the nodal layer closest to the walls and two successive points with negative and positive u- velocity were identified. A simple linear interpolation of the form of equation (4.6) then yielded the reattachment length. This was then normalized with the step height and was 163 Post . Compression of Processing key files FORTRAN Program UNIX Sh ll Figure 4.2b Steps involved in the continuation approach. 164 referred to as L, U.+ x+ -x,. x =x'.+1 " ’2; i 1 U ) (4.6) 1+1 i 4.3 Finite elements grids Nine node isoparametric quadrilateral elements were used in the computations. Biquadratic and discontinuous linear interpolating functions were chosen for the velocity and pressure representation. A mixed discretization for the pressure was used. The Newton-Raphson method was employed to obtain the nonlinear steady solution. Successive substitution was also tried and it yielded the same results. However, the rate of convergence for the latter method was slower due to its asymptotically linear convergence rate (as opposed to the quadratic rate of Newton—Raphson method). The solution was assumed to have converged when the maximum difference in the velocity between two iterations was less than 10“ times the velocity in the earlier iteration. The convergence criterion for the residual was also set to 10" . To investigate the effect of grid resolution on the outcome of our calculations, three grids - Gl, GZ and G3 were designed with 2351, 5871 and 11431 nodes respectively. The mesh was graded finely in all the comers and was less dense away from the comers. Figure 4.1 schematically shows the variation of the grid density in the channel. In the axial direction (i.e., along the x axis), the mesh density was the maximum close to the x = 0 plane. In the transverse direction, the mesh was more dense near both the 90° corners (y= i 1) and the 270° corners (y = :1: 1/13) and was less dense in between. The bifurcation point for a 165 channel with an area expansion ratio of 3 was used to compare the performance of the three grids. Figure 4.3 illustrates the result. 61 and 62 produced results to within 0.1%. The performance of 62 and G3 was nearly identical. Future results have been computed on the grid G3. 5. Results and Discussion 5.1 Flow bifurcation in expansion flows 5.1.1 Validation of the perturbation - continuation approach To test the accuracy of the continuous - perturbation approach, our findings were compared with the existing computational results of Newtonian flow through 1:2 and 1:3 planar expansions. Figure 4.4 demonstrates the three branches of the bifirrcation curve which result fi'om the perturbation - continuation approach for a channel with expansion ratio 3. The difference in the reattachment lengths on the two walls normalized by the step height is used as the index of the degree of asymmetry in Figure 4.4 (and in subsequent bifirrcation curves). Up to Re = 27, no asymmetry exists (i.e. the diflerence in the reattachment length is zero). This stable branch (1) is the one that is picked up experimentally. At Re greater than 27, the vortex lengths become unequal. The degree of asymmetry increases with increasing Reynolds number. Either of the branches 2 or 3 may be followed at Re > 27. At a critical Reynolds number of 27, the unique solution (1) is said to have bifurcated into multiple solutions (2 and 3). The branch of the solution representing symmetry beyond the critical Re (branch 4) is the one that will be picked up by computations without using the perturbation - continuation approach. Durst et al. (1997) have recently performed a stability analysis and have shown that the branches 1, 2 Difference in reattachment length 166 Acr 0G2 x G3 I, ‘. r . i . ' K s ‘c 30 Reynolds number Figure 4.3 Effect of grid refinement on bifurcation curve. Newtonian flow, Expansion ratio = 3. 35 Difference in reattachment length 167 . 8 ' U T I I r x Asymmetric grid 4 ’ O Symmetric grid ' 4 0 ..... ~4- - '8 A J a l a l 4 7 0 10 20 30 40 Reynolds number Figure 4.4 Demonstration of the results using the perturbation - continuation approach for Newtonian flow through a 1:3 planar expansion. 168 and 3 are indeed stable solutions and branch 4 is the unstable solution and therefore would not be observed experimentally. The predicted onset Reynolds number of 27 for Newtonian flow through a 1:3 planar expansion using the perturbation - continuation approach is in very close agreement with the computations of Feam et al. (1990), which also predict the onset of flow asymmetry at the same Reynolds number. The corresponding computations for an expansion ratio (B) of 2 showed flow bifurcation to occur at 72. This bifurcation point is in close agreement with the computational results of Shapira et al. (1990) and Drikakis (1997) but is higher than the experimental findings of Cherdron et al. (1978) and those of Durst et al. (1993). Figure 4.5 shows the bifirrcation curve obtained in this work. The difl‘erence in the reattachment lengths of the two vortices has been used as the degree of asymmetry. Another commonly used measure of the degree of asymmetry is the normal velocity at the center line (Y = O). The bifurcation curve using the V - component is illustrated in Figure 4.6. Non - zero V at X = -O.5 indicates that the fluid anticipates the enlargement even before reaching the expansion plane. For the purposes of clarity, only half of the bifurcation curves are shown at various axial locations. The degree of asymmetry increases fi'om X = O to X = 1.25 and then falls down further downstream. Between Re of 70 to 85, symmetry was regained at X = 15 when the flow became firlly developed. Difference in reattachment length 169 10 u u u I 6 . 2 .. .2 - c ........ -6 - '1070 72 7l4 7.6 71 Reynolds number Figure 4.5 Bifurcation curve for a Newtonian liquid in a 1:2 expansion. Normal velocity at center - line Y = 0 170 0.06 . r . u . r T r x = b 1.25 2.5 0.04 " i 5 0.02 - 0 ’ -o.s 0“0070 74 A 78 A 82 86 Reynolds number Figure 4.6 Bifurcation curve using center - line velocity as the degree of asymmetry for a Newtonian liquid through a 1:2 expansion. 17 1 5.1.2 Use of the perturbation approach to study Newtonian flow bifurcations in a 1:16 channel The computations for a Newtonian liquid flowing through a 1:16 planar channel, similar to the one used in our optical experiments (reported in Chapters 2 and 3), revealed that the critical Reynolds number was around Re = 6. The corresponding bifirrcation curve is shown in Figure 4.7. The computations predicted a higher critical Reynolds number than that observed in our experiments. As mentioned earlier, such an over prediction has also been observed by other workers with 1 :2 and 1:3 channels. The lowering in the experimental critical Reynolds number for the onset of flow bifirrcations could be brought about by uncertainties in the experimental configurations. Computations for a 1:16 channel are also significantly different from the corresponding 1:3 channel in the far severe comer singularity and the required more dense mesh grading close to the corners in the former. The effect of geometrical asymmetry on the lowering of the critical Reynolds number in a 1 :16 channel is shown in Figure 4.8. Only half of the bifirrcation curve has been included for purposes of clarity. In this case, one of the steps forming the expansion has been” shortened and continuation calculations have been made on such an asymmetric domain. Grid asymmetry is defined as Grid asymmetry = 100 % ‘2" where H is the height of the larger channel and AH is the reduction in the step height. The results indicate a finite degree of asymmetry even at low Reynolds numbers. A grid Difference in reattachment length 172 3 . . . 1. .1- '32 :1 a i Reynolds number Figure 4.7 Bifurcation curve for Newtonian flow in a 1:16 expansion. Difference in reattachment length 173 18 . . J 03.1% 15 ' 01.25% ' ' 110.6% ‘ 12 - 0% « 9 - . 6 n- -r l 3 P q D a u 4 o M3 Reynolds number Figure 4.8 Effect of geometrical asymmetry on Newtonian flow bifurcation in a 1:16 channel. 10 174 asymmetry of 3% results in shifting the critical Reynolds number to values lower than 2, an almost 70% reduction from the value of 6.3 calculated with zero grid asymmetry. 5.1.3 Effect of non - Newtonian behavior on flow bifurcation in a 1:16 planar expansion As far as this author is aware, no results - experimental or computational - indicating the effect of shear thinning on the flow bifurcation in planar channels have ever been reported previously. The present computational work brings out the efl‘ect of non - Newtonian behavior on the critical Reynolds number for the onset of flow asymmetries in planar channels. The corresponding experimental findings have been discussed in Chapters 2 and 3. A generalized Oswald-dc Wale power - law viscosity model ( equation (4.7)) was used to describe the viscosity of the shear thinning liquid. The parameters used are shown in Table 4.1. n = k (t)‘"‘ " (4.7) Here n is the shear viscosity, 7 is the shear rate and k and n are rheological constants called the consistency index and the shear thinning index respectively. 175 Table 4.1: Parameters used in the viscosity model Designation n k (Pa-s') P1 0.7 7.82 P2 0.5 77.46 Since the viscosity of the polymer solution is dependent on the shear rate, equation (4.8) was used to define the Reynolds number (denoted by Re") of the shear thinning solutions. This took into account the power-law effect of shear thinning. The halfheight of the upstream channel, the upstream average velocity and the wall shear rate in the upstream channel were taken as the characteristic parameters to define the Reynolds number. n 2-n h Um,g p Re. z 2(1+2n)]n-1 (4‘8) 2H The computations to obtain the flow bifurcation curve for n = 0.7 in a 1:16 channel yielded about 18.5 as the critical Re’. Shear thinning, therefore, delayed the onset of asymmetry in a 1:16 planar expansion. The bifurcation curve for n = 0.7 is shown in Figure 4.9. Until Re" of 18.5, flow is symmetric and a zero degree of asymmetry is observed. At higher Reynolds number, flow becomes asymmetric and the degree of asymmetry rises to around 3 for almost a 100% increase in Reynolds number above the critical value. With increasing shear thinning (n = 0.5), bifirrcation was observed at an Difference in reattachment length 176 5 - . . . . . a 3. 1. .1- .3- '510 15 ‘ 20 25 A 30 35 Reynolds number Figure 4.9 Bifurcation curve for n '= 0.7, B = 16. Difference in reattachment length 177 45 b c : : : : : : : : : : : 1 o; t 15 20 25 30 35 40 Reynolds number Figure 4.10 Bifurcation curve for n = 0.5, B = 16. 178 even higher Reynolds number of around 27.5. Figure 4.10 demonstrates the corresponding bifurcation curve. Thus shear thinning clearly results in delaying the onset of the flow asymmetry in abrupt planar expansions. 5.2 Flow patterns during transitions in planar expansions 5.2.1 Newtonian liquids The various flow transitions in a Newtonian liquid flowing through a channel with B = 2 are shown in Figures 4.11a through 4.11d. Figure 4.11:: represents the symmetric state at Reynolds number of 38, which is less than Re,l (which for this case is 72). Figure 4.11b reveals the flow patterns at Re = 77. A distinct asymmetry is observed in terms of the difi‘erence in the reattachment lengths. This asymmetry increases at higher Reynolds numbers (seen in Figure 4.1 1c) before the second flow transition occurs (at around Re = 200) leading to an additional vortex on the wall with the smaller vortex (Figure 4.11d). Computations at higher Reynolds numbers were very expensive, with convergence requiring anywhere between 8 - 12 hours on a SPARC Ultra workstation. The nature of the second flow transition reported for Newtonian flows through 1:2 and 1:3 channels at Rec2 is different from that of the first one in at least one aspect. Our flow calculations revealed that the branch of the solution representing the simultaneous existence of three asymmetric vortices (the streamlines for which have been shown in Figure 4.11d) could be reached by a steady state, two - dimensional computation on a symmetric grid alone, without using the perturbation - continuation approach. Such a flow transition in experiments would therefore not be dependent on the uncertainties introduced by the =38 (a) Re (b) Re = 77 = 150 (c) Re (d) Re = 250 Figure 4.11 Flow transitions of a Newtonian liquid in a 1:2 expansion. 180 geometrical configuration or other aspects of the experimental procedure. The streamlines showing the efl‘ect of increasing Reynold numbers on the flow patterns in a more severe expansion of 1:16 are shown in Figure 4.12a through 4.12d. The more severe expansion ratio results in essentially similar trends in the transition. The corner vortices, however, fill up most of the transverse length of the downstream channel close to the expansion plane, resulting in a thinner core between the recirculation zones. In the 1:16 channel, the second flow transition resulting in three vortices was detected at around Re = 13. Reynolds numbers above 26, revealed the formation of more than three vortices in the 1:16 channel. No experimental evidence of such flow patterns has been reported. 5.2.2 Shear thinning liquid Figure 4.13a through d depict the flow patterns in a shear thinning solution (P1) through the 1:16 channel. At Re“ = 18, the two comer vortices are of equal lengths. Figure 4.13b shows that at Re” = 20, the reattachment lengths are unequal and the difference in the reattachment lengths increases at higher Reynolds numbers (seen in Figure 4.13c). At high Reynolds numbers, a thin jet of liquid in the core is seen to move toward one wall and then toward the other. At around Re“ = 44, the second flow transition was detected, wherein three vortices coexist in the channel. Our flow visualization and laser Doppler velocimetry experiments were not able to pick up the first flow transition. Instead the shear thinning liquid P1 went from a state of two symmetric vortices to a state of three asymmetric vortices directly. Computations, however, show the flow transitions in the shear thinning liquid to be similar to that demonstrated by the Newtonian liquid. 181 (a) Re=6 (d) Re = 24 Figure 4.12 Flow transitions of the Newtonian liquid in a 1:16 expansion. 182 (a) Re“ = 18 (b) Re* = 20 (d) Re" = 44. Figure 4.13 Flow transitions of the shear thinning liquid P1 in a 1:16 channel. 1 83 5.3 Velocity profiles in planar expansions 5.3.1 Velocity profiles in the Newtonian liquid before and after the onset of asymmetry Figures 4.14 shows the velocity profiles at various axial locations in a 1:3 planar expansion before the onset of asymmetry. At Re = 26 (critical Reynolds number for this case is 27), the profiles at X = l, 5.2 and 9.3 are all observed to be symmetric about the center line Y = 0. Closest to the expansion plane, negative velocities clearly indicating the presence of the recirculation regions are seen between Y = :L- 0.6 to :t 1. At X = 5.2, the smaller vortex is no longer present and negative velocities corresponding to the larger vortex only are observed. At X = 9.3, flow has approached the fiilly developed profile (U = 0.33) expected far downstream of the expansion plane. The velocity profiles at Re = 34 (higher than the critical Re“) are shown in Figure 4.15. The asymmetry in the flow is obvious at X = 1 and X = 5.2. At the former location, the velocity peaks slightly ofl‘ the Y = 0 axis and shifts toward the wall with the smaller vortex. At X = 5.2, the shift toward Y = 1 is stronger. The flow is still not fully developed at X = 9.3, indicating that higher Reynolds numbers result in a longer flow length over which asymmetry persists. However, the profile has acquired considerable symmetry by then. Flow profiles in channels with expansion ratios of 2 and 16 were qualitatively similar. Figure 4.16 demonstrates the computed velocity profile after the onset of asymmetry for a Newtonian liquid in a 1:16 expansion at Re = 8. The corresponding streamlines are shown in Figure 4.12b. At X = 5, asymmetry in terms of off-center peaking and difference in the sizes of the recirculation zones are seen. By X = 20, the smaller vortex ceases to exist and the velocity profile is markedly asymmetric. Fully developed flow is observed at X = 75. The velocity profiles Axial velocity, U 184 1.0 Figure 4.14 Velocity profiles prior to the onset of asymmetry. B=3,Re=26. 1.0 Axial velocity 185 1.0 I w u u u p — x = l 1 0.8 - - X = 5 - °°°° X = 20 . 0.6 ' . 0.4 " 0.2 - . 0.0 '0.2-1.5 -1.0 -0.5 0.0 0.5 1.0 Y Figure 4.15 Velocity profiles after the onset of asymmetry. B=3,Re=34. 1.5 Axial velocity 186 0.5 1 I ' I V I r I ' DX=5 OX=fll D AX=75 a D D 05 - g a . II D D D D a 00000 O 0.1 - ° ° ° - a...“ "I ”use... a 'o'l-m -0.6 .02 02 0.6 1.0 Figure 4.16 Computed velocity profiles with Newtonian liquid at Re = 8. Axial velocity 187 0.7 ' I ' I V I v I v UX=5 & ox=3o ° 0'5 ' AX=60 1:1 ‘ D '0'311.o A -0.6 A -o.2 0.2 ‘ 0.6 I 1.0 Figure 4.17 Computed velocity profiles with Newtonian liquid at Re = 25.3. 188 corresponding to the streamlines shown in Figure 4.12d are shown in Figure 4.17. At X = 5, two recirculations regions corresponding to the two comer vortices are seen. At X = 30, only the larger vortex exists along one wall and at X = 60 the vortex on the other wall is detected. 5.3.2 Velocity profiles in shear thinning liquid P1 through a 1:16 planar expansion Figure 4.18 shows the velocity profiles at Re“ = 20. The corresponding streamlines are shown in Figure 4.13b. At X = 5, both the comer vortices are obvious. The velocity peaks at around Y = 0.05. Further downstream at X = 15 and 20, the velocity peaks closer to the wall with the shorter vortex. The smaller vortex has disappeared at these locations. Figure 4.19 illustrates the velocity profiles corresponding to the streamlines shown in Figure 4.13c. The trends followed are very similar to that described above for the Newtonian flow at Re = 25.3. In Chapter 2, the effect of expansion ratio and inertia on the reattachment lengths has been carefirlly laid out. Expressions have been proposed to relate the three in the low and high inertia regime for Newtonian flow. These will not be discussed here. 5.4 Effect of expansion ratio and rheology on the excess pressure difference during flow through expansions To determine the effects of vortex enhancement, expansion ratio and inertia, the excess pressure difference was calculated for the entire flow channel. This is defined in equation (4.9). Axial velocity 189 0.5 ' I ' I r U ' I _ D uX—S r: a » ox=15 a n r AX=20 a D 05 - a a ‘ D 0.1 - '0'1-1.o Figure 4.18 Computed velocity profiles of the shear thinning liquid P1 at Re“ = 20. Axial velocity 189 0.5 ‘ I ‘ s r I v 3 v _ D aX—S u a > OX=15 a u ‘ AX=20 g D 0.3 - u a ' D 0.1 ' .0'1-1.0 Figure 4.18 Computed velocity profiles of the shear thinning liquid P1 at Re“ = 20. Axial velocity 190 1.0 0.8 . . . . . DX=5 0.6 - ox=3o . AX=45 ° U 0.4 - - as a 0.2 - '3 °°°°° - .5 f AAA D A 0'0 manual: 3333:“ 00000 ”24.0 41.6 ‘ 4; 2 0:2 0:6 Figure 4.19 Computed velocity profiles of the shear thinning liquid P1 at Re" = 44.3. 191 Ape = (“Amnesia ' (’AP)fd,u ‘ (-AP)fd,d (4-9) GAP)“ = Pi - Po, Pi is the computed wall pressure at the inlet of the upstream channel and P, is the computed wall pressure at the outlet of the downstream channel, (~AP),¢, is the pressure drop in the upstream channel assuming fully developed flow conditions and (- AP)“ is the corresponding firlly developed pressure drop in the downstream channel. As per our definition of the pressure difl‘erences, all of the three terms in round braces on the right hand side of equation (4.9) are positive. For firlly developed flow through a channel with B = 1 (plane Poiseuille flow), the excess pressure difl‘erence should theoretically be zero. For expansion ratios greater than one, the behavior of (AP), is shown for Newtonian liquids in Figure 4.20. Here the viscous scaling has been used for the pressure using Um and the step height as the characteristic velocity and length respectively. With an increase in the Reynolds number, the excess pressure difl‘erence decreases. As the expansion ratio is raised fiom 2 to 16, the excess pressure difference also rises. For B = 16, a distinct flattening is observed above the critical Reynolds number. A similar leveling ofi‘ at higher Reynolds numbers is expected for the channels with lower expansion ratios. To understand the effect of B and inertia on the development of the shown pressure difl‘erence, a careful breakdown of the components of (AP), reveals that the excess pressure difference consists of two parts - the first is the pressure difi‘erence downstream of the expansion plane between x = 0 to x = 1,, where l, is the portion of the larger channel that experiences non-fully developed flow due to the presence of the vortices. This part is positive at low Reynolds numbers but becomes negative at high Re. The second part 192 10 ' I ' I v y w ' 1 D :2 0 B " éA AB=3 8 P a“ 16 ‘ O = § .10 - 0AA 5 . é a b ’ ”MA 2 u A :r -20 - . i: » . 8 .30 - , S Er.) U 4 ‘40 ’ 4 “a: n '500 20 4o 60 so 100 Reynoldsnumber Figure 4.20 Effect of expansion on excess pressure difference in Newtonian flow. 193 which is always negative is the fully developed pressure difi‘erence corresponding to length 1,. The magnitude of this part is proportional to 1,. It has been shown earlier in Chapter 2 that the vortex length is proportional to the Reynolds number. Therefore, it may be assumed that 1, follows a similar trend. For any fixed expansion ratio, low Reynolds numbers result in a small 1, which in turn translates into a small negative term. As inertia increases, 1, increases and the magnitude of the second part increases. Simultaneously the pressure rise across the expansion falls down resulting in reducing the first part. The combined effect then is the reduction in (AP), with increasing Reynolds numbers. At the same Reynolds number, an increase in the expansion ratio increases (AP), consistently. Since it has been already demonstrated that the reattachment length scales with the step height and the step height is the same in all our computations, it follows that the magnitude of the second part of the excess pressure difl‘erence decreases with increasing expansion ratio. Based on a macroscopic momentum balance across an expansion (Bird et al., 1984), the magnitude of the pressure rise component also reduces with increasing expansion ratio. Since this component is also negative at high Reynolds numbers, the effect of increasing the expansion ratio is to raise the excess pressure difference. To determine the effect of shear thinning on the excess pressure difference a suitable parameter was used to normalize AP, This shown in equation (4.10). This positive normalization quantity represents the fully developed pressure drop between parallel plates. 194 _ = _2_k{ 2(1+2n) ~ ( AP)...” H [ "H, 0...,1 (4.10) U" is the average velocity of the fluid in the downstream channel and H and l are the height and length of the downstream channel. k and n are the rheological parameters of the fluid and have been defined earlier. The excess pressure difi‘erence divided by (AP)mull will be called the normalized excess pressure difi‘erence and will be represented by (AP),,. Figure 4.21 shows the effect of varying expansion ratio on the normalized pressure difference for a Newtonian liquid. The crossing over of the curves is due to the reduction in the normalization parameter with increasing expansion ratios. The efi‘ect of varying shear thinning on the excess pressure difi‘erence is shown in Figure 4.22, for a 1:16 channel. It was observed that the reattachment length in the shear thinning liquid changed very slowly at low Reynolds numbers. This shows up as a plateau in Figure 4.22 at low Re. At high Reynolds numbers the normalized excess pressure difference reduces with decreasing pseudoplasticity. In this sense, increasing the shear thinning is similar to reducing the expansion ratio. The rate of fall of (AP),u is much higher for a less shear thinning liquid. Figure 4.23 compares the normalized excess pressure difference for all the three expansion ratios for n = 0.7. Data for expansion ratios of 2 and 3 are limited to small Reynolds numbers before the onset of flow bifirrcation. Trends observed are similar to those seen in the Newtonian liquid. The magnitudes of the pressure differences are considerably lower than those observed for Newtonian flow. Normalized Excess Pressure Difference 195 2.5 ‘ I ' I f T ' I P D B = 2 1.5 .9 a A B = 3 .0 o p = 16 o 0.5 - s o o . A" .. -0.5 a A AI: 0 a o “A n d 6 a -1.5 - 0 . 0 Ch; 0 u u . '2'5 o 20 4o 60 80 Reynolds number Figure 4.21 Normalized excess pressure difference in Newtonian flow. Normalized Excess Pressure Difference 196 2.5 w s . s 1 . ,o on=1 15 - ° An=0.7 _ o 0.5 " “AA 0 A AA 0 W .05 - Mu \ AAAAAAAAAA o % -1.5 ' 0 o o '250 10 20 30 Reynolds number Figure 4.22 Effect of pseudoplasticity on excess pressure difference, B = 16. Normalized Excess Pressure Difference un L0 . . u . u - 03:2 0.6 ° ‘5 = 3 O B = 16 c2- ». o, 02 a - . A 0000 g o 0000 fifi’ 0000 O O O O o .1.0 o 10 20 30 Reynolds number Figure 4.23 Excess pressure difference in shear thinning liquid, 11 = 0.7. 198 5.5 Effect of expansion ratio and rheology on the flow resistance To evaluate the flow resistance in a planar abrupt expansion, a parameter called fr was defined. This non-dimensional parameter utilizes the pressure drop downstream and upstream of the expansion plane and it may be used as a modified overall pressure drop in the channel. (—’;—(-AP)). +( ’; (-AP». _ 2R8 Uavg avg (411) f' - [ ] p 11 + 12 The subscript d and u refer to the channels downstream and upstream of the plane of expansion respectively, h refers to the channel height, U", is the average velocity in and - AP is the pressure drop. For plane Poiseuille flow, fr would be 12. The Newtonian flow resistance for B = 3 and 16 are shown in Figures 4.24 and 4.25 respectively. Increasing inertia reduces the flow resistance. Interestingly, both the curves show a discontinuity at Re close to the critical Reynolds number. Just above the bifiircation point, there is a sudden increase in the flow resistance. At higher Reynolds numbers, fr reduces again. Figure 4.26 compares the Newtonian flow resistances for the three difi‘erent expansion ratios. As expected, the flow resistance increases as the expansion ratio is decreased. At very low Reynolds numbers, the flow resistance approaches the plane Poiseuille flow resistance. In diverging channels, the expansion effect results in a negative pressure drop for part of the channel and a positive drop in the firlly developed region. This results in a net pressure drop which is lower than that in plane Poiseuille flow, thereby yielding a lower flow resistance. Increasing inertia results in a longer separation length and consequently even more lowering of the net pressure drop. Flow resistance 12 199 D O O O O ' o O .. O O 00 o O 0 10 20 30 Reynolds number Figure 4.24 Increase in flow resistance at critical Re. B = 3, n = 1. Flow resistance 12 o o O O O I- o d O 0 00000 °o O O O 0 3 6 9 12 Reynolds number Figure 4.25 Increase in flow resistance at critical Re. B = 16, n = 1. 15 Flow resistance 201 1 ....... B = 2 --_- 5:3 + —— B= 16 . 0 - . -4 l' cl .3 1' . '12 o 20 4o 60 so 100 Reynolds number Figure 4.26 Drop in flow resistance due to expansion; Newtonian flow. 202 Figure 4.27 shows the flow resistance in a 1:16 channel for the two Newtonian and the shear thinning liquid. fr for firlly developed flow with a power-law viscosity is given by Ur)” = 40 +2") (4.12) For n = 0.7 (fi'),, is about 13.7, which is higher than that for n = 1. At low Reynolds numbers, flow resistance approaches the value corresponding to fully developed flow, thus indicating negligible expansion effect. The flow resistance increases with the lowering of the shear thinning index. The discontinuity observed close to the bifirrcation point in the Newtonian liquids is also seen in the pseudoplastic liquid. Figures 4.28 and 4.29 compare the flow resistances in a l :2 and 1 :3 planar expansion respectively. Similar trends as in the 1:16 channel are observed even for the lower expansion ratio channels. 6. Conclusions A perturbation - continuation approach was developed and used to compute the bifurcation curves for Newtonian and non - Newtonian liquids flowing through abrupt planar expansions. Detailed flow patterns depicting the various flow transitions and velocity profiles prior to and after the onset of flow asymmetry were presented for the Newtonian and non - Newtonian liquids. With Newtonian fluids, the onset of asymmetry occurred at a critical Reynolds number of 72, 27 and 6 for a 1:2, 1:3 and 1:16 planar expansion respectively. Calculations for the lower expansion ratios showed an excellent agreement with the available results in the literature. Excess pressure drop was calculated for all three expansion ratios. For any particular channel, increasing inertia reduced the 203 15 7 ' I ' I ' I ' LAAAA on= 1 A An=OJ A 0000 m 10 ' o A g o AAAAAAA AA .9 0 AAA A f ' 0 i a». E % 5 ’ o O ' o 0 0 10 20 30 Reynolds number Figure 4.27 Effect of pseudoplasticity on flow resistance. B = 16. Flow resistance 15 ' I V I I I A 00 A On=l 10- O ‘ An=0fl O 5- ° . O 0' a O .5 - d % o O 40' ‘ '15 o 20 40 so so 100 Rumdflnmmhn Figure 4.28 Effect of pseudoplasticity on flow resistance in a 1:2 channel. Flow resistance 205 ’ A D An=0J o o A O 10 - o O A i O O 5 r- 000 o O 0 0 10 20 30 Reynolds number Figure 4.29 Flow resistance in a 1:3 channel. 206 excess pressure drop. At a fixed Reynolds number, the excess pressure drop increased with increasing expansion ratio. Flow resistance in a channel was defined. Higher expansion ratios resulted in lowering the flow resistance. At the bifirrcation point, the flow resistance shot up and then gradually reduced at higher Reynolds numbers. This discontinuity was observed for all the expansion ratios investigated. A power - law model was used to describe the shear thinning behavior of a fluid flowing through a 1:16 planar expansion. Two shear thinning indices - 0.7 and 0.5 - were studied. Bifirrcation curves showed the onset of asymmetry at Re“ of 18.5 and 27.5 respectively. Shear thinning, therefore, delays the onset of asymmetry in flow through planar abnrpt expansions. Pseudoplasticity resulted in a higher normalized excess pressure difference at high Reynolds numbers, for all three expansion ratios. Flow resistance curves for non - Newtonian liquids also showed discontinuities at the critical Reynolds number. Increased pseudoplasticity led to a higher resistance in flow. Chapter 5 CONCLUSIONS AND RECOMMENDATIONS FOR FUTURE STUDY 1.1 Conclusions Symmetry breaking flow transitions were investigated in Newtonian and non - Newtonian liquids flowing through abrupt planar expansions. The efl‘ects of fluid rheology, expansion ratio and inertia on the flow transitions in planar expansions was studied in detail. A model configuration with an aspect ratio of 10 in the downstream channel and an area expansion ratio of 16 was designed. Newtonian model fluids and inelastic shear thinning model fluids were prepared. The present study was divided in three parts. In the first part streak photography was used to visualize the flow patterns at Reynolds numbers spanning 0.001 to 4, 0.1 to 3.5 and 0.1 to 1.6 for the model fluids with power - law shear thinning indices of 1, 0.7 and 0.5 respectively. Appropriate Reynolds numbers (Re‘) were defined for the non - Newtonian liquids to incorporate the shear rate dependent viscosity. Bifurcation curves using the differences in reattachment lengths on the two walls as an index of the degree of asymmetry were presented. The second part employed laser Doppler velocimetry to measure the axial velocities of all the model fluids at various locations in the downstream channel. The center - line shear rate was used as a measure of the degree of asymmetry and the flow bifurcation in these liquids above the critical 207 208 Reynolds numberwas illustrated. The rate of decay of asymmetry with increasing axial positions was evaluated. In the third part of the study, an innovative protocol involving grid perturbation and continuation was devised to compute the flow bifirrcation curves for Newtonian and non - Newtonian liquids through channels with expansions ratios 2, 3 and 16. Velocity profiles, flow patterns, critical Reynolds numbers for the onset of flow transitions, excess pressure difi‘erences and flow resistances were evaluated and the efl'ects of fluid rheology and expansion ratio on these were determined. Relations between the Newtonian reattachment length, expansion ratio and Reynolds number were proposed. Flow transition in the Newtonian liquid (liquid N) occurred at a critical Reynolds number (Refi) of 0.8, which is significantly lower than the critical Reynolds numbers reported previously for 1:2 and 1:3 planar channels. This extends the findings of Cherdron et al. (1978) who reported that increasing expansion ratios fi'om 2 to 3 resulted in the lowering of the critical Reynolds number at which flow transitions were witnessed. With the shear thinning liquid Pl (n = 0.7), flow transition was observed between 1.25 - 1.9. Shear thinning, therefore, delayed the onset of asymmetry. No flow transition was observed with the more shear thinning liquid P2 (n = 0.5), for the entire range of Reynolds numbers studied. Higher shear thinning and/or higher elasticity could be responsible for the absence of the expected flow transitions in P2. With P1, the flow transition occurred fi'om a state of two symmetrical vortices to a state of three asymmetrical vortices. The intermediate step of two asymmetrical vortices was not observed. Others have reported a similar second flow transition from two asymmetrical vortices to three asymmetrical vortices with Newtonian liquids, at much higher Reynolds numbers. Therefore, it may be said that 209 pseudoplasticity hastens the second transition in a 1:16 planar expansion. For the Newtonian liquid, LDV was used to measure the axial velocities at normalized axial positions ofX = 1, 8 and 15 at Reynolds numbers (Re) of0.6, 1.5, 2.5 and 3.5. Corresponding measurements for the shear thinning liquid were made at X = 1, 8, 16 and 45 and at Re“ = 1, 2, 2.5 and 3. Detailed observations on the dynamics of vortex growth at Reynolds numbers above the onset of flow transitions were presented. At Re = 0.6, the Newtonian liquid demonstrated symmetric velocity profiles at all the axial locations. At Re 2 1.5, flow was asymmetric close to the expansion plane (X = l) and also at X = 8. All asymmetries decayed by X = 15. The second flow transition to a state of three vortices was not observed for the range of Reynolds numbers studied. At Re“ = 1, the shear thinning liquid showed symmetric velocity profiles at all the axial locations. A flow transition to the simultaneous presence of three vortices was observed at Re“ = 2 and above. The intermediate flow transition resulting in two asymmetrical corner vortices was not seen in the experiments with the pseudoplastic liquid. Shear thinning, therefore, seems to hasten the onset of the second flow transition experienced by the Newtonian liquids at very high Reynolds numbers. The shear thinning liquid with a power - law index of 0.5 (liquid P2) revealed symmetric profiles at the maximum achievable Reynolds number of 1.5. Fluid viscoelasticity at high Reynolds numbers and a high degree of pseudoplasticity could be responsible for the delayed flow transitions. Asymmetry in the flow in terms of the center line shear rate decreased downstream of the plane of expansion in the liquids N and P 1. However, the degree of asymmetry in the shear thinning liquid was greater than that in the Newtonian liquid and it also persisted for a longer flow length. 210 Computations performed with a grid perturbation - continuation approach for Newtonian fluids, predicted the onset of asymmetry at Re,,-, = 72, 27 and 6 for a 1:2, 1:3 and 1:16 planar expansion respectively. The calculations for the lower expansion ratios of 2 and 3, showed an excellent agreement with the available computational results in the literature. Excess pressure drop was calculated for all three expansion ratios. For any particular channel, increasing inertia reduced the excess pressure drop. At any Reynolds number, the excess pressure drop increased with increasing expansion ratio. The flow resistance for a diverging channel was defined using the friction factor for flow between parallel plates. Higher expansion ratios resulted in lowering the flow resistance. At the bifirrcation point, the flow resistance shot up and then gradually reduced at higher Reynolds numbers. This discontinuity was observed in all the expansion ratios investigated. A power - law model was used to describe the shear thinning viscosity of the pseudoplastic fluids. Two shear thinning indices - 0.7 and 0.5 - were considered. The perturbation - continuation approach was then used to compute the flow bifirrcation of the shear thinning liquids. The onset of asymmetry was identified at Re" = 18.5 and 27.5 for shear thinning indices of 0.7 and 0.5 respectively. This was consistent with the experimental observation that shear thinning delayed the onset of asymmetry in flow through a 1:16 abrupt planar expansion. Pseudoplasticity resulted in a higher normalized excess pressure difference at high Reynolds numbers, for all three expansion ratios. Flow resistance curves for non - Newtonian liquids also showed discontinuities at the critical Reynolds number. Increased pseudoplasticity led to a higher resistance in flow. 211 The computations revealed both the flow transitions for the Newtonian and the shear thinning liquids. As already mentioned, the first flow transition fi'om a state of two symmetrical corner vortices to the state of two asymmetrical comer vortices was not observed in the experiments with the shear thinning liquids. Although the predicted bifurcation points were higher than the corresponding experimental observations, trends of increasing degree of asymmetry with increasing Reynolds numbers and of decaying asymmetry downstream of the expansion plane were confirmed by the computations. The computed Newtonian and non - Newtonian vortex reattachment length prior to the onset of flow asymmetry showed excellent agreement with the experimentally obtained data on a 1:16 channel. Using the results from computations performed on channels with expansion ratios of 2, 3 and 16, relations between the Newtonian reattachment length, Reynolds number and the expansion ratio were proposed for the entire range of Re prior to the onset of asymmetry. A Newtonian vortex length of about 0.44 step height was predicted for creeping flow, for all the three expansion ratios investigated. The creeping flow reattachment length decreased with increasing pseudoplasticity. More work needs to be done to obtain a modified relationship that successfully predicts the non-Newtonian reattachment lengths. Figure 5.1 shows a three parameter plot which summarizes the effect of fluid rheology, expansion ratio and inertia on the occurrence of flow transitions from symmetric to asymmetric flow patterns. An approximate division between the conditions resulting in flow asymmetry and those retaining symmetry is shown by a dotted line for the Newtonian liquid. For the sake of completeness, the experhental findings of others has also been Critical Reynolds number 212 75 . n l 1 fl 0 ‘ D n = 0.7 1 An=05 60 X‘ G - 0 n = l l l 45 l x I “ ASYMMETRY 30 l A G \ x \ \ x \ \ \ \ El 15 ‘ \ SYMMETRY \ \ \ \ e 1 A r . 1 l 0 10 15 Expansion Ratio, B Figure 5.1 Three parameter plot summarizing the effect of inertia, rheology and expansion ratio on the occurrence of flow transitions. Filled - Experiments, Unfilled - Computations, X - Others' work. 213 included. A combination of high enough expansion ratio, a fairly non-shear thinning viscosity and high injection rate will lead to early flow transitions in planar expansions. 1.2 Recommendations for future work (1) Experiments and/or computations to determine the bifurcation points for shear thinning liquids through channels with low expansion ratios of say 2 and 3 are needed to complete the findings reported in Figure 5.1. (2) Appropriate relations for the vortex reattachment lengths, analogous to those developed in the present work for Newtonian flows, still need to be developed for shear thinning liquids. (3) Borgas and Pedley (1990) have used a boundary - layer analysis to predict flow bifurcations in geometries with very gradual expansions. Such an approach is semi - analytical and if adapted for abrupt expansions could increase our understanding of bifirrcations in diverging flows. (4) Studies on injection molding (Dee and White, 1974, Serrano et al., 1995, etc.) have shown that during the filling of cavities by polymer melts, flow transitions occur above a critical injection rate, which depends on the polymer rheology and the geometry of the cavity and gates. The present study which deals with steady flows through expansions has also revealed the occurrence of flow transitions above a critical flow rate. A possible connection between these two different types of flows needs to be explored. APPENDIX A Appendix A COMPARISON OF ABRUPT EXPANSION FLOW WITH JEFFERY - HAMEL FLOW Sobey (1985) and Sobey and Drazin (1986) have shown the bifirrcation in Jefl‘ery - Hamel (II-I) flow to be subcritical and that in the planar expansion flow to be supercritical. They, therefore, conclude that Jefi‘ery - Hamel flow may not be used to explain the bifirrcation in abrupt expansion flows. Very recently Allebom et a1. (1997) have performed a linear stability analysis on abruptly diverging flows and have compared the flow in an infinitely diverging channel with JH flow. In this section, the comparison of JH flow with the flow in a 1:16 abrupt planar channel has been presented. The objective is to explore any similarity in the two flows at low Reynolds numbers prior to the onset of flow transitions in abrupt channels. JH flow may be described as the radial flow between two plates, with an angle of 2a in between them. Using cylindrical coordinates with the origin being at the intersection of the plates, the flow may be described as - .U = (U,, 0. 0); X = (7.3.2) 214 215 The equations of continuity and motion yield a fourth order ordinary difi‘erential equation shown in equation (A. 1). f’”’ + 4f” + 6Refff” = 0 (Al) Here the non - dimensionalization parameters used to normalize the locations and velocities are the same as in Chapter 4. f is the stream firnction and is related to the velocity by equation (A 2). U, = L33)- (A2) The boundary conditions are: l feta) = 4:3; f’(=*=a) = 0 (A3) a = ‘lt/Z represents the case of abrupt expansion. The boundary conditions on f imply that the normalized net volume flux is equal to 2/3. The ode system (equation A] and A3) was solved by using an IMSL routine BVPFD, where the basic discretization is the trapezoidal rule and the resulting nonlinear algebraic system is. solved by Newton’s method. A tolerance (the ratio of the error to the maximum f) of 10“ was used. The corresponding velocities were translated to planar coordinates using the following relations: (1,412» = mow—jigs); Y =Xtan<6> (A.4) 216 In Figure A.1, the velocities in the 1:16 expansion are compared with the JH flow at X = 1 at Re = 1. At locations close to the expansion plane, r approaches very small values and blows up the velocity. Since the upstream channel is of a finite height, the 1H flow closer to the expansion plane behaves as if expanding into a channel with expansion ratio less than 16. This results in higher velocities than in the abrupt expansion. As X is increased (Figure A.2), the two profiles show more agreement (X = 10) and finally the 1H flow resembles flow in a channel with a higher expansion ratio and consequently under - predicts the velocity (X = 15). Further downstream, the flow in the channel will not change much because fully developed profile will be achieved. However, the JH flow will continue to approach lower magnitudes with increasing X and therefore the agreement with the channel velocity will go on deteriorating. The disparity close to the expansion plane will be reduced if a much higher expansion ratio is used to build the abrupt channel. Higher Reynolds numbers, result in a higher maximum velocity in the JH flow (similar to that in the channel). This is evident from Figures A.3 and A.4, where the velocities are plotted at Re = 2. A better agreement is observed at X = 5 and 10 at Re = 2 than at Re = 1. As mentioned above, Sobey and Drazin (1986) have already shown conclusively that the bifurcation structure of JH flow is difi‘erent fi'om that in abrupt planar flow. For a above 73°, they have shown that JH flow is unstable. For an abrupt expansion (for which a = 90°), therefore, the critical Reynolds number of 0 is predicted for JH flow. As the expansion ratio of an abruptly expanding channel increases, the critical Reynolds number for the onset of bifirrcation goes down. It may be hypothesized that at infinite ratios, Re, approaches zero and flow will approximate IH flow. Urn 217 0.6 fi 1 . i . v — J H flow - - - Channel flow 0'0-10 A .5 o 5 ' 10 Figure A.1 Comparison of velocity profile with J H flow. X = 1, Re = 1. U111 218 ' V ' V ' 1 —JH,X=5 AChanneLX=5 ’ "-‘JH,X=10 OChannel,X=10 ----- in,x=ls xChanne1,X=15 Figure A.2 Comparison of channel velocity with JH flow, Re = 1. Urn 219 0e6 ' I V A v I > — JH flow - - ' Channel fiow 0.4 ' ‘ 0.2 " . 0'0-10 .5 o 5 10 Y Figure A.3 Comparison of velocity profiles at X = 1, Re = 2. 220 ' r I ' I —JH,X=5 AChannel,X=5 . "’JH’X=10 ' 0Channel,X=10 °°°° JH,X=15 , . XChannel,X=lS Figure A.4 Comparison of channel velocity with JH fiow, Re = 2. LIST OF REFERENCES LIST OF REFERENCES Abdul-Karem T., Binding D.M. and Sindelar M., "Contraction and expansion flows of non-Newtonian fluids”, Comp. Manufacturing, 4(2), 1993, 109-116. Acrivos A. and Schrader M. L., “Steady flow in a sudden expansion at high Reynolds numbers”, Phys. Fluids, 25(6), 1982, 823 - 930. Allebom N., Nandakumar K., Raszillier H. and Durst F., “Further contributions on the two-dimensional flow in a sudden expansion”, J. Fluid Mech., 330, 1997, 169-188. Baird D. G. And Collias D. I., “Polymer Processing - Principles and Design”, Butterworth - Heinemann, 1995, 179-188. Baloch A., Townsend P. And Webster M. E, “On two- and three-dimensional expansion flows”, Computers & Fluids, 24(8), 1995, 863 - 882. Baloch A., Townsend P. And Webster M. E, “On vortex development in viscoelastic expansion and contraction flows”, J. Non-Newtonian Fluid Mech., 65, 1996, 133 - 149. Bird R. B., Stewart W. E. and Lightfoot E. N., “Transport Phenomena”, Wiley, New York, 1984. Boger D.V., "Viscoelastic flows through contractions", Ann. Rev. Fluid Mech., 19, 1987, 157-182. . Boger D.V. and Binnington R.J., ”Experimental removal of the re-entrant corner singularity in tubular entry flows", J. Rheol., 38, 1994, 333-349. Boger D.V., Hur D.U. and Binnington R.J., "Further observations of elastic efl‘ects in tubular entry flows”, J. Non-Newtonian Fluid Mech., 20, 1986, 31-49. Borgas M. S. and Pedley T. J ., “Non - uniqueness and bifirrcation in annular and planar channel flows”, J. Fluid Mech., 214, 1990, 229 - 250. Bowen P.J., Davies AR. and Walters K., ”On viscoelastic efl‘ects in swirling flows", J. 221 222 Non-Newtonian Fluid Mech., 38, 1991, 113-126. Cable R]. and Boger D.V., "A comprehensive experimental investigation of tubular entry flow of viscoelastic fluids: Part I. Vortex characteristics in stable flow", AIChE J ., 24(5), 1978, 869 -879. Cable P.J. and Boger D.V., "A comprehensive experimental investigation of tubular entry flow of viscoelastic fluids: Part II. The velocity field in stable flow”, AIChE 1, 24(6), 1978, 992-999. Cable R]. and Boger D.V., ”A comprehensive experimental investigation of tubular entry flow of viscoelastic fluids: Part III. Unstable flow", AIChE J ., 25(1), 1979, 152-159. Chakraborty AK. and Metzner AB., ”Sink flows of viscoelastic fluids”, J. Rheol., 30, 1986, 29-41. Chang M. C. 0., “On the study of surface defects in the injection molding of rubber- modified thennoplastics”, ANTEC Proc., 1994, 360 - 363. Cherdron W., Durst F. and Whitelaw J .H., "Asymmetric flows and instabilities in symmetric ducts with sudden expansions", J. Fluid Mech., 84, 1978, 13—31. Chiba K., Ishida R. and Nakamura K., ”Mechanism for entry flow instability through a forward-facing step channel", J. Non-Newtonian Fluid Mech., 57, 1995, 271-282. Chiba K., Tanaka S. and Nakamura K., "The structure of anomalous entry flow patterns through a planar contraction", J. Non-Newtonian Fluid Mech., 42, 1992, 315-322. Christiansen E.A., Kelsey SJ. and Carter T.R., "Laminar tube flow through an abrupt contraction", AIChE J., 18, 1972, 372-380. Drain L. E., “The Laser Doppler Technique”, Wiley, New York, NY, 1980. Drikakis D., “Bifurcation phenomena in incompresible sudden expansion flows”, Phys. Fluids, 9(1), 1997, 76-87. Durst F., Melling A. and Whitelaw J.H., "Low Reynolds number flow over a plane symmetric sudden expansion", J. Fluid Mech., 64, 1974, 111-128. Durst F ., Melling A. And Whitelaw J. H., “Principles and Practice of Laser Doppler Anemometry”, Academic Press, 1976. Durst F., Pereira J CF and Tropea C., "The plane symmetric sudden-expansion flow at low Reynolds numbers", J. Fluid Mech., 248, 1993, 567-581. 223 Evans RE. and Walters K., "Flow characteristics associated with abrupt changes in geometry in the case of highly elastic liquids", J. Non-Newtonian Fluid Mech., 20, 1986, 1 1-29. Fearn R M., Mullin T. And Clifi‘e K. A, “Nonlinear flow phenomena in a symmetric sudden expansion”, J. Fluid Mech., 211, 1990, 595 - 608. Foumeny E. A, Ingharn D. B. and Walker A J., “Bifirrcations of incompressible flow through plane symmetric channel flows”, Computers & Fluids, 25(3), 1996, 225-351. Giaquinta AR and Hung T., "Slow non-Newtonian flow in a zone of separation", J. Eng. Mech. Div. - Proc. Am. Soc. Civil Eng, 1968, 1521-1538. Halmos AL, Boger D.V. and Cabelli A, "The behavior of a power-law fluid flowing through a sudden expansion", AIChE J ., 21(3), 1975, 540-553. James D.F . and Saringer J .H., "Extensional flow of dilute polymer solutions", J. Fluid Mech., 97, 1980, 655-671. James DP. and Saringer J.H., "Planar sink flow of a dilute polymer solution", J. Rheol., 26(3), 1982, 321-325. Jordan C., Rankin G.W. and Sridhar K., "A study of submerged pseudoplastic laminar jets", J. Non-Newtonian Fluid Mech., 41, 1992, 323-337. Lawler J .V., Muller S.J., Brown R. A. and Armstrong R.C., "Laser Doppler velocimetry measurements of velocity fields and transitions in viscoelastic fluids", J. Non-Newtonian Fluid Mech., 20, 1986, 51-92. McKinley G.H., Raiford w.p., Brown RA. and Armstrong R.C., "Nonlinear dynamics of viscoelastic flow in axisymmetric abrupt contractions", J. Fluid Mech., 223, 1991, 411- 456. Moffatt H. K., “Viscous and resistive eddies near a sharp corner”, J. Fluid Mech., 18, 1964, 1-1 8. Nguyen H. and Boger D.V., "The kinematics and stability of die entry flows", J. Non- Newtonian Fluid Mech., 5, 1979, 353-368. Oda K, White J. L. And Clark E. S., “letting phenomena in injection molding”, Polym. Eng. Sci., 16(8), 1976, 585 - 592. Quinzani L.M., Armstrong RC. and Brown R.A., "Birefiingence and laser-Doppler velocimetry (LDV) studies of viscoelastic flow through a planar contraction", J. 224 Non - Newtonian Fluid Mech., 52, 1994, 1-36. Raiford W.P., Quinzani L.M., Coates P.J., Armstrong RC. and Brown R.A, "LDV measurements of viscoelasic flow transitions in abrupt axisymmetric contractions: interaction of inertia and elasticity", J. Non-Newtonian Fluid Mech., 32, 1989, 39-68. Rama Murthy AV. and Boger D.V., "Developing velocity profiles on the downstream side of a contraction for inelastic polymer solutions", Trans. Soc. Rheol., 15, 1971, 709- 730. Serrano M., Little J. and Chilcoat T., "Critical shear rate for the injection molding of polycarbonate, polystyrene and styrene acrylonitrile", SPE Tech. Papers, 41, 1995, 38-40. Shapira M., Degani D. and Weihs D., “Stability and existence of multiple solutions for viscous flow in suddenly enlarged channel”, Comput. Fluids, 18, 1990, 239 Sobey I.J., "Observation of waves during oscillatory channel flow", J. Fluid Mech., 151, 1985, 395-426. Sobey I. J. and Drazin P. G., “Bifilrcations of two dimensional channel flows”, J. Fluid Mech., 171, 1986, 263. Townsend P. and Walters K., "Expansion flows of non-Newtonian liquids", Chem. Eng. Science, 49(5), 1994, 749-763. Teschauer I., “numerische Untersuchung der symmetriebrechenden Bifirrkation bei Stromungen durch plotzliche Kanalerweiterungen”, Studienarbeit Lehrstuhl fur Stromungsmechanik Universitat Erlangen-Numberg, 1994 Vrentas J .S. and Duda J .L., "Flow of a Newtonian fluid through a sudden contraction", Appl. Sci. Res, 28, 1973, 241-260 Walters K. and Rawlinson D.M., "On some contraction flows for Boger fluids", Rheol. Acta, 21, 1982, 547-552. ' Watrasiewics B. M. And Rudd M. J ., “Laser Doppler measurements”, Butterworths & Co. (Publishers) Ltd., 1976. White J. L. And Dee H. B., “Flow visualization for injection molding of polyethylene and polystyrene melts”, Polym. Eng. Sci, 14, 1974, 212 - 224. White J. L. and Dietz W., “Some relationships between injection molding conditions and the characteristics of vitrified molded parts”, Polym. Eng. Sci., 19(15), 1979, 1081 - 1091. 225 White S.A, Gotsis AD. and Baird D.G., "Review of the entry flow problem: Experimental and Numerical", J. Non-Newtonian Fluid Mech., 24, 1987, 121-160. MICHIGRN STATE UNIV. LIBRARIES llllllll WWW” Ill H 1111 W lllllllll 31293016822466