}V1ESI.J RETURNING MATERIALS: Place in book drop to LIBRARJES remove this checkout from —;«-—. your record. FINES will be charged if book is returned after the date stamped be10w. 9‘14. ~ as".- aware; A STUDY OF THE GAMDW TELLER STRENGTH IN 40’42’44’4803 FROM THE (p.11) REACTION AT 119 Mev BY Janaki Narayanaswamy A DISSERTAIION Submitted to Michigan State University in partial fulfillment of the requirements for the degree of DOCTOR OF PHILOSOPHY Department of Physics and Astronomy 1983 ABSTRACT A STUDY OF THE GAMOW TELLER STRENGTH IN 40:42:44,48Ca FROM THE (p,n) REACTION AT 119 MeV By Janaki Narayanaswamy The (Pm) reaction at 119.3 MeV has been employed to measure the 140,142,144 and “Ca. The experiment was carried spin transfer strength in out at the Indiana University Cyclotron Facility using the neutron time of flight apparatus and time compensated scintillation detectors at a target-to-detector distance of 131.5 meters. Analyses of the data by several different methods indicate that a significant amount of 1+ strength is contained in what is conventionally taken as the background in neutron energy spectra. This finding explains at best partially the apparent quenching of the spin depdendent operator V0T when the data were analyzed ignoring such a background. An earlier observation that the 16.8 MeV state in 11830 is wider than the parent state in “8 Ca at an excitation of 2.52 Mev is confirmed by the present data. The 2.73 MeV u state in 88c is found to have an angular distribution corresponding to L=O. DEDICATED TO Seethalakshmi and Narayanaswamy (My Parents) ACKNOWLEDGMENTS It is a pleasure to thank Professor Sam M. Austin for his guid- ance. His patience and constructive criticisms have been indispensable to the completion of this work. I have also benefited greatly from the assistance provided by Professor Aaron Galonsky during data acquisition and by Dr. Olaf Scholten during the final stages of the analysis. I express my gratitude to the Department of Physics and Astronomy of Michigan State University and the National Superconducting Cyclotron Laboratory for financial support during my graduate program. The faculty, staff and fellow students at the M.S.U. Cyclotron Laboratory deserve special mention for their kindness. The hospitality extended by the Indiana University Cyclotron Facility and the assistance provided by Professor Charles D. Goodman and Dr. T.N. Taddeucci are gratefully acknowledged. Thanks to R. Geetha, Shobha Prasad and Parul Vora for making life in East Lansing more enjoyable. I am also most grateful to Barbara Uacak and Patty Pirnie for their support during the difficult time of thesis writing and to Ron Fox for helping me understand the mysteries of the program SCOPEFIT. Special thanks to Shari Conroy for the typing of this thesis. Lastly, thanks to my parents for their love and support to a daughter with unconventional ambitions, to Rukku and Raghu (my sister and brother-in-law) for the countless pep talks, to my sister Hema for her wishes and to my brother Kedarnath for repairing everything from wristwatch to car and keeping me going. iii II. III. IV. TABLE OF CONTENTS List of Tables List of Figures List of Abbreviations Introduction Experimental Techniques Data Acquisiton and Reduction Data Analysis Summary Appendix A Appendix B Appendix C Appendix D List of References iv Page vii xi 17 31 68 86 9O 92 100 110 117 1.1 3.2 3.3 3.4 3.5a 3.5b 3.6 3.7 3.8 3.9 3.10 4.1 4.2 4.3 4.4 5.1 LIST OF TABLES Relevant Operators for different probes Target Information Energy Band Centroid Shifts (in channels) Normalization of Relative to Absolute Differential Cross Sections (at 0°) Computation of R as a function of assumed threshold energy Dependence of Efficiency corrected peak areas on threshold energies 7Li(p,n)7Be (g.s., 0.429 MeV) ENeutron . 117.0 MeV Dependence of efficiency corrected peak areas on threshold energies 12C(p,n)12N (g.s.) ENeutronalloo'O MeV Angular distributions for “°Ca(p,n)“°$c Angular distributions for “2Ca(p,n)“23c Angular distributions for I”‘Ca(p,n)"“Sc Angular distributions for “BCa(p,n)“°Sc Neutron energies (in MeV) below which TAC nonlinearity is present in energy spectra Optical Model parameters I“'Ca(p,n)""$c. Contributions to 0° cross sections from 1+, 1 and 3+ states. “8Ca(p,n)“BSc. Contributions to 0° cross sections from 1+, 1' and 3+ states Comparison of 1- behavior from present data and background falloff energies (from 0f 82) Total GT strength from the present data (as percent of minimum sum rule prediction) V Page 31 35 45 47 50 51 55 55 56 S7 58 72 74 83 87 D.l D.2 D.3 D.5 LIST OF TABLES (continued) Computation of total background) for “20a Computation of total background) for l”‘Ca Computation of total background) for I”Ca Computation of total GT strength (with experimenter's GT Strength (with Experimenter's GT Strength (with Experimenter's GT Strength for “Ca (with 1+ Strengths derived from DWBA analysis of data) Computation of total GT Strength for “30a (with 1+ Strength derived from DWBA analysis of data) vi Page 112 113 114 115 116 1.1 1.2 2.1 2.2 2.3 2.4 LIST OF FIGURES Page Graphs of K, defined in Eq. 1.7 and deduced from the 11 measured 0° (p,n) cross sections vs. and 2. The top graph contains only the pure Fermi transitions while the lower graph contains the complete data set. Error bars on K reflect uncertainties in measured cross sections only. The transitions are labeled by specifying the target nucleus with the excitation energy in the final nucleus given in parentheses. The solid curves represent the fits to 2 Mg data, the dashed curves are the impulse approximation strengths, and the dot-dashed curve the one-pion-exchange-potential strength. (Figure and caption from Goodman et al., (Go 80).) The empirical quantity R(E ) for odd- and even-A 13 targets. The solid line represents the average value R(Ep)/Ep=-(S4.9:t0.9 MeV)’1 determined from the even-A target data for bombarding energies Ep_>_50 MeV. (Figure and caption from Taddeucci et a1. (Ta 81).) Floor plan of experimental areas showing locations of the 19 new pion spectrograph, beam swinger magnet and neutron time-of-flight area. (Figure and caption from IUCF Annual Report 1977-78.) Magnet layout for beam swinger 21 (Figure from Goodman et al., (Go 79.) This figure shows the geometrical parameters of time 23 compensation. B is the ratio of neutron velocity to the velocity of light. n is the index of refraction of the scintillator. tn is the transit time of the neutron and tp is the transit time of the light (photon). L is the length of the scintillator. (Figure and caption from Goodman et al., (Go78b).) (a) The curves show the fraction of forward emitted light 25 that has reached the phototube by time t, measured from when the neutron crosses the plane through the front face of the scintillator. The parameters used are: length of scintillator=1 m, index of refraction= 1.6, phosphor decay constant - 2.4 ns, neutron energy = 100 MeV. The vii 2.4 2.5 2.6 2.7 3.1 3.2 3.3 3.4 3.5 3.6 3.7 3.8 (a continued) three curves are for scintillations at the front, middle and back of the scintillator. (b) This shows how time compensation is achieved by tilting the scintillator. The calculation is the same as for Fig. (a) except for the tilt. (Figure and caption from Goodman et al., (Go 79).) This shows the required tilt angle o, as a function of neutron energy to achieve exact time compensation for the axial light rays. (Figure and caption from Goodman et al., (Go 78b).) Block diagram of phase drift compensator. (Figure and caption from Goodman et al., (Go 79).) Block diagram of electronics as used for data taking in the (p,n) experiment. (Figure and caption from Goodman et al., (Go 78a).) Arrangement of detectors in the 0° hut. Time flight spectra for “0’“2’““ 0°. and “BCa (p,n) at (top) Cosmic ray spectrum (data) (bottom) Cosmic ray spectrum (average) Time of flight spectrum for HCa(p,n)“Sc at 0°, with cosmic ray contribution subtracted. Solid line indicates foldover neutron background. (a) Time of flight spectrum for 7Li(p,n)7Be. (b) Time of flight spectrum for 12C(p,n)12N. (a) Plots of log Y and log e vs. R(Th) in units of Compton Edge. Note that these threshold values are only nominal. (b) Plot of R(Th) vs. E(Th) (in units of Compton Edge). Solid line is the weighted average of the four values and agrees with experimentally determined absolute cross section ratios for (p,n) reaction on 7L1 and 12C for states shown in Figure 3.6(a) and 3.6(b), to experimental uncertainties. The threshold values shown are only nominal. Energy spectra for “0’"2’““ and “8Ca(p,n)“°’“2’““ and “BBC. Experimenter's backgrounds defined to fit peaks are indicated by solid lines. viii Page 25 25 27 27 30 32 37 39 39 41 43 44 48 49 53 3.9 3.11 3.12 4.1 4.2 4.3 4.4 4.5 4.6 4.6 4.7 Angular distribution of 1+ state in “03c (dotted line). Solid line shows an average of the 1+ angular distributions derived from “2’““ and “88c. (a) Angular distributions of observed states in l‘ZSc. (b) Same as Figure 3.10(a). “MS (a) Angular distributions of observed states in c. (b) Same as Figure 3.1l(a). (a) Angular distributions of observed states in “88c. (b) Same as Figure 3.12(a). Schematic representation of the microscopic model used for the background calculations in the figure 8F denotes the Fenmi energy, E the nucleon separation energy, and Ep the S incident projectile energy. For the effective projectile target nucleon interaction Veff the GBY interaction of Love and Franey (Ref. 8) is used. (Figure and caption from Osterfeld's work (0f 82).) Zero degree spectra for the reactions “8Ca(p,n) (a) and “°Ca(p,n) (b). The data (thick full line) are taken from Refs. 13 and 14 (see text). The discrete lines are calculated cross sections due to bound and quasibound states. The arrow labeled with AL=-1 indicates the loca- tion where the AL==1 resonance (0',l-,2-) would occur if nuclear collectivity were included for these states. The theoretical cross sections due to the GTR and IAS are not plotted. The Optical parameters for the cross section calculations have been taken from Ref. 20. (Figure and caption from Osterfeld's work (0f 82).) Comparison of measured and DWBA 79 predicted differential cross sections for 1+ states in “2Ca(p,n)“28c and “8Ca(p,n)“°Sc. Plot of 1+, 1- and 3+ strengths vs. excitation energy in HCa(p,n)“Sc at 0°. Plot of 1+, 1- and 3+ strengths vs. excitation energy in “8Ca(p,n)“BSc at 0°. Application of Goodman's method in an idealized case. continued L#0 spectra at Glab=0.0 , for “2’““’“90a(p,n). ix Page 59 60 61 62 63 64 65 69 70 73 77 78 79 80 82 Page 5.1 Energy spectra for Blab=-0.0°. Present study. 88 5.2 High-resolution inelastic electron scattering spectra of 88 no “2 H ”Ca all measured at 8 -165° and E0 =39 MeV. Magnetic dipole transitions are denoted by an arrow. (Figure and caption from Steffen et al., (St 80).) Appendix B Spectra (Efficiency Corrected and Energy Calibrated) 92-99 Appendix C.1 Relative detector efficiency versus neutron energy. 109 Threshold energies shown are electron energies. DWBA DWIA GT IAS IUCF N x Th NTOF PWBA TAC TOP LIST OF ABBREVIATIONS Distorted Wave Born Approximation Distorted Wave Impulse Approximation Fermi Transition or Operator Gamow Teller Transition or Operator Isobaric Analog State Indiana University Cyclotron Facility N times the zsth Compton edge Neutron Time of Flight Plane Wave Born Approximation Time to amplitude converter Time of Flight I. Introduction The discovery of the neutron in 1932 was fundamental to the formulation of successful nuclear models. An underlying assumption in all such models and verified experimentally is that the two body nucleon-nucleon force possesses charge:sym- metry and charge independence i.e., it is the same for p-p, n-n, and p-n systems. In this picture, the proton and the neutron are viewed as different manifestations of the same fundamental entity, the nucleon. It is in the z axis pro- jection of the isospin (tz) in iSOSpin space that the two differ: the proton has tz==-l/2; for the neutron, tz==+l/2. Then the nucleus can be viewed as an aggregate of nucleons, whose intrinsic states are distributed among spin up or spin down, and isospin up or isospin down donfigurations. But recent experiments at intermediate energies have led to speculation that one may have,to consider additional degrees of freedom for the nucleon, for example, the A resonance (Os 79, Bo 81, Go 82, Ra 82, Ga 82). To be specific, this has been brought about by an apparent quenching of the spin dependent Operators observed in (p,p') (Ml strength) and (p,n) (GT strength) reactions. Obviously, such a coupling Of nucleon structure to nuclear structure is of fundamental :hmportance to our picture of the nucleus. The goal of this 1 2 study is to locate the spin transfer strength from 40'42'44 and 48Ca, and to study the systematics of the strength as a function of neutron excess. We employed the (p,n) reaction on the calcium isotopes at a proton energy of 119 MeV. The following considerations will explain the par- ticular usefulness of the (p,n) reaction in this context and the relevance of the chosen bombarding energy. The strength of the nucleon-nucleon interaction at short range forces one to use an effective interaction, Veff’ in calculations of nuclear structure and reactions. This interaction is assumed to be the sum of two body interactions over all possible pairs of nucleons in the system. Many body forces present in nuclei contribute less than 10% of the binding energy (Be 72). Therefore, the nuclear Hamiltonian can be written . H = Z K.-+ Z V.. l i i -+Ga , 1.4 where t - 2 B (F) : (F) f 731:: 112 Bt(GT) =2= l ll2 f ‘ ‘f—M k k k |i>, |f> are the initial and final states and ti, okt: are the spin and spin-iSOSpin operators that mediate the transi- tions. The presence of other nucleons may block some transitions because the single particle states into which they must decay may already be occupied. It is useful to define the reduced transition probabil- ities B(F) and B(GT) such that B(F) =1 and B(GT) =3 for a free neutron as is implied by Eq. 1.3. In these units, it can be shown that the difference in beta decay strengths for a nucleus with a neutron excess N-Z is given by ll U) I 0') 1| B(F) N-Z for a Fermi transition B(GT) ll 0') I (I) ll 3(N-Z) for a GT transition This model independent sum rule is derived in Appendix A. Therefore, we can write B(F) _>_N-Z and B(GT) _>_3(N-z) Thus, N-Z and 3(N-Z) are the minimum strengths one would expect to find for Fermi and GT transitions respectively. The equality holds when 88* is negligible. It had been a puzzling observation that measured beta decay rates were slow compared to simple model expectations. The discovery of the isobaric analog state (IAS) in (p,n) reactions contributed greatly to the understanding of this phenomenon. The IAS happens to be nearly the projection of the collective Fermi operator on the final nucleus and in heavy nuclei the Coulomb displacement energy puts this state out of the reach of beta decay, hence the slow rate. This discovery further prompted postulation of the existence of a giant GT resonance that would contain most of the GT strength and would be located at an excitation energy near and slightly above the IAS (Ik 63). In fact, if the nuclear Hamiltonian were Spin independent, then the IAS and the GT would be degenerate. But the spin dependent interaction shifts the GT distribution. Obviously, the existence of this giant GT resonance, out of the reach of beta decay for N2>Z nuclei, had to be tested by some probe other than beta decay. Table 1.1 lists the relevant operators for differ- ent probes Table 1.1 Relevant Operators for different probes Transition O+-+O+ L==O 0++1+ S=0 s=l + + + ++ + In XV ' . XV ° - . (p ) . TIP T] ' OTop ojrp Tj J 3 B decay Z I. (Fermi Z o.-r. (GT) j J - J J J 14* ( >7 7' f :1 -I.G‘OT.I l j'JP "‘3 3 J: * Ignoring current and small isoscalar parts of the operator. In the (p,n) reaction, the target nucleus gains one more proton and loses a neutron. In this sense, the reac- tion is similar to beta decay. Since the operators have the same form in spin-isospin space one would expect strong transitions in GT beta decay or M1 to be strong in (p,n) reactions. This similarity suggests that the (p,n) reaction can be used to mimic beta decays that are prohibited by energy considerations and to determine GT strengths. But one has to study first, nuclei with knowncxrmatrix elements so as to understand the signature in the (p,n) reaction that corresponds to beta decay strength and establish empirical quantitative relationships between the two. More important- ly, the beta decay conditions have to be simulated with the (p,n) reaction as closely as possible (near zero momentum transfer, for example) and quantitative corrections made for deviations from these conditions. Then it is possible, in principle, to extract beta decay information from the (p,n) reaction in an almost model independent way (Go 80). It was seen that the IAS, corresponding to superallowed Fermi transitions stood out in (p,n) spectra. But the GT transitions were not apparent in low energy (p,n) reactions. The first evidence for the existence of GT giant resonances came from 45 MeV (p,n) data taken at M.S.U. (Do 75). It was soon apparent from intermediate energy proton beams (up to 200 MeV) at IUCF that GT transitions dominate the 0° (p,n) spectra at energies greater than about 100 MeV (Go 78). This is a direct consequence of the relative behavior of VT and VOT as a function of proton energy (Ta 81). These inter- mediate energy (p,n) reaction studies led to the following observations (Go 80). The (p,n) reaction is mediated by isovector parts of V. i.e., V 3p or transfer) only low momentum components contribute appreciably and VT in Eq. 1.4. At 0° (small momentum to the cross section. Therefore, at 0°, the (p,n) reaction favors states with significant allowed Fermi (L =0, S =0) and GT (L==0, S:=l) matrix elements. At intermediate ener- gies, strong transitions in (p,n) are direct; central parts in Vjp dominate; for small q, noncentral parts can be neglected. Also at 120 MeV, the impulse approximation has some validity i.e., Véffw§the free nucleon-nucleon t matrix. In the distorted wave approximation the cross section for a reaction A(a,b)B is prOportional to the square of the transition matrix element and can be written (Go 80) d k 0 = ( 11 )2 f 1 35 2557 ET (2Ji+l)(2§p-+l) 2 i p] 1.5 Zlfxé-)*(£p)x(+)(gp)d3r where the x's are distorted waves generated in an appropriate Optical potential; u and k denote the reduced mass and wave number in the center of mass system respectively; JP the effective nucleon-nucleon interaction; knockout exchange is the target matrix element, and V. is J is excluded by the term l--Pjp where Pjp is the permutation operator. The inner sum is over all the nucleons in the target; the outer sum is over the initial and final spin projections of the projectile and the target. Under the conditions observed for (p,n) reactions at 120 MeV, the 0° differential corss section can be written k do ~ u f D 2 D 2 d (00) _ (‘an ) E—i {NTIJT] +NOTIJGTI I 1.6 where J,f and Jor are the magnitudes of the volume integrals of the effective spin independent (Tj-Tp) and spin dependent (Oj-Op Tj-Tp) isovector central terms in Vjp(l-Pjp), N3 and N21 are distortion factors defined to be the ratio of the DWBA and PWBA cross sections; ||2 and ||2 are the squares of the Fermi and Gamow-Teller matrix elements given by 1.4. Following Goodman et al., (Go 80) define for a pure Fermi or GT transition, k __ do(0°) u 2 f 1) Then from a plot of K vs. B(F) or B(GT) one can extract empirically the corresponding interaction strengths, Jr and JOT in Equation 1.6. Goodman et al., used the local t-matrix interaction of Love et al., (LO 78) and computed the distor- tion factor ND. They find that ND shows a smooth exponential A dependence and is only moderately sensitive to the reac- tion Q values and the model nuclear wave functions. By com- paring the 0° (p,n) cross sections of the IAS and GT states in the case of several nuclei to known F and GT beta decay matrix elements, Goodman et al., find that there is a linear correspondence between these two quantities and that interaction strengths at Ep==120 MeV are 168 MeV-fm (spin flip) and 89 MeV-fm (non spin flip). Figures 1.1a and l.lb show the data and the fits from their work. This finding demonstrates that the (p,n) reaction can serve as a precise probe to measure GT strength for light and medium weight nuclei. Taddeucci et al., (Ta 81) define another convenient empirical ratio oGT(0°)/|[2KGT(E ) .E— 1.8 2 {R(E )} = o p OF(0 )/1TZKF(EP) where OGT(O°) and OF(0°) are cross sections in the same nucleus for a 1+ state with known Bf(GT) and the IAS with B(F)==N-Z, respectively. In terms of the quantities in Equation 1.6 J ~ or D D35 1.9 _ 2 It has been found from DWIA calculations that at intermedi- ate energies the distortion factor ratio is approximately in- dependent of energy and has the value 1.2 t0.l for GT and F~ transitions not widely separated in energy. The quantity R(Ep) then represents roughly the ratio of interaction strengths JCT/JT at momentum transfer q==0 but corrected for small distortion effects. Taddeucci et al., considered the variation of R with incident proton energy for several odd and even mass nuclei and found that R<==Ep to a good 10 Figure 1.1. Graphs of K, defined in Eq. 1. 7 and2 deduced from the measured 0° (p,n) cross sections vs 2 and 2. The top graph contains only the pure Fermi transi- tions while the lower graph contains the complete data set. Error bars on K reflect uncertainties in measured cross sections only. The transitions are labeled by specifying the target nucleus with the excitation energy in the final nucleus given in parentheses. The solid curves represent the fits to stg data, the dashed curves are the impulse approximation strengths, and the dot- dashed curve the one- pion-exchange-potential strength. (Figure and caption from Goodman et al. (Go 80). ll AGE. .~>o<: «7.0. X. v. I. _ _ _ _ _ _ .15 q _ _ 3m 3. «H _ .. . x. 1. ,m 1.. r. S .1 m 3.0....433s11l/ x W . .v n . i / e .m :mwhNom ’@ M .. a 1m 4,... e \ 1 m 0 I flew. .YT S 1... A» 6 12 m 2 _ :. in. C \l . n... . . 11111 1.1 . .. .. < . , ImM 2.30sz / I .O T no Is 3362 1...; Wan/u. 1 3.323111%”). 1... 1. d ... 1.14 A.W.Ovoan / “/ mF. ..m.om.<- (1.1»; . III e bl. all .m. v0 \ Z 2 A n. I a 3.9923 x Z _ _ b _ b _ _ _ . m w. 00 m M m m 8 6 4 2 . 00 (ME)2 Figure 1.1 12 approximation above Ep==60 MeV. Figures 1.2a and 1.2b show the data that they used and the linear fit to the data. For example, at 120 MeV, R =2.l9. This linear and model inde- pendent relation can be used to compute GT strengths from (p,n) reactions at 120 MeV with an accuracy only slightly worse than that of the cross section measurement i.e., 20%. One simply compares the IAS cross section with the l+ state of interest and applies Equation 1.8. Note that such a deter- mination is independent of calibration transitions, cross section normalizations, and DWIA mass dependent extrapola- tions. Hence, this method has a particular simplicity and we use it exclusively. Some measurements have already been made of GT strength 40,42 48 from (p,n) reactions on and Ca at 160 MeV, (Ga 81,An 80) ;. but the current work is more complete and includes a 44Ca target; it will serve as a parallel to the electron scatter- ing studies of Steffen et al., (St 80). The measured B(GT) is compared to the simple sum rule prediction to determine the quenching of the spin dependent Operator or-. In recent work on heavier nuclei, roughly 0.6::0.1 of the sum rule strength was seen. This has been interpreted as evidence for the coupling of the nucleon to the A isobar (T==Tz==3/2, S =3/2) by several authors (Os 79, Go 82, Ra 82, Ga 82, Bo 82). There seems to be some evidence from pion inelastic scattering also that such a coupling exists (Mo 82). Cal- culations including this coupling to the spin-isospin degrees of freedom of the nucleon suggest that roughly 65% l3 ‘ I Even-A ,’ 3»— s4 1 ' C i r 1 b . u I- 42 4 2L ‘ Co .4 A“). d .1321 I C 1- .1 D . 11- «:1 b c1 D d 1'. ‘1 -/ cl I LL LLLLL4 1 LLI 111 A 1 1 J 4 LJL 1 I, ‘1 Odd-A , J - 7L1 2 I ‘q o 36 A 7 .. -3c: . .1 WW. 0 50 ED 50 ax: 233 5,, mm Figure 1.2. The empirical quantity R(E ) for odd- and even-A targets. The solid line represents the average value R(Ep)/Ep = (54.9 e 0.9 MeV)‘1 determined from the even-A target data for bombarding energies Ep _>_50 MeV. (Figure and caption from Taddeucci et a1. (Ta 81).) 14 of the classical strength should fall in the nuclear excita— 208Pb (Ga 80). Sagawa used the constituent tion region for quark model to calculate the isobar-hole coupling matrix element and finds that the combined effects of RPA correla- tions and particle-hole coupling decrease the transition strengths of M1 and GT states by about 35% (Sa 82). If true, all the above observations point towards a significant coupling of the nucleon structure to nuclear structure. However, the work of Bertsch and Hamamoto, including 90Zr, indicates that the strong tensor 2p-2h states for force shifts the strength to between 10 and 45 MeV excita- tion (Be 82). Yet another approach to the problem of spin- isospin excitations in terms of a unifying response function by Ericson suggests that at low momentum, in addition to creating a collective mode, the strong repulsive ph force, also produces a quenching of the GT strength due to a Lorentz-Lorentz effect similar to that of electromagnetism (Br 82). Microsc0pic background calculations for (p,n) 40 and 48Ca at 160 MeV, carried out by Osterfeld reactions on imply that a significant part of the missing l+ strength is contained in what is conventionally taken as an experimen- ter's background and this accounts at least partly for the larger values of the observed quenching of the spin depen- dent Operators earlier deduced from (p,n) reactions (Of 82). Thus the precise amount of quenching may bear importantly on the question of the number of degrees of freedom in the nuclear wave function. In the present work, an attempt has 15 been made to verify the last of the above hypotheses as will be discussed in Chapter IV. Finally, one notes that these results may have substan- tial applications. The GT strength is a measure of the degree to which nucleons are unpaired in the ground state of a nucleus. The measured strength for 40Ca should therefore be useful for an estimate of the same. The present study also verifies a recent claim that the analog of the 10.3 MeV state in48 Ca is significantly wider than the parent state (An 80). The energy systematics seen in this study seem to indicate what was already noted by Bertsch--i.e., one does not expect pion condensation in nuclei (Be 81). The width of the GT strength function is a necessary input in calcula- tions of stellar nucleosynthesis. In the gross theory of 8 decay, Takahashi et al., use the mean energy of GT strength to be degenerate with the IAS which is not quite right and use a width of 10 MeV, much larger than seen in (p,n) reac- tions (Tk 73). Redoing these calculations using the mean energy and width of the GT strength values as suggested by the current (p,n) reaction studies might improve our under- standing of the r-process nucleosynthesis. Further, GT matrix elements are of considerable importance in computing weak decay rates in supernovae (Fu 80). We hope that the current measurements will therefore, aid in calculations of reaction rates in these stages of stellar evolution and nucleosynthesis. The organization of this thesis is as follows: Chapter 16 II contains a description of IUCF and the neutron time of flight apparatus. Methods of data acquisition and reduction are described in Chapter III. An analysis using DWBA 79 and interpretation of our results are given in Chapter IV. A summary of our findings is given in the concluding Chapter V. The simple sum rule quoted earlier is derived in Appendix A. Plots of energy calibrated spectra for all the four tar- gets at the three angles measured (0°,6.3°,and ll.l°) are shown in Appendix B. Neutron detector efficiencies are listed in Appendix C. Appendix D contains Tables giving the details of the computation of the GT strength. II. Experimental Techniques The electric charge neutrality of the neutron.doesxun;permit conventhmuu.detection techniques, using magnetic spectrographs and solid state detectors. Neutrons can only be detected by the charged particle recoils, or the charged reaction products produced when they scatter ffiwxn, or react with other nuclei. Although the energy signals thus produced are not proportional to the neutron energy, the time of emission of these signals in the detector relative to a fixed time reference is proportional to the time of flight, which in turn, defines the neutron velocity, and hence, the neutron energy. Thus, precise time signals and long flight paths are required in high precision neutron spectroscopy. Quantitatively expressed, neutron energy E, neutron velocity v, time of flight t, and the path length L are related as 2 u 2.1!. 3.1. E Mnc (2 2+8 14'”) C C t = L/v (2.1) 2 A ~ 2 1 L 3 L E'Mn°( 22+ 1111) t c t c where Mnc2 is the rest mass energy of the neutron. In the nonrelativistic limit, energy resolution and time resoluticni are therefore, related as 23/2 E3/2 ; ___. ____. 2.2 A8 M1/2 L At ( ) ‘n 17 18 Note that this is a lower limit on AB. The different factors contributing to At are electronic, beam bunch width, scintillator transit time, target energy loss and straggling, beam energy spread, kinematic broadening, and intrinsic state width. One way to improve energy resolution is to increase the flight path with a consequent loss in count rate a: 13-2. Using large detectors can compensate partly for count rate loss; but then, scintillator transit time causes a major loss of time resolution unless one compensates for it by other means. At the Indiana University Cyclotron Facility (IUCF) where the experiment was carried out, typical proton pulse widths are 0.5 nsec. Using large volume scintillators and a time compensation technique described later in this chapter, Goodman et. al., have achieved subnanosecond resolution for 100 MeV neutrons (Go 79). To get an estimate of the pathlength involved, note from Equation 2.2 that for At-1 nsec, roughly a 115 meter long flight path is required for an energy resolution of 300 Kev for 115 MeV neutrons. With these limitations, the major technical problems associated with neutron spectroscopy are the need for (a) a beam swinger (b) large detectors and (c) a stable stop signal. (a) Beam Swinger: It is not very practical to move detectors around the target to measure angular distributions, when the flight path is long. This requires not only large space, but also very carefully placed shielding along the flight path to insure that the detector sees only neutrons from the target. It is easier to change the direction of the incident beam on the target. The floor plan of the experimental areas at IUCF are shown in Figure 2.1. The neutron station is located at the northern end of the laboratory. The remoteness of this location allows one to set up long flight paths with little inconvenience to and l9 731:3 buomom 32:2 .53 scum cofloeo use 3235 .mmum unmaHMIwOIOEHu :Ouummc ocm umcmmE womcazm Econ .zmmumou . . . nommm :Oam 3m: ms... «0 macawmoOH amazonm mmmum Hmucmfiflummxm no code wooden .H.N musmfim A1 - 2 o. ... o .11 3!}: i . elk. ]\ ex .. /,\ n\\\\\ -1 ’ § \\\ . .. . V.“§t§.o.\\ Y" . ”..J . . / , . . / v . . oONxoO / / — . (M11 l I _ . ... . ‘ / 9) AF . .\\ “x. III-I- hDO>229?— zochOJuro 5.595223 421.02. 20 from other sections of the laboratory. A major feature of the neutron station is a beam swinger using three fixed magnets that enables one to change the angle of incidence of the beam on the target; for a fixed flight path, this is equivalent to changing the effective reaction angle. Figure 2.2 illustrates the geometry. The first magnet bends the beam away from its original path, the second magnet bends it back towards the target. The pole faces of the second magnet are large enough to accept a range of paths that impinge on the target at a range of angles. The third magnet steers the beam into a dump. ‘With the use of the third magnet, the beam dump can remain fixed, as the angle is varied. Tins feature is particularly useful at high energies, when massive shielding is required around the beam dump to keep the neutron background low. It also makes possible Observations at 0°, where Lao spin flip processes dominate. In the NTOF system currently in use at Indiana, the angular range on target Of incident protons is 260. The scattering angle 6 is determined by the radii of curvature of the beam protons in the two magnets, 91(6) and p2(e). Thus, to set the system for a given angle, one sets the fields 82 and B1 to correspond to the magnetic rigidity of the incident particle. The angle is then measured more precisely by centering the beam on a motor driven slit that pivots around the target position. The slit is used only when the beam is being focused and the angle measured and is retracted during data runs to avoid neutron background.owxn it. Since the scattering plane is horizontal one can have multiple paths with all detectors at ground level. Currently, there are three time of flight lines covering angular ranges of 0-260, 24-500, 21 A.Amn 00V ..Hm um :mEoooo Eouw Owsmflmv .ummcw3m Emma Hem usoxma uocmmz .N.N musmwm 22 and 145-710. The detectors are housed in huts that can be moved with a fork lift and placed at the desired locations. (b) Detectors: To get an idea of the size of the detectors needed for our purpose, note that for a solid angle of 1rmn‘(typical for a solid state detector of area 50 mm2 at a distance of 22 cm and therefore, a comparable count rate assuming same efficiency of detectnxn, a neutron detector at a distance of 100 meters from the target has to have an area of 10 m2. A second consideration is that neutron detectors are not 100% efficient. These two effects point in the direction of large detectors. In a large scintillator (>10cm in any dimension), there is some loss of time resolution because (i) the measured time of detection of a neutron depends on the position at which the scintillation event occurs; and (ii) the spatial distribution of the light on the photocathode is different for scintillations occuring at different points in the scintillator. The resulting loss of time resolution can be reduced if one arranges to determine the position of scintillation and applies a correction later. Alternately, a time compensation technique can be used. At IUCF, Goodman et. al., have employed a geometric approach to tube compensation (Go 78a, Go 78b, 00 79). The detector axes are tilted relative to the incident neutron direction such that the neutron and photon transit times are independent of the position at which the scintillation occurs. As can be seen from Figure 2.3, the time of arrival of a photon at the phototube from a scintillation occuring at coordinates x,y in the scintillator is . . .214... 3.9.51-4 151mb t(x,y,8,e) C0 + 0 cos 6 + c ( 8 cose) + c 8 (2'3) 23 .— OINL°OWG 77 - 7035 V \\ NEUTRON xcoso ysin¢ (Icos¢+ysin¢1 ' OIL-x1 '8. B: I- teas? Fig. 2.3. This figure shows the geometrical param- eters of time compensation. B is the ratio of neutron velocity to the velocity of light. c is the velocity of light. n is the index of refraction of the scintillator. tn is the transit time of the neutron and t is the transit time of the light (photon). L Es the length of the scintillator. (Figure and caption from Goodman etaal" (Go 78b).) 24 where to is the neutron time of flight up to the scintillator and other variables are defined in the figure caption. What one would like to achieve by time compensation is to make t nearly independent Of’ic and y for a given neutron energy i.e., a given value of B. It is assumed that the light is emitted isotropically. Light emitted with e>emax (limiting angle for total internal reflection) is lost. For an index of o refraction n - 1.58, emax = 51 . The time equation then implies that light from an instantaneous flash will arrive at the phototube over a period from t(x,y,8,e - 0°) to t(x,y,B,6 - 51°). In a real scintillator, the light is not emitted instantaneously; it follows an exponential decay curve with a characteristic decay time which for example, is 2.4 nsec for NE 102 scintillator. This is dominant ha determining the light curve at En - 100 MeV. Note that the light profiles illustrated in Figure 2.4a exhibit varying risetimes as well as varying amplitudes, (due to random scattering angle in the neutron reaction). Constant fraction timing can only compensate for variations in amplitudes. A form of extrapolated zero timing is employed at IUCF to compensate for varying risetimes. The principle behind this method is as follows: The puLse shape of the signal from the photocathode is found to have a parabolic shape near the origin, represented by A(t) . A ((t-t )/r)2 (2.4) 0 0 where t0 is the origin of the light pulse and both A arui T vary. 'The 0 objective is to determine t as marked in Figure 2.4b. Ikfidne two 0 9 25 TWNflE(ns1 (o) TIME (as) (b) Figure 2.4 (a) The curves show the fraction of forward. emitted light that has reached the phototube by time t, measured from when the neutron 'crosses the plane through the front face of the scintillator. The parameters used are: length of scintillator - l m, index of refraction - 1.6, phosphor decay constant - 2.4 ns, neutron energy - 100 MeV. The three curves are for scintillations at the fkont, middle and back of the scintillatOr. (b) This shows how time compensation is achieved by tilting the-scintillator. The calcula- tion is the same as for Fig. (a) except for the tilt. . - (Figure and caption from Goodman et al. , ‘ (Go 79).) 26 amplitudes A and A 1 2, such that the corresponding times t and t 1 2 satisfy t1 - to . t2 - t1 . (ta-t0) - (t1-t0) (2.5) Set up two discriminators with thresholds at A1 and A2 to start two time to amplitude converters (TACs) and measure (T-(t1-to)) and (T-(tZ-t )), O the stop time I being provided by the cyclotron rf to be described later. Subtracting the output of the second TAC from that of the first yields t -t ; with our choice of A and A 2 1 1 2, this is exactly the origin of time. Thus, if Equation 2.4 is a valid approximation to the portion of the pulses sensed by the discriminators, the required amplitude ratio A2/A1 can be shown to be 14. Then the tilt angle should be chosen to line up the the origin of the pulses and extrapolated zero timing should be used with A2/A1 - 14. Figure 2.4b shows how tilting the detectors lines up the origins of the pulses. It can be seen that time compensation is exact for neutrons of a particular energy only, because the tilt angle to accomplish it is derived from B, the neutron velocity (Equation 2.3). Calculated tilt angles vs. neutron energy for axial light rays are shown in Figure 2.5. In an experimental set up with long flight paths, one is far from having axial light rays; therefore, the tilt angle is determined by trial and error. A known sharp line is obtained from a known target. On line analysis gives the FWHM of this peak in the TOF spectrum. Tilt angle is changed until the highest resolution is obtained. At IUCF, a triple discriminator is used with levels 2 and 3 set fOr amplitudes A1 and A2 defined earlier. See Figure 2.7. Level 1 (the lowest threshold) .Ls set as high as 1744 to 1/2 of the maximum neutron energy because the flight 27 BO 70 4O 30- HLI ANGLE (no) 20— 10v— I i 1 1 1 I i 1 0' 20 40 so so too 120 140 160 180 200 NEUTRON ENERGY (Mew 0 Figure 2.5. This shows the required tilt angle O, as a function of neutron energy to achieve exact time compensa- tion for the axial light rays. (Figure and caption from Goodman et al., (Go 78b).) .‘ 013C11- mllt - [1:3- ....... ...... .... . “A: u "nu SHIFTII ’ 4 > m 5'” “st f—d 1111(qu 'cnuumn w . um 3mm. Fig. 22.6 Block diagram of. phase drift compensator. Figure and caption from Goodman et al- .(Go 79). 28 time of neutrons at that fraction of the energy becomes greater than the separation of the beam pulses, and neutron spectra from adjacent bursts would overlap if the threshold were set lower. (0) RF Timing with phase drift compensation: A precise timing signal for STOP input to the MOS can be derived from the cyclotron rf signal" ‘The Indiana cyclotron is a three stage system consisting of an ion source, a preaccelerator cyclotron and a main stage cyclotron. Under normal operating conditions, there are 4 to 6 bunches per orbit in the cyclotrons. Since the time separation between the bunches is too small for TOF studies with long paths, one bunch per orbit is selected, with the help of a pulse selector and a buncher located on the beam line between the ion source and the first cyclotron. The beam is swept across an aperture in a circle with a subharmonic of the cyclotron frequency, f. One uses 3/4 f or 5/6 f to achieve 1 of A or 1 of 6 selection respectively. The reference time for the TOF system 1:: taken from a phase coincidence between the f signal from the cyclotron master oscillator and the subfrequency. If the magnetic fields on the cyclotrons were stable, the proton transit time through the accelerator system would be constant and the stop signal would be stable. In practice, small phase drifts of the order of a few nanoseconds occur between the accelerating voltage and the proton bunches and compensation is necessary for good time resolution. The phase compensation method devised by Goodman et al., is illustrated in Figure 2.6. Protons elastically scattered from the target are detected with a fast scintillation counter located along a o 12 line with respect to the undeflected incident beam. The proton signal is set to trigger a discriminator which generates a pulse with a 29 width of about 1/2 the rf period. This pulse opens the current gate of a diode bridge. If the opening time is centered about the crossover point cm? the rf sine wave, then the net charge passing through the gate is zero. If there is a phase drift, this net charge is nonzero, being positive or negative, depending on the direction Of’the drift. The integrated output of the gate is a measure of the phase drift and is used as an error signal into a phase shifter that shifts the phase of the rf signal going to the stop pulse generator. The standard electronics employed at IUCF by Goodman et. al., for NTOF studies is shown in Figure 2.7. To obtain the highest resolution, the tilt angle was varied to optimize the peak to valley ratio of the barely resolved states in the 7Li(p,n)78e(g.s., 0.429 MeV) reaction. Level 1 was set at nominally 10 times the Compton edge from 228Th. Total charge was measured by split Faraday cups at the end of the third magnet in the neutron station. The other details of data acquisition are described in Chapter III. .Ammn oov..ue no seapoou sown coauomo can shaman b 30 .ueeeteexe as...» 05 e. we}: 3... .3. e3: 3 $29.30: no ...-.32.. zoo; m.~ .3..- .a:< .:.¢ua_e. A . ez<._ua . au>ud . t... on . weez>e . eepeupue ..IL. I“ :33 T N :23 , . L1 392 a Jesus ¢e~az.:.¢um.e 35.5. III. Data Acquisition And Reduction The experiment was carried out at the IUCF with a 119.3 MeV proton beam. Beam energy was obtained from the calibration of tune beam 40,42,44 and “8C8, 711, and 12C) were analysis system. The targets ( loaded on the ten position Geneva drive target ladder at the beam swinger» Thais target drive was remotely controlled through the Sigma-2 cyclotron controls computer. The targets were protected from oxidizing by the vacuum interlock of the target drive. The 00 flight path from target to center of detector was 131.52 meters long. The cyclotron rf was 28.72 MHz. With a 1 in 11 pulse selection, this corresponds to a beam repetition period of 139.3 nsec. Target information is summarized in Table 3.1. Four large volume plastic scintillators Table 3.1 Target Information Target Thickness Purity (mg/cmz) (Percentagefl “08a 29.2:0.3 99.965 l‘ZCa 30.5:0.5 93.60 ”“Ca 28.5:0.S 98.68 “88a 28.5:0.5 97.30 7L1 A3.1:0.3 99.99 ‘28 3u.9:o.5 99.99 and two anticoincidence paddles (to veto cosmic rays) were arranged ir1 the 00 hut as shown in Figure 3.1. The scintillators were coupled to 5" phototubes with tapered light pipes at both ends. Another scimniillator was housed in the 240 hut at a distance of 39.0 meters from the target, and data were accumulated, but were not used in the analysis. A 31 32 .u:: oo on» :H muouomumo mo ucmEmmcme< .H.m musmflm \\\\\\\\\\\\\\\\\\\ phonXX 1livn\ ptwm_ . oh 531,1321 I U. /../....n.m-m....w-m ....de. t mmmooonm 6cm nexmm nexmm on sexmm nexmm on sexed sexed 6» sexed . e ecmm m camm a camm H ocmm wouomumo Amamccmzo ca. muwflzm pfiouuzmo ocmm xmumcm .~.m manna 36 final TOF spectra for all targets and all angles including the cosmic uo,u2,uu and ray run. Figure 3.2 shows the results for 00 runs for the 8Ca targets. 2. Cosmic ray and foldover neutron background contributions and subtraction Cosmic ray events were partially vetoed by the arrangement of the anticoincidence paddles marked in Figure 3.1, but some background remains. This can be seen from the cosmic ray spectrum measured between the 0° and 60 runs. In the absence of any major transient phenomena occuring on the Sun during our runs, it can be assumed that the diurnal variation of the nuuni component of the cosmic ray background is negligible (W1 76); therefore it is possible to correct for the different counting times and subtract the cosmic ray background from the TOP spectra. The low counting rate for the cosmic ray background combined with the brief mmnudng time (1uh1 seconds) resulted in relatively large statistical uncertainties for all the thresholds except the lowest one. In addition, examination of the cosmic ray spectra revealed that the TAC had a nonlinear response for channels (290. To treat these effects, we first obtained average counts by summing over every 50 channels. Figure 3.3 shows the cosmic ray spectrum for the lowest threshold, with the open circles representing the averages over 50 channels. It can be seen that the TAC is linear for channels >300. There are 500 channels in this region which we define as the flat portion of the cosmic ray spectrum. The weighted average of the flat portion was obtained hm“ each threshold. Next, the region of the spectrum between channels 100 and 250 was examined for the lowest threshold (11xTh case) and a COUNTS PER CHANNEL ' 37 MSU-83-226 2501. 4000 1 0 l 1 1 1 _ Co(p,n)Sc 42Co Ep=|19.28 MeV 6LA&3=(31)° 400% THRESHOLD=18.7X r L O L 1 4‘ W 1" I “T 8000- ' 44Co 0 W1 1 1 1 1 48cc 3000- M V LA (3 :i“iA‘—;fi 1 l 1 l 250 500 750 TIME OF FLIGHT (CHANNEL NUMBER) Figure 3.2. Time of flight spectra for uo,u2,uu a nd “SCa (p,n) at 0°. 38 straight line approximation obtained. The two regions, channel >250 and channel <250, were joined smoothly for the 11x case where the statistics are good. The higher threshold spectra were obtained by scaling down the 11x spectrum using as scale factor, the ratio of the flat portion of the spectrum to that of the 1x case. Poor statistics made it impossible to obtain reliable TAC nonlinearities directly from these spectra. Figure 3.u shows the averaged cosmic ray spectrum for the lowest threshold” These spectra were then time normalized and subtracted from the TOP spectra for the different targets. In neutron time of flight studies using a pulsed beam, there exists the problem of slow neutrons from a certain beam burst and fast neutrons from the next burst arriving at the detector at the same time. To minimize this slow neutron background, the foldover neutron background” one has to set the hardware threshold fairly high; in our case, this was set at roughly 36.0 MeV neutron energy. The dynamic range of 120 MeV neutrons at a distance of 130 meters for pulsed beam of period 139 nsec is approximately 32.0 MeV. This means that to avoid the foldover background completely one has to have the hardware threshold of at least 88 - (120-32) MeV. But this will reduce the count rate severelyu .As a compromise, software thresholds between 50.0 and 80.0 MeV neutron energy were set within the data acquisition program; the plan was to accumulate all the data, and decide on a proper choice of threshold for analysis at a later time. Offline analysis of the data revealed that the foldover neutron background can be eliminated by extrapolating the TOP spectrum from below the ground state to higher excitation energies and subtracting it. This was done by examining the foldover neutron u u behavior in 60 and 110 spectra of the OCa(p,n) OSc reaction which has a no C) COUNTS PER CHANNEL (1) O O) C) 20 MSU-83-228 I T T f 1 I I f 1 j T I T COSMIC RAY SPECTRUM THRESHOLD = II x .L __ «b— l n I l l L l J I r f I I i I l AVERAGED COSMIC RAY SPECTRUM THRESHOLD = le .1 l J l 1 L 1 L L l 1 l L 200 400 600 TIME OF FLIGHT (CHANNEL NUMBER) Figure 3.3 (top). Cosmic ray spectrum (data) Figure 3.4 (bottom). Cosmic ray spectrum (average) 40 large negative 0 value and using this to guide the extrapolation in the case of the other calcium targets. The 00 spectrum from uoCa(p,n)uOSc which would have been ideal for this purpose had additional peaks arising from a leakthrough beam burst and could not be used. The foldover background thus obtained for the OO uoCa run was found to be selfconsistent. Figure 3.5 shows 1mCa(p,n) spectra at 0°, with the foldover background indicated. The errors accumulated by these subtractions are discussed in section 7 of this chapter. The spectra with the second lowest threshold (18.7x the 228m Compton edge) were found to be the best compromise between poor statistics and minimum foldover neutron background and were chosen for final analysis. 3. Deadtime Correction The ADC is dead to incoming signals while it is processing a previous event. This effect is significant at high count rates and has to be taken into account when we calculate the differential cross sections. In order to determine the ADC dead time, signals from the proton monitor and the four detectors in the 00 hut were sent into a sealer and also to the ADC. The ratio of the counts registered by the ADC to the counts registered by the scaler is a measure of the live time and is typically of the order of 80%. These fractional livetimes are the correction factors to the Faraday cup readings and measure the effective charge incident during the run. 11. Neutron detector efficiency and determination of absolute cross sections. In order to compute differential cross sections from the TOF measurements, it is necessary to measure, or calculate reliably, the detection efficiency of the neutron counters. The latter approach has NUMBER OF COUNTS 41 MSU-83-227 10000. t 44Co(p,n)44Sc ED: II9.3 MeV 7soo- 9 '-' 0.00 THRESHOLD = 18.7 x soon)- 2500 - Tl W TOF (CHANNEL NUMBER) Figure 3.5. Time of flight spectrum for HCa(p,n)“Sc at 0°, with cosmic ray contribution subtracted. Solid line indicates foldover neutron background. 42 been used by Rapaport et al., to predict the relative efficiency of the neutron counters for detecting neutrons in the energy range 30 MeV to 200 MeV for different light thresholds (Ta 82). Basically the program computes the probability that an incident neutron of a given energy will induce in the scintillator material, nuclear reactions whose charged products create more than a specified amount of light. Appendix C shows the computed efficiencies for the neutron energy range of interest. The relative differential cross sections so derived have to be normalized to absolute values. Two calibration runs were made at 00 with targets of 7Li and 120 and are shown in Figures 3.6a and 3.6b. The absolute cross sections are known in the two cases by independent means-"from angular distributions normalized to activation analysis cross sections for 7Li(p,n)7Be(O.0 + 0.A29 MeV) and from 12C(p,p')12C(15.1 MeV) and arguments of isospin conservation. These measurements have been made at Ep-120 MeV and reported elsewhere (Ta 82, Ha 81, 01 79). Comparison of these relative and absolute cross sections at 00 yields the cross section normalization constant; the relevant numbers are listed in Table 3.3. Note that the absolute cross section for the 1‘2C(p,n)12N(g.s.) reaction is only known to within 16% and the 7Li(p,n)7Be(g.s. + o.u29 MeV) cross section is known to within about 3%; but the normalization constants derived from the two cases agreed to within 6%. We took an arithmetic average of the two constants, 1vithout weighting them by their errors. The 7Li(p,n) and 12C(p,n) data can also be used to check the relative efficiencies used in the analysis. Define 43 .mmAA:.mvHAa How Esuuommm unmwaw mo mafia .Amvo.m mwsmflm EmeDZ JmZdeov 1.5;. ooh cow OOH oo. a11HaJIQwHildaai1nuflafluflnuflflnaMfiflflflflflflfifllflflflflflflfiflhfluflflfl r 1 08 0 0 flu MN , 60¢ a x Hm. u omozmmmE. «m r 00.0 n m 1 com 8 Ad >22 0m: 1 am w .. smacdrd 68W. 3 ..I . 1:22 810+ 000.9 . coo. — p P b — b — mONImQIDmZ 44 300 T , 1 r , M§”‘83'2°.8 (0.0, I') 270- .. 240- I2C(p,n)'2N d Sp: ”9.3 MEV 9=OO° d 2“” Threshold =I8.7 x " Z: :2 < IBO- « II o G: LLJ ISOr . Q. m I 1— 1 z 1on- ; . D 1 O 11 u .; 90H I n I BOr ‘ so 3 ! I a l l l l L l IOO 300 500 700 TOF (CHANNEL NUMBER) Figure 3.6b. Time of flight spectrum for 12C(p'n)12N. 45 .29 x h.ma u paocmmucfi um omen mmwocmwowwmm « .Nm m9 “mocmummwm An .mm 69 .mn Ho "mmocmummmm Am A.m.mv 1 .d «oh x meao.m Ano.fi+o.o mod x moo~.~ omoH.o m.ood ZNHA: .Omfl :6: mme.o..m.mv «OH x mHHm.m Amo.auo.dm sea x oma~.H oema.o m.HHH mmaxc.dsnaa .Amnmymm\Aamwvmm a Aumxnsv Am>HumHmuv A>mz. O ..mnmvae\oe A.Hmw.ce\oe «socmnOSOMmaonusmcm acnuommm . A00 UMV QQOMUOGm mmOHU HQMUCGHQHMHQ QUDHOmQ/N Cu m>wumHOm mo :ofiumNHHmeoz .m.m want 46 Peak Area (TOF) T,Effectivex Ndx Yield 5 rT,Effective a Faraday cup (total) x live time Ndx Target thickness in units of number/cm2 Y s Yield(7Li(p,n)7Be(g.s.+0.429 MeV)) Yield(12C(p,n)12N(g.s.)) Efficiency (117 MeV) (Th.) Efficiency (100 MeV) (Th.) 6(Th.) E 5(Th.) 5 Threshold (in equivalent electron energy) If the calculated efficiency had the correct energy dependence, then, (a) Plots of log Y vs. B(Th) and log e(Th) vs. B(Th) should be parallel curves; (b) Plot of R(E(Th)) vs. B(Th) should be a constant, independent of B(Th). The constant value - the ratio of experimentally determined absolute cross sections, to within experimental uncertainties. As indicated by Table 3.11 and Figures 3.7a and 3.7b, the relative efficiencies do have the correct behavior. Yet another check on the definition of the threshold and the corresponding efficiencies used in the calculations is to look for the constancy of do/d0 with respect to the threshold. For the nominal thresholds, there is a steady decrease of the inferred cross sections for 7L1 and 12C, totalling 36%,as one 47 00 on» nauun can «wagon .0663 due: 06:» cash ououomoa N can 0» vacuuowuoo «up new codenx no «you 03» one aa.ofihu.m I Aauaoaousaaoa unoccoampcu Beuuvm oos.cfi-o.m n amoum>a a .y mcw>auoc :« can: no: a» no ommuo>o may “menu ammumu ESMOAOO 1 HNIcH x omno.. o~.o+mcam.m ~oo~.~ a.ao.- .auoa a omnm.n HHNo.o nanoa x onmm.v oooo.¢ as x «a 1 Hausa x om~s.a m~.o+m~mo.o Sac..g ao~m.m n~1o~ x wa.o.~ ance.: n~1c~ x o.n~.a ammo.o as x MN . 1 , Nuuom x moam.~ ma o+~nnm.m ~um~.~ oewo.o nanod x n~h~.~ ma-.o -1¢~ x mace.“ ohm~.c as x as 1 -1o~ w amps.“ -.c+vnsm.m o~eo.~ hm~o.o MNIcH x ~o.~.v o~m~.o -1oa x m~mo.~ mno~.° as x cm .o>uuouomw Ao>wummmuv .~>. egos» .«u.»ocoao«uum ..A». edema .gus so:0w6uuum u a I hm n u uh I osmowne mmmmm a an A» .x >6: m.oe~n:ouuaozu ..a.m. >0: n.a-n=ouusmzm .>o: a~«.c ..u.ms ea 0 I Q 0 I u s nsoxgncqxnn a x62 awake .ONH, "SO\HNo~x~a n x62 can.= a.aah xmumcm paocmmunu Umasmmm no mewuocsm m mm m we :ofiumuameou ¢.m OHQMB .Hmcfifio: haze mum mosam> paonmmwnu mmmsu umnu muoz .mmpm :oumaou mo 3?: 5 3.8m .85 mod 6.8 a mod mo 3on 46:5 853m 2:: mu ON . m. o. q . i 48 :Nunoaami 49 .HmcfiEoc xaco mum czonm mosam> paozmmunu One .mmHuCHmuumoc: Hmucmeflwmmxm ou .Anvm.m pcm Amvo.m newsman cw csonm mmumum new UN_ can anazomCOwuommw Ac.mv uON mOHumH :oHuOOm mmouo OuDHOmnm pmcfiaumump adamucmEHHmmxm spa; mmmumm can mmsHm> HDOM may no mmmum>m pmunmamz msu ma mafia pflaom .Ammpm coumsou mo mbncs anvanevm .m> Assam mo scam .Ansa.m mnsmnm Aghvm Om mm ON m. . O. m q 4 q « O_N-mm-Dms_ 50 Table 3.5a Dependence of efficiency corrected peak areas on threshold energies 7L1(p,n)78e (g.s., 0.429 Mev) ENeutron‘=ll7‘° MeV éThreshold Peak Efficiency A/e A/s Area A e (A/e)10xTh (0.9) leTh 0.2150 141884 1.00 (1.0) leTh 30505 0.2035 149902 1.00 (1.1) leTh 0.1922 158715 1.00 (1.15) leTh 0.1866 163478 1.00 (0.9) l7xTh 0.1508 123607 0.87 (1.0) 17xTh 18640 0.1370 136058 0.91 (1 1) lTxTh 0.1246 149599 ' 0.94 (1.15)17xTh1 0.1185 157337 0.96 (0.9) 23xTh 0.1106 96130 0.68 (1.0) 23xTh 10632 0.0930 114323‘ 0.76 (1.1) 23xTh 0.0776 137010 0.86 (1.15)23xTh 0.0696 152715 0.93 (0.9) 28xTh 0.0866 65485 0.46 (1.0) 28xTh ~ 5671 0.0600 94517 ”0.63 (1.1) 28xTh 0.0427 132810 0.84 (1.15) 28xTh 0.0347 163618 1.0009 51 Table 3.5b Dependence of efficiency corrected peak areas on threshold energies 12C(p,n)”N (g.s.) ENeutron==100.0 MeV lThreshold Peak Efficiency A/e A/e Area A e (A/€)10xTh (0.9) leTh 0.2055 29188 1.00 (1.0) leTh 5999 0.1918 31277 1.00 (1.1) leTh 0.1801 33307 1.00 1.15 lOTh 0.1734 34595 1.00 (0.9) l7xTh 0.1358 23675 0.81 (1.0) 17xTh 3215 0.1185 27131 0.87 (1.1) l7xTh 0.1030 31229 0.94 1.15 l7xTh 0.0945 34021 0.98 (0.9) 23xTh 0.0857 17330 0.73 (1.0) 23xTh 1485 0.0660 22500 0.83 (1.1) 23xTh 0.0463 32080 1.03 (1'15)23XTh 0.0373 39812 1.15 (0.9) 28xTh 0.0477 11667 0.40 (1.0) 28xTh 557 0.0277 20108 0.64 (1.1) 28xTh 0.0194 28682 0.86 (1'15)28XTh 0.0148 37635 1.09 52 moves towards higher thresholds. A detailed analysis of the Compton spectrum from the 228Th source revealed that the thresholds were, in fact set about 10% higher than the nominal 10, 17, 23, and 28 times the Compton edge; therefore, the thresholds were at 26.18, 44.51, 60.21, and 71.97 MeV equivalent electron energy. With this correction, the cross sections do remain a constant to within 15% for all the thresholds. (See Tables 3.5a and 3.5b). This was further verified with the calcium target data. Tests (a) and (b) mentioned above worked as well as they did because ratios were considered in each case; this shows the insensitivity of the derived normalized cross sections to the precise value of the threshold. 5. Neutron Energy Spectra The TOF spectra (after subtracting the Cosmic ray and the foldover neutron background) have been converted to neutron energy spectra with the relative detector efficiency folded in, using the M.S.U program TOFTOEN. The input data required are distance from target to detector, detector efficiency as a function of neutron energy, proton beam repetition period, TAC calibration in terms of nsec/channel, and the centroid of one peak with known neutron energy. The neumwxienergy calibration for the spectra shown in Figure 3.8 is ENeutron(Mev) a (channel number + 2125)/25 Appendix C shows energy spectra for all calcium targets at the 3 angles 0.00, 6.30 and 11 .10 These spectra have been analyzed with the peak fitting program SCOPEFIT, defining backgrounds as shown in Figure 3.8. A reference peak was defined in each case based on a sharp peak in the 53 MSU-83-23I 4 4CRSO 2( (D|flflaaiam~uzi§PEEhZl*$==-nn-_dm__¢__.dh__.__ 4| 20- C0(p,n)Sc C0 Ep= II9.3 MeV 3> Q) 9 =WDID° :5 LAB 3;K)r \ .0 s I 00 U 0 1 1 1 1 C3 1’ 44 blCN- N ‘U Figure 3.8. Energy Spectra for and “3Ca(p,n)“°'“ ' Experimenter's backgrounds defined 105 110 115 ENEUTRON (MeV) 95 H30 40,42,44 ““ and “88c. peaks are indicated by solid lines. to fit 54 high neutron energy end of the spectrum, peaks fitted and areas and centroids obtained. See Tables 3.6, 3,7, 3.8 and 3.9. 1x;should be noted that a constant time resolution does not yield a constant energy' resolution; but the neutron energy range in the parts of the spectra that were fitted with a given reference peak shape was small enough that that peak width did not change by more than 9%. This has a negligible effect on the derived centroid for the strong peaks which is known to + 40 Kev (i 1 channel). Relative differential cross sections were converted to absolute values using the normalization constant derived by the method outlined in Section 4 and are listed in Tables 3.6, 3.7, 3.8, and 3.9. Angular distributions are plotted in Figures 3.9, 3.10a, 3.10b, 40,92.”“ and “80a respectively. The 3.11a, 3.11b and 3.12a, 3.12b for TAC nonlinearity mentioned earlier is reflected N1 the energy spectra” ‘Table 3.10 shows theineutron energies at which this effect is starting to influence the energy spectra 6. Calculation of the GT strength The angular distributions were used to pick 3 (N~Z) (Ta 81). (See Appendix D). It should be noted that the experimentally extracted strengths are independent of the absolute cross section normalization. The case Of l‘2Ca is an anomaly within our measurements. This has been brought about by the fact that the target was contaminated with oxygen and that the beam was apparently hitting the alwmnumitarget 4 frame during at.least part of the 00 run. The bump in the 2Ca(p,n) SS emd.oHomm.H wv~.oumom.H H>~.ofievo.m am.ma 0» em.o m~.oH oao.oumea.o emo.oflsm~.o mmo.owm~e.o .mm.o 00 mm.m ~H.6 omc.ouodm.o mac.oufima.o mmo.cumm~.o mm.m on mm.e mm.v mmo.cHon.c oeo.oHHmo.o mHH.onm~.H e~.6 ob as.~ mv.m ano.oumsm.o omo.ouosm.o amH.cH~ms.H ma.~ on mm.o om.a oma.oudom.a Hav.oummm.q mam.cH~qm.oH m~.H 00 Ha.c Ho.o meo.oweom.o mmo.cum~m.c Hea.oumvm.fi mm.o on me.o1 oo.o X 0H.HH 0m.o oo.o A>mzv m .Aum\nsvee\oe muflsga ¥>0zvxm OmNeA:.me00ms Ooh mcoflusnfiuumfle Omasmcm .e.m manna mmo.oHH6N.o mao.oumva.c Ado.oueo~.o m~.o on ea.m ms.m mac.oumom.o ~mo.owemm.o Heo.ouemm.o am.e on mm.m -.e omo.ouoqa.o mmo.oume~.o omo.cwemm.o m~.m on mm.~ me.~ oeo.oueae.o smo.ouem~.o «Ho.chOH.o mm.~ on H4.H Hm.a oHH.oHHm~.H mAH.oHv-.o mmo.ofi~sm.o mm.H 00 am.o om.o 0H.HH 0m.o oo.o A>0zvxm Aum\mav cp\oc muHEHA ¥>mzvxm .0 omovA: .moo v Hem mcoHusnwuumwp undamC¢ .o.m manna S6 ovo.onmm.o mmc.oH~mH.o mma.ouqmn.o ms.qa 00 om.Hd mm.- mvo.oudme.o oe~.ommoe.~ om.HH 0» 66.8 aa.m mao.oumso.o meo.oHvem.o msa.owmeo.fi oe.m cu mm.o Hm.s hmo.ouemm.o msa.ouokm.a emq.oumam.v mm.o ob om.v s~.m mmo.owmam.a HHH.oHaHH.H Hmv.owmos.v mm.e 0» oo.m om.m moo.ouoem.o mma.oudmm.a «mm.ouamm.m mm.m ob mo.m NH.m sac.ofieee.o som.ousflm.m qvv.onsm.v m~.m ob 8~.~ me.~ omo.oueom.o mmo.cummfl.o mec.oflmmv.o -.~ 00 mm.H me.a omo.oumoo.~ eo~.onHm.m emv.oum-.m mk.a 00 va.o 56.0 OH.HH Om.m oo.o A>0zvxm lum\nsvee\oe mugsfia A>02smeL omva:.QVOU new mcoHuznfluume Hmasmcd vv m.m manme _ 66H.6+~66.HA 66H.6H666.~ 66~.6H66m.m 6.6H ob 66.6H 6.6M 666.6HHH6.6 mam.oH6H~.6~ 666.~Hsm6.6~ 66.6H 00 66.6 ~6.HH A6H.6H666.H H66.6HH6H.6 666.6H666.6 66.6 00 66.6 66.k 66H.6H~66.H mam.6u666.6 666.6flmmm.6 66.6 on 66.6 66.6 M66.6H666.o ~66.6Hmm6.o mm~.oH6~6.~ H6.6 on 66.6 66.6 ~66.6H6M6.6 moa.oua6o.a 66H.6H6~6.H 66.6 on 66.6 ma.6 6~H.6H6Hm.d 666.6H666.6 666.6H666.6 66.6 on mm.~ 66.m 666.6HN66.H 666.6HH66.6 666.6H666.6 6H.6 0» 66.~ 6m.m 66H.6H~6H.H 6mm.oH6H6.m 666.6H66H.6 Hm.m ob H6.H ~6.~ 666.6HN66.6 H66.6H66m.6 666.6H66~.6 66.A on 6~.H 66.H M66.6H666.6 6H6.6H~6H.o mmo.oH~Hm.o 66.H 00 mg.o 66.6 0H.HH Om.6 06.6 A>0zvxm .wm\nssce\oe mugsga A>0zvx6 Ommv.:.mvmo HON mcoflusnfiuumflc unazmc< mv 6.6 0~nme 58 Table 3.10. Neutron Energies (in MeV) below which TAC nonlinearity is present in the energy spectra \. 6 Target x“ 0.0° 1 6.3° ll.l° “°Ca 97.40 97.16 97.20 “2Ca 98.04 97.12 97.20 HCa 98.12 97.20 97.20 “°Ca 98.36 97.12 97.24, 1 dJ/dfl (mb/Sr) 59 MSU-BB-ZOI '0-0_ 1 T I T _, ,_ 4OCO(D,O)4OSC .. E E =119.3 MeV 7 L- p d r- -I L . AVERAGE 1_=O/ _ DISTRIBUTION 3 FROM 42~44v4806(p.n1 (from IAS states) (.0:— -_I g .. \i\ \ 2.73 MeV .. \ \1/ - \ \‘E J l L I 0.2) 5 IO Blob Figure 3.9. Angular distribution of 1+ state in “°Sc (dotted line). Solid line shows an average of the l+ angular distributions derived from “2,4“ and “88C- 60 MSU-83-202 42Co(p,n)425c 7 E =119.3 MeV 4 . ~ ‘ 10.28 MeV P \ \ 1- ‘ \ - . . \\i~ L x1O 10.0 , .3 I: \ \ 0.6l MBV : \ .- \ .1 P '\ \’ 4 D \ ‘i d r- \ c1 ’2 \ 3 (D ‘ \ B .. ._ ‘43?) MeV \ x10 E - 6 l g i} 3 <2 .‘-l‘ \ U \ 9.5. (I.A.S.) 9 \ . *4 LO:’ ‘\ \. 'j .. L j P \ ' 4. \ q 4,... _ ‘ 6.!2 MeV \ .. 4’ § ‘ ‘ \ 1- ‘ .1 16 I \ \- - r ‘\ \I l l 0.10 5 ‘0 Figure 3.10(a). 69Iob Angular distributions of observed states in “28c. dU/dfl (mb/sr) OJ 61 MSU-83-203 ¢ I‘x \ ‘ ~ \ I.BO MeV 42Co (p, n) 423c Ep =119.3 MeV 7 Figure 3.10(b). .. \ _. .- \ .1 . §-_~ -. I— ‘ ‘ ~i .4 h 4 .. XIO. )— -I (L _ T \ \ 3.43 MeV _ 1— \ d \ F \ fl .- \ -I {6 I— \ d H \‘\‘ - \ \ \i 1 )- d I l O 5 IO Glob Same as Figure 3.10(a). 62 MSU-BS-ZOS 44COIp,n)44Sc ‘ I- \ .1 \ \ I- \ d ‘L \ \ \ \ Ioo- \ u. I- \ .1 - ~§ 3 _. x10 3 ,1 1'- 6-‘ 2.79 (1.4.5.) 7 b 1- \ Q ‘\ 7 g I- §\ 1 v \ d \ ‘D >- \ -( 'B \ ‘R \ ‘ \ LOr- \ .— : \f : I .1 1*\ P -1 __ \ \ -( \ I- '\ -I \ \ \ ,—§ OJ 1 3-..-‘T l O 5 IO {Rob Figure 3.ll(a). Angular distributions of observed states in ““Sc. 63 MSU- 83-204 44CO(D, n) 445C \ \ q \ \ 0.67 MeV E = 119.3 MeV - «\ “ P .‘ - x.\ \n\ 6 \ \ \ \.\ \R\- §\'\ 7 . .\ . \ \ \ 977’NEV \ '\ IO \ \ 1/ \ \ ' 3' \ \ ‘\ i -: H \ \ ,/\'\ . I 2‘ \ \ 3.12 MeV\§ : f 7.31 MeV \ \§ _. E7 4" \ \ -1 .o \ \ E h \\l.78 MeV \ " V 1 <3 \ \ 1E . \\~ \ l’,§ .q ‘o \i_..—-‘<\ \ 0.“? \ -—I - \ g ‘13 f 7 1L ‘\ 7 \ 12 82 M v 1‘ .. \ . e . - \ q \ . F \ //T H \ // x10 '- \ / .1 ‘\f ‘,‘/ 0.010 g '10 Blob Figure 3.ll(b). Same Figure 3.ll(a). ch/dfl (mb/sr) 64 MSU-83-207 r T 148 ‘48 “3.0L CoIp,n) Sc —1 .. E =119.3 MeV '1 - “ P ‘ 1- \ -‘ H ‘6‘\ . 4 . \\6.67 MeV (1.4.5.) .. , \. . 1- §\ q ‘\ _ ‘x - \ Ix \ \ \536 MeV \\ ‘\ 1.0; \\ —- _~‘ 7.8 MeV ~ ~ ‘\ . ‘\ - I- \ \ i‘ .- _ .- ..- .{ -I _ \6 - \ h— \\ "' 1— §\ ’ "‘ ‘4 1 __ \ .. ‘\ \ \ 1- \i "" x10 1 I 0.10 5 ‘0 Blob Figure 3.12(a). Angular distributions of observed states in “88c. dU/dfl. (mb/sr) MSU-83-206 T T i 48CoIp,n)"‘8Sc .. \ ‘I ~\ Ep =119.3 MeV .. ‘\ ”.02 MeV 4 '\ '\ \ \\ 40.0"" §\ "1 1- \ q 1’." \ 'I ~. \~ ‘ ‘\ 2.52 MBV \ .1 \ \ \ -1 \\\ \‘§ .1 ‘ ‘ \ q ‘ \ \ x \ \ \ ‘ \\ .1 \ ‘-_§ \ \ \ - i '0'" T‘\ -1 I- \ d I" \ \ d b \ d , sf. 4 \ d f 6 0.67 MeV fl} . I‘ \ / \ / r- \ / “ \ / \ .. \ ,’ . 0.1 1 1 Glob Figure 3.12(b). Same as Figure 3.12(a ). 66 . 42 . spectrum just below the ground state in So is at the correct energy for the 27 Al(p,n) reaction. Therefore, the apparent measured GT strength of roughly 82% of the sum rule prediction does not have much reliability. The following reasoning might give a rough estimate of what was actually seen from our run, excluding possible contributions from oxygen and aluminum. Consider the high excitation regions of the “2’“ and l‘8Sc spectra with no sharp resonances. The cross sections to this part of the spectra can come from (a) valence neutrons, and therefore, should scale roughly as the neutron excess in the target and should be compared at the same excitation energy in the residual nuclei and (b) valence neutrons from the “00a core, and therefore, should be the same for all Ca isotopes, and should be compared at the same Q value (same neutron energy). For the sake of simplicity, let us assume that the knockout neutron background is independent of excitation energy in the residual nucleus within the region of interest. Then we can write, Height(Bkg) - C0 + (N-Z) x C1 .. . 1111 48 where to and C1 are constants to be determined. From the and So cases, we can solve uniquely for CO and C1. Comparing the measured background height to that predicted by the constants C and C for “23¢ O 1 would then provide us with a scale factor with which to reduce the 14 measured strength in 2Ca. For example, choose a neutron energy of 100.0 MeV; the measured heights of the backgrounds for the three cases 112,49 and ”880, are 1.83, 2.16, and 3.41 mb/sr, MeV respectivelY- Solving for CO and C1 from the uu’HSCa data one gets 67 CO - 0.91 mb/sr, MeV, and C1 - 0.31 mb/sr, MeV; Then the predicted height for 142Ca is 1.53; comparing this to the measured value of 1.83 mb/sr MeV one gets the correction factor to be 0.83 in the knockout region. The measured GT strength of 82% should be scaled by this factor to give a corrected strength of 68%. One sees in the results for 44 and u8Ca the so called quenching of the GT strength (40.5% and 51. % respectively of the sum rule prediction) that has been seen in recent (p,n) reaction studies at intermediate energies. Suggestions by Osterfeld that substantial 1+ strength may be hidden in the experimenter's background drawn to extract the above cross sections was investigated in detail, and is discussed in Chapter IV. 7. Error Analysis There are two types Of errors affecting our measurements--systematic and statistical. Sources of systematic error include target thickness uncertainty (1 to 2%), current integrator error (2%), and error in the normalization constant to convert relative differential cross sections to absolute values (8.5%). Sources of statistical errors are the uncertainties in the Monte Carlo calculations of the relative efficiencies (1 to 3%), Cosmic ray and foldover neutron background subtraction (0.1 to 3%), and background definition and peak fitting (0.5 to 5%). By the nature of the method used to compute total OT strength i.e., as a ratio to the IAS peak, the systematic errors do not contribute, only the statistical errors are relevant. But the absolute differential cross sections quoted here carry both the statistical and the systematic errors, which were added in quadrature. These were in the range of 8 to 19%, typically 10%. IV. Data Analysis In this chapter, some of the methods used to determine if there really is a quenching of the GT strength in calcium isotopes are discussed. It is appropriate to start with the question of whether the experimenter's background contains substantial 1+ strength and the basis for such a claim. Recently, Osterfeld performed microscopic background ”O’H8Ca at 160 MeV (0f 82). His calculations for (p,n) reactions on model assumptions were: (i) For (p,n) reactions at incident energies >100 MeV, the reaction mechanism is direct, i.e., one step processes dominate; (ii) The effective projectile-target nucleon interaction can be represented by the free nucleon-nucleon t matrix, iHAe., by the G3! interaction of Love and Franey (impulse approximation); (iii) The (p,n) background is dominated by spin-flip transitions, i.e., 8:1, T-1; The final nuclear states are assumed to be simple proton particle-neutron hole states, including bound, quasi bound, and continuum states. The cross sections were calculated with a DWBA code. This code includes knockout exchange amplitudes exactly. Figure 4.1 shows a schematic representathmicfi'the model. This model reproduces 00 data for usCa (p,n)u8Sc in the continuum to within a factor of 1.3. A striking prediction of these calculations is that the continuum background drops to zero rather sharply at Q - -20 MeV, for uaCa; a similar behavior is predicted for uOCa (p,n) at‘.‘N~2\\V{\\ 7O 3.— 1 1.3 -' (a) Ca (p, n) ‘aSc ... i" f E:160 MeV 111.; 1 2‘“ : 69'“? 0' oius 11m .‘5’, 10 L “-‘talttatw ‘ \ ‘--- talc. oxhqmtuxt 331 ‘1 2 [ --°~-eta.:atiu9rm 1' 7:1. I - I inbfl'xtoc ' ‘ 6° % S L j 'o g: ’ ~ . ‘ ’ --.~::."—-"“ """"" 1’ ("‘50 T1} ....... Li” D L’ 735.. L l 0.1 ‘3 ‘ ‘ L I to - ‘ T *— ‘ LO LO (0) 1 I CaIp.nI Sc 1 6:160M9V S .- 10 -Olp,nl IMeVl FIG.4.2 Zero degree spectra for the reactions "Cam/t) (a) and ”Ca(p.n) (b). The data (thick full line) are taken from Refs. 13 and 14 (see text). The discrete lines are cal- culated cross sections due. to bound and quasibound States. The arrow labeled with AI -1 indicates the location where the AL -1 resonance (0’. l’.2’) would occur if nuclear oolleetivity were included for these states. The theoretical cross sections due to the GTR and IAS are nor plotted. The optical parameters for the cross-section calculations have been taken from Ref. 20. (Figure and caption from Osterfeld’s work (Of 82).) 71 nuclear surface; this means that the proton wavefunction is small near the nuclear surface and so are the transition rates to these states, particularly when L .. O. The implication, then, is that most of the background subtracted in the analysis of “8Ca(p,n) is in fact, GT strength. Osterfeld finds that including this background raises the fraction of the sum rule strength observed in this case from H31 to 51%. Inspired by the above work, we have analyzed our data following a method suggested by Rapaport (Ra 82). The energy spectra were used to compute cross sections in 2 MeV bins from the ground state upwards, peaks and background included. The angular distributions so derived, were fitted with linear combinatins of DWBA cross sections to final states 1+, 1-, and 3+. A least squares fitting routine was used to minimize X2 for combinations of these final states, taken two at a time and that pair which gave the least X2 was chosen to obtain the corresponding spectroscopic strengths. The code used was DWBA 79, with the free nucleon-nucleon matrix of Love and Franey; only «f5/2vf;}2 configurations were considered. Including 1rf caused negligible vi"-1 7/2 7/2 Change in the angular distributions. Table ll.l lists the optical model parameters used in computing the DWBA cross sections; Figure 14.3 shows comparisons of measured and predicted DWBA cross sections for known States in ”2 and “880. Tables 14.2 and ”.3 list the results of this type Of analysis for “MB Ca. A similar analysis was not carried out for Ca because of contamination with oxygen and aluminum. As a rule, we 0- Li” ’48 T. + + a ind that for Ca and Ca a mixture of l and 3 states represents the + .. data at low excitations and a combination of 1 and 1 is required to reproduce our data at higher excitations. It is interesting to note that Osterfeld's prediction is borne out by the behavior of l- strength, as 72 Table 4.1 Optical Model Parameters+ RC: 1.25 fm Vol. Real V: 9.73 MeV r5 = 1444 fm a0 = 0.52 fm Vol. Imaginary W==13.73 MeV r0 = 1.24 fm a0 = 0.57 fm 80 Real VSO = 3.0 MeV r50: 1.06 fm aSO= 0.6 fm SO Imaginary WSO==-l.00 MeV r = 1.06 fm Wso a = 0.6 fm Wso 1'Optical Model parameters provided by N. Anantaraman (Ar 83) and derived from p+53Ni data at 157 MeV. See also Comparat et al. (Co 74) . 73 MSU-83427l r I 1 48Co(p, n)488c Ex=2.52 MeV '0 2 42Co(p,n)42$c Ex=0.6l MeV air- l g .. I- \ \ \ fi 5 — x \ _. - \ \ + d .\ ... . x‘ \ . 3’ ‘ 1 .LD _ ‘\ - 5: \ C3 ‘\ 'U 1’ \ B \l 13 |() .~ )( '1: - L .‘ x.“ 4;: p \t - _ - \ fl 5'-' .‘axz‘: '- - ‘\ a \ 2 ‘\ _ \. - _ 0 Data \\ l X DWBA '79 \\ I 1 l (3 5 H3 6lob Figure 4.3. Comparison of measured and DWBA 79 predicted differential cross sections for 1+ states in “2Ca(p,n)“ZSc and “°Ca(p,n)“§Sc. '74 Table 4.2 HCa(p,n)""Sc Contributions to 0° cross sections from 1*, 1' and 3+ states. Ex(MeV) do/dQ (mb/sr)(0°) 1+ 1' 3+ 1.0 6.401 - ' 0.208 3.0 8.757 - 0.256 5.0 7.298 - 0.377 7.0 4.024 - 0.321 “9.0 4.690 - 0.508 11.0 4.632 - 0.774 13.0 5.439 0.155 - 15.0 4.806 0.246 - 17.0 5.104 0.348 - 19.0 6.223 0.234 - 21.0 5.694 0.692 - 75 Table 4.3 Ca(p,n) Sc Contributions to 0° cross sections from 1*, 1' and 3+ states. Ex(MeV) + do/dQ‘(mb/sr) + 1 l 3 1.0 0.488 - .405 3.0 6.754 0.426 - 5.0 3.181 - .689 7.0 5.093 0.283 - 9.0 11.045 0.169 - 11.0 13.799 0.174 - 13.0 8.516 0.165 - 15.0 5.008 0.214 - 17.0 6.814 0.339 - 19.0 5.232 0.488 - 21.0 5.247 0.699 - 76 extracted from our data. The 1+, 1‘ and 3+ strengths from the best fits are plotted vs. excitation energy in scandium and displayed in Figures 4.4 and 4.5 for A =- 44 and 48. One can also see that 1+ strength extends to higher excitations than was previously thought. Another way to extract 1+ strength from (p,n) spectra was recently’ suggested by Goodman and applied to the case of “20a(p,n) (Go 82). The criterion for GT strength is that the angular distribution be that of L - 0. The object is to subtract L40 contributions from the Co spectrum. This is done by first subtracting the 00 spectrum from the 2.50 spectrum scaled by the angular distribution for the L - 0 part so that the strong GT peak subtracts out. The result is taken to be an approximation of the La-O spectral shape as seen at 0°. This is then sealed by the cross section ratio between the 2.50 and 00 spectra in the region of the L-1 1°esonance and is subtracted from the 00 spectrum to yield the L-O .spectrum at 0°. It is instructive to apply the above method in-the idealized case shown in Figure 4.6(a) to see its usefulness and check the validity 6: the argument. We see that the method would work well if only one Lao component, say L-1, is important, and if there were no [.80 (1+) strength in the region of the 1- resonance. These are implicit assumptions in Goodman's method. If one used the ratio of cross sections in the Lai region to Scale the so called L-O spectrum, and subtract it from the OO spectrum to obtain a pure 1+ spectrum, then at least a part of the 1+ strength Present in that region is subtracted out too. There is no reason for an a priori assumption of no 1+ strength at high excitations. In fact, our fits to the data (peak + background) through the observed range of excitation indicate just the opposite. Therefore, we believe that 77 :oHumufloxw .m> mnumcouum +m one N ¢ m .oo um omsgA:.m.muss :fi xmwmco 1H .+H no uon .v.q ouomflm :62 v x u IV. 0 O. N. S m. m. ON I ”.......u...ooo.co ..o.....oManaflu-nI.f_fl..01.-4:le 00.0nm >62 mm: om: E 3 53. mNN-mm-Dm§ 78 GOflumuHOXQ .m> m . . :umcou m u. +m Uflm 0° um UWQ:A:~vaUQ: :fl hmumcm H .+H «0 uoam .m.v mHflmfim AV §>053ulel'v m O_ N. V. @— .nHwIH.nrn‘Hu?LHQIITH WIL I. mw_ AON ..l-:o N4 I. V: _ 1 m. + AwnFDo 1 01 n21 .LUAVHQ NT. >oJ_MA£. ommv E 3 come . .V— p . . p p - OMN-mm-3m_2 79 MSU-83-212 (o) I+ 9=0.0° _ 8 A 'I+ 3; 2 9: r- (b) 8=2.5° 3. 1* <2- |+ A .. {5 Q i L 7°" (c) I" k x (9=2.5°) k=4/2=2 5. . g l 5. l" 3. at (d) "' L’O SPECTRUM. = kX(9=2.5°)- g; (9=O°) 1i Figure 4.6. Application of Goodman's method in an idealized case. 80 MSU-83-243 (e) I- "LfO" spectrum rescalsd to match "1 of 6-6 ;* scale factor 7.5 7.5 25 L5H41'3”° (2jfi (f) _ "’ "Pure 1+" spectru- (Goodman's) (Note loss of 1* from high excitation, as a result of the assumption). (413) 5. *Including the l+ at high excitation as 1- leads to the wrong scale factnr of 3.0; should be 7.5/1.5 - 5.0; making this correction leads to (e') and (E'). (er) '- "Lia" rescaled a I correctly. :5 "F (1") “Pure 1+" spectrum '4' (413) urn ,__ Figure 4.6 continued 81 Goodman's method is correct only up to the point where he obtains the Lao spectrum. Therefore we used it to obtain the Lao spectra from the 42,44 and ”80a. These are shown in Figure 4.7. The 00 and 6.3° data for small peaks in the region of the strong GT (1+) at low excitation arise from the fact that we did not apply a correction for kinematic and electronic shifts of the peak. A comparison can now be made of the 1- behavior as derived from the methods of Rapaport and Goodman and an estimate of the background falloff energy for 120 MeV protons on “2"“; and l‘8Ca from Osterfeld's work at 160 MeV. As can be seen from Table 4.4., the agreement is not bad, considering the crudeness of our procedure. The 1+ cross sections at 0°, derived from our DWBA analysis (peak and background included) were used to compute the total GT strength again. We found that for M and ”Ca, 78% and 63% of the Sum rule predictions were obtained respectively. Appendix 0 contains the Tables listing the computations of the GT strength. Our analysis conforms with Osterfeld's calculations; there is some 1‘F contribution from the background; but one has to look elsewhere for at least part of the sum F‘Ule strength. It should, however, be remembered that the decomposition of the data into different final state angular momenta, with only 3 f‘Oicward angles is far from reliable. We therefore, believe that additional data at somewhat larger angles would help resolve this question unambiguously. One should also bear in mind the limitations of uSing the code DWBA 79 which assumes that the final states are bound While, in fact, they are not. Further, one does not have a check on the Constancy of the angular distributions with excitation energy in the 1"esidual nucleus. Very often, DWBA predictions are not accurate because, 82 4338......“ .. new Joannflo um. 630096. 83 .54 953a :63 62.32“. . 0: no. 00. mm oN_. n: 7 q . . . 0 0x4 1 00.0 um . >02 ndzwau $24.53 oomv OOOn . o I g .608. ,. >22 3:781 .068 - T WENNVHD 33d SanOD . 00.0 u G >62 m 27am . omwct? Eoouvr . mON-mm-:m2 83 A>oz :«v mofimuocm codumufioxo out ~H<+ H.h~ c.m~ e.ma moo: m.m~ o.m ~.m mos: q.oH c.HH m.m mu~: coHumasono . Atacama m.:macoooy m.©aomuoumo Avonuos m.uuoammmmv Eswuoomm cumq Eoum uomwme Eowm oucEaumm nuacmuum IH mo ummco +amwmem buoqamu -H ANN mo Eouwv mmwmumcm umOaadw ocsoumxomn cam mutt ucommum Scum on>mnon Ia wo cowawcmeoo ¢.v mane? 84 for example, the effects of density dependence of the two body force Verr are not very well understood. There exists yet another way to extract GT strength in a straightforward way from our data. Recall that the method outlined in Chapter I and used to compute the GT strengths quoted in Chapter III relies on normalizing the 1+ cross sections to that of the IAS; therefore, it is very sensitive to the measured cross section for the IAS. When there is an overlap of peaks near the IAS as in 44,48 errors are larger than if the IAS were isolated as in "2 Ca. Consider Ca, the now the measured GT strength from the 0.611 MeV peak in “280. Our calculations give a value of 2.55 (using an experimenter's background) while the matrix element obtained from B decay is 2.67 (Go 81). Therefore one can normalize all the measured 1+ cross sections to the 0.611 MeV cross section in l‘ZSc, with a known strength. This way, we can also extract BEx(GT) for the 2.73 MeV state in noSc. We carried out such an analysis and obtained total GT strengths of 57.2% and 69.4% of the minimum sum rule prediction for 44 and 1”3C a, using an experimenter's background. When one includes 1+ contributions from the background as derived from the DWBA analysis, the total GT strengths are 110.7% and 82.9% of the sum rule prediction for 44 and “Ca. The major limitation of this method is that it is sensitive to errors in normalizations arising from charge and target thickness uncertainties while the method of Taddeucci et al., is independent of such errors. Note also that the difference between the 2 methods results partly from 42,44,481 the fact that the measured IAS cross sections for Ca do not scale exactly with N-Z. Another reason the strength is larger when 85 normalized to 0.611 MeV state is that the extracted strength of 2.55 for the state is scaled to 2.67 (obtained from 8 decay measurements). The large GT strength for uuCa as indicated by the DWBA analysis is presently not understood. Unfortunately, there are no previous (p,n) measurements on this target at intermediate energies for us to compare to. Evidently, this results from the persistence of considerable 1+ strength at high excitations (see Figures 4.5 and 4.6) for 1mCa, unlike the case of uOCa. We are currently investigating this. In the uoCa (p,n) data, there is a peak at 2.73 MeV, with L - 0 angular distribution. Normalizing to 0.611 MeV gives a strength of B (GT) = Ex 0.098 which compares well with the values of B x (GT) 0.15 5 0.04 and E 0.13 5 0.04 at 159.34 and 200.0 MeV respectively reported by Taddeucci et al., (Ta 82) V. SUMMARY The total GT strengths (percent of minimum sum rule prediction) extracted from our data using the different methods outlined earlier are shown below in Table 5.1. If one believes the fits obtained with the DWBA 79 analysis, it would seem that substantial GT strength is contained in the background and extends to higher excitations, as proposed by Bertsch, et al., (Be 82). But one should be aware of the ambiguities of these fits, as discussed in Chapter IV. Our data for “00a indicate a GT strength of 0.098 from the peak at Exza' 2.73 MeV. This compares with the values of 0.15 + 0.04 and 0.13 + 0.04 reported by Taddeucci et al.at rip-159.0 and 200 MeV respectively, (Ta 81). Another finding from our data is that the 16.8 MeV state in “880 is about 13% wider than the state at 2.52 MeV excitation. The FWHM's in the TOF spectra for these states are 8.5 channels (Ex . 16.8 MeV) and 7.5 channels (Ex - 2.52 MeV); this observation was made earlier by Anderson et al., (An 80). Comparison of our data to the electron scattering studies of Steffen et al., (St 80) indicated the following (see Figs. 5.1 and 5.2). (a) The 2.73 MeV peak in ”03c has been identified on the analog <0f the 10.32 MeV state in “00a (Ta 82); it has an angular distribution corresponding to L - 0. (b) More structure is seen in “23c than just the analog of the 11.2 MeV state in “ZCa, although it has not been isolated and identified in our data. (0) Electron scattering reveals practically no structure in uuCa, While the (p,n) experiment indicates significant GT'strength in the excitation range 10.8 to 14.5 MeV. 86 87 .Ammmas mos .mm o .>0m .msne .eamobmbmo .mln .Aammac woe .meoa .0004 .m>:m ..Hm um cmeeooo .o.olm I O O O O O m Ano am a mm o No Ano mv v mm m Hm Umv I h.oaa m.mh I «.mm m.ov Mva II I ll 0 .I. e mu Amp mm 0 mm Na oumum >02 oumum >0: unmEowsmmoz Ham.o ou de ou acoEmemmwz Ham.o ou m02 xucocm cozozuxm N. 2 O— o 4 .11 14.47.41 4-- 1. 14-1111- 0 r — — i Illi’f}; Nu!" i‘e;‘zev\e .5 + . a w a o . ..o 3 609 ... n . .. 1“ L0 _ . a fig)... .’}3§~2§¥)t n 0 v a. l n . .6. .% A.0.0vOUNv MO 9 a {31%} .. w 3 v A n D :. Aoo.0v OU" A. u v . o W . ll.)t(.(/I..7.I7\I\IJ r)?§.£re\a 1 W .1 «M II . .. 1 a 000— I 0 H .. O. . >oZmn.ou .. 1 Tod. cu? . . . a. ubplphbl. hpbb>b> DP78rrb7>bbt77FP*bbrh!>)¥ .xcsum ucomoum .oo.o .4 ago how euuoodm zwuocm .~.m ouswam ~>013 2003.3”: U n: 0: n9 8. mm 1 d d o 9 O (MW-AS/QW) 39 {SP/039 9 .oo . 93s >22 3.1m 02:.38 . 18 aoov .3353 89 u (d) The analog of the 10.3 MeV M1 state in 8Ca is seen clearly . 4 . . in 8Sc at Bx . 16.8 MeV; this seems to be the only strong resonance in the range of excitation observed. APPENDICES APPENDIX A Derivation of nonenergy weighted sum rule of isovector (T-l) spin flip and non-spin flip Operators APPENDIX A Derivation of non-energy weighted sum rule of isovector (T=l) spin flip and non-spin flip Operators: Consider H57? 6 = t Fermi (non-spin flip) w k 0 = 2 0 t5 Gamow Teller (spin flip) k - The sum 2 is over the nucleons in the nucleus. Define S(B_-B+)= 21|2 f éll2 A * A X f A * A - Z f z f - Z f A + A ' , - It can be shown that for both Fermi and GT operations, + _ 7 _ 0_ - 0+ and 0+ — 0_ 9O Then, S(B_ - 8+) = <110+0 - 0-0+ll> = <1!EO+IO Jll> For Fermi, [0+,0_]= 2 [tftf J k,k' SB--SB+=<1[ E Skk' 2t§l1> k,k' =2 2 t}; k -2 l - “2" (N‘Z) =N-Z k k' For GT, [0+,0 ]- E'Eokt+,0k,t_ ] 11> APPENDIX B SPECTRA (EFFICIENCY CORRECTED AND ENERGY CALIBRATED) 92 A >23 zomszm omovic.avoooe 1 m... o... 8. 8. mm .. 1.5.82.6 m3 1 .6. 00.0 .1. Q . >6§m.m__nam 3 vNN-mm-3m_2 l0. (Aaw-JS/QUJ ) 39 1513/5320 Ail. $2): zomszm 1 m: 0.. mo. 8. no >63: xm. . . . 1 11111111141113.4330, A o . o. o 1 1_ 6mm .. m 6.1. . a m >22 m m: . m 4m ... emote 38? ..me 1.4.15.1 81.13.44 31.4 i 312* «1914 s. . .3. .14.“? 4 4 O 1 M q 1. W 60:. m w >62 mm. _ ”am -N1 Memos? 388 m mNN-mm-Dm2 94 A>®§v ZOEPDUZ w m: 0: mo. 00. mm 13.2 M. 1.. . .... ( 7265;531:1771}; 00.0 n ® >62 mm: ”am ,. ommvEéoomv LO 0 9 0 (MW 48/91“) 312 UP / 029 O N LO N NNN1mm5m2 95 A>m_>: ZOthwZ .1”. ...—L MNNAmmimS. m: 0: mo. Om: mam 56.99-36 “4,49... 6. . 6 1 f a .... pa 2 6mm . m 6m - >22 mm: Ham -mm Ummicéoome -mml. 4 _ at; 1w .. >635 cram 54m ommv c a GUNs mm 96 A>m<$ ZOthwa m. o: 8. 00. mm o 32>.va o. , ow o .111 J 2 q q q . .m 6. O0.0u© >62 mm. _ .am 1 ”$vach 0034 -m. ONN-mm-:m§ (Aaw-JS/qwmp “(SP/020 97 m: 0.. mo. 00. mm 4 . _ q q q .. 1%. $23.; 0. 8 o r 1N om.®u® .. >o_>_m.m: new ..0 M2 82.? s 8:. w. . -mU p . 1 a a 0...)”. w 0. v - . .2721 -Nw 2.20976”. 1 - omit? 883. .8 .NNumm -sz 98 A>m§v ZOGPDUZW 1 m... 04: mm: Om: mm 0 .222qu Os. - 2 ON 1 5. OOWOHQ - >22 3.. "am . 532.3003 10 0 Q '20.. (AGW-JS/QUJ) 313 09/sz m.N1mm-Dm.2 99 2262282822 6.: o: no_ 00. mm 026.21% _ o_ 2 2 cm 2 d d 12: .2 . $8.2 . 2 >22 mm: "am om .:.d.ou x m.» me o 322. m o. 8 . 3 q s . 6:72 1 >22 Om: . am m.N1mm-Dm$_ ‘0. N O. 87 O (Aaw.1$/qw) 3909/0213 ‘0. N 0. L0 APPENDIX C MONTE CARLO CALCULATIONS OF NEUTRON DETECTOR EFFICIENCIES (RELATIVE) At each energy 32000 neutrons are incident on the detector. The tabulated numbers are the percentage of neutrons detected at a given bias. The bias is expressed in MeV of electron energy. The first row contains results for biases of 0 to 9 MeV, the second row results for biases of 10 to 19 MeV, etc. 100 mama.a m«s«.n omm=.m «:64.» “mag.” mama.~ zaaa.e moeu.a Nana.a 2222.: «229.2 “222.2 om~n.o mmdq.a 2:24.: w:2~.m .efin.a e~2=.= «022.2. nadn.u suma.u «-a.a on~a.a omwa.n 2522.. mama.» .Nnn.u c n:na.a nonu.. «um=.a m«:=.u. n::a.a sesame Nays.a mama.m amm~.e mmms.n. moms.a ance.: 3262.2. uses... ooma.n mum‘.n mzaq.a :Nmn.s aena.n .snma.m.. omoa.o noos.. 2292.; mama... 6824.: ooma.s m~=2.u mm22.m ~a=2.a mw«..a 9. om««.n naad.a oa~«.a. o=~«.a -~«.a osm~.s ann4.~ msn2.e woma.m an22.a.r no:«.a 2222.. m2m«.a ~mm«.a ~om~.a a~od.a “maq.m «mon.m N-2.a shud.mon s«o«.a. mmo«.a 8222.9 n:o«.u. smm«.. una~.u a»sm.~ ~n2~.m am2~.a o-~.e p --.a o~n~.. a~n~.a. n~:~.a. nu:~.a enm~.a acnu.a nno~.s m¢o~.a n~2~.a s ~m-.a Nze~.. omo~.u. smm~.a wean.» hoaa.a .soqn.n mama." ennn.m owsm.e . w r . .a .... ... ..., m . 6 % .m<.mee¢2~ a. mazgammmmsu z_m awe—u 2.22 >m: nau.«. 229.: 2.2 >mx «92.2 ".m.m mzo.>uzm_o_duu 2(22.>2. “use” embomhm: mzoehzuz ma 222222 -422— :aaeano2~ emmzuz gem» pma- >3: 0: .... 25:39. 32:2. :82: .2. um:n.e 2.. 1426.4 «max—mas zo__uum_o mmzuz_ .a.s a.a 6.9 u~.>.x c< pzmo_oz_ >6: oo.~”.oo.o~2 >mbmcm to 6:620:62 ooomm 101 mama.” mnuq.a «flu... nmaa.s m:na.s amas.s ~51... :m.u.a un.a.m udaa.a ...... wmda.n “ram.a ghsga.a omda.s hofia.s m~d=.a ma...a Noda.o mn...= amwn.n Jana.m .qu.o mowe.s. «ow‘.m nana.a am...“ o:om.u :an.= ...... mfizn.n “33a.“ us:a.ao¢ ma:s.a mwma.n mmmm.a «oflm.= gang.» uneu.s. do...» omen.» hd~§.n .umn.saa ohms.“ \mmsg.a anps.a mm...a ~mna.n -wn.e. rm»... maau.m mm...” mmad.sov mma«.n adfiq.a «:d«.m as...a n-d.a mNNH.~ doufl.m :mma.n .mmn..m "mmd.ae. mama.» o~:4.n mesa.» nunq.s onn«.a mm“... “mo... moa«.n «amd.a ~=~«.man Ho~«.a o~o«.a guod.s mm...~ mo...n oaa~.m moa~.a m..m.m wm«~.s mamu.ao¢ a=-.n nmm~.a ~mnm.a. mm:~.a km:~.n ~«mm.~ -n«.a ”Non.“ m~o~.w aw“..o.. aon~.a m~m~.a :mm~.s‘ mna~.a .m.~.m «can.» we...» m:~n.s .mnq.m ad“... mu m. A. m. .m b. m .N . o om<~m omwu ch mitommmmmau z—m hmm_u mhuz >w= mason. Ibo—z z—m >m: «macs nowox m1¢~>uzw~o~uuw 44mwmb4~ ombuwpwo mzamhauz no ummzzz 4qx ~< FZuQ—uz~ u~:n.. a.. ..a... muzuz_ 5.9 a.. «.5 >02 22 3.2: :35 t 283.2 83 102 .mmuao9 omuo.s unsuoa. Nmoooa. smudge umnaoa cumuoa mmwmon. :so~.n m mat... na~a.9 omamon masses :nadoa osm«.a. mnuaou «nnw.a mowmoa & ' mason? muanoa mums-a omsugu «mhmos Nosuoa muzdoa nwouon omnmou. m~m~.. m masses «Nance unwaoa «awaou Nana... cos... 53:..u mum... osw~.a ama~.a d >mz aaaodq thou; >mz oo.~ s~na.u onsa.m ma.a.n cnfim.a. msfio.a. 3m...» «mma.a nu~n.a hmwa.c c~mn.a ozns.u. m~na.u ~«ma.o mama... -na.a n.«.n :sdd.a a.~q.s mc:«.u «mm... son«.e ~nm..a hmm«.. .:m~.. nw:~.a mda~.n .Nnm.s “nan.a. oufin.u mNan.~ my .9 . z_m >mz ~.~.. o«:a« a~:non mmzoz~ non Newman News.» amnuoc sewage nwmnow mnwuom cannon wmuwos snowes «amass \H ow<~m ozaN a. mazcmmwmmco aowmnonomu asnnom uuuwom banana snosos onwaon ummdoo oaodca. mzuwam nmowos finance 1* mwam. smawe «mm». or mmus.=.a an...” 3.. oh m." .....n 3:05 cmowoslw wumcm mo mcouuamz OOONM mumzqmou za_pou¢_a u->~x b< ~2u:_uz_ 103 was... was... swan.a.. .33..... can»... mnau.a. «was... «a...m «Nd... ”ma... ma...” mm...” mmdn.u 3 enac.u mca~.uaumo«a.u. oswn.a imam... anmn.u imam... ~m~n.a no~a.u dunmwwwv smna.a_ mana.a nun..a :c:n.a Kn:».s moza.o. maau.a anmn.n:ixmmaqfizaquu.u.J ofioa.a.\nmo~.u ~mma.u unna.a no...u coma... an...» moan.n “an... unwa.mpv muma.u msu«.u use... onsa.u ofiad.s «ma... .mdu.c w«~«.m omw..u =mu..... o~n..u. «and... ~a:«.o sn:..a_ “5:..a =.m«.s, mam... own... “noq.a «mm..m.. “Nu... as“... o~o«.. “sad... m~m..n «a...» ~n.~.u scam.” on.~.n mo.~.~.a om-.n. n.n~.a mon~.u. .~.~.a. mn.~.a mnm~.. .~.m~.m “mom.” ...~.n was“...: ano~.n mmo~.a. czm~.a mann.a moun.u ...».s ss~n.n :Nnn.. wag».a anom.~ kw .m An ”w m. .¢ .m .N _ o .m<~m ommN oh mazommwmmoo zum hmmuu who: >m: aau.«q zhouz zum >w: Nos-s nomom mZOq»ozu~ouuum 4amwmpzu cmhomhwc mzomhamz as mumanz ...oh ooeasmu~m mwmzaz a... hw.4 owned .. za~__m°¢ 4._p~z~ zoaz0: oo.Nnfloo.moa xwumcm mo maouuamz coomm ll. 104 , ...... ......m ...... ...... 52.... ...... ...... ...... .....~.M ........ ...... M2.... ”...... ....... ....... ...... ...... ...... 2......» ...... ”mm... .-m... ..N... ......_ «2.... ~50... ...... ...... w....... ~.m.... 2...... m...... 2..... ...... «...... 2..... ...... ...... ......pm mm..... ...... ...... ...... «...... .....q. ...... ...... 2..... new..... n2..... «...... ......_ ...... ..2.... ..2... “.2... ...... ...... ........ 2...... N...... .m..... 2...... ...... ...... 2..... m..... ...... ......Qa ...... «mm... ...... ...... ~27... =.m~.. ...... .2.~.. ...... ......o. ...... ...N... ~2.~... ...... ...... ...... m2.... «2.... .22... ...... o 2.0 o W .w n v x. -... . , ... ...—m o..~ .. mozcmmumaco z_. .m2_u ...: >mz ...... 2...: 2.. >mz «.... ".... wzo.».2u_u.... 4....»2_ aw... .u_om_uo “2.2.3.: .. mmmzzz 4.... ......mu2 .umznz a... p.22 .. z._b_m.. 4....z~ :c.z<. .. ..2... ... ..2... .uc.z_m.o z.__u_2_o mmzoz. ... .... ... u~.».x .2 pzaohoz. >mz o... .oo.oo. ...mcm .o acouuamz co... 105 .5..... .2..... «.5..9 .2..... sundae omu~09 soomou m. nunaon madman Nuns-a. no~599 «madam Naouoa NN-ca «com... Aw nw.aunr:~nnnuptlmmnfiwpl:55..ma. . .....9 ..2.... ...p.. ...... :oo«.u. «ammoa nzanoa P mn-ou mmsaoa sumac: acmqoa nnmdou aonwoa 2..... w >m= can... rhea: 22...n. ...... no2... ...... ...... ...... 5..... .5»... 5.5.... ...... ..2.... ...... ...... ....... .m .2 2.. >w:.m.... ..... ..2... ..292. ... III-.-- nmwaoa .szsoa .5.... 2.2... ...... ...... ...... m nmmnpstm..mu. "l'. ...... .5.... ...... 5.2... n5.... 5..... .52... .N snun-aun .2.... ...... ...... ...... .aamaom anamoc nnmwom «@wnon ..<.. .... .. ..2...w.2.. 2.. ...—u u.... .2..».7._...u. ..2...2. ......Qfi mwmn.202 okvnncn 5...... .2..... 29mm... 5...... ...... Am ...r Qw—ombw: mzompzm: no mwmznz JuhOh xwmzsz owwu wm<» 2. 2....mog .....2. coez<2 .. new asau.a ‘09. >02 oo.Nnfloo.om hwumcm «0 mcouuamz ooon umuz—moo zonpUmc—o u~.».x ~< hzwo_oz~ 106 .uaaa on. unmcou. onsaou «Nmaoa «msdog a:a~.9 summon m. nmmnom “035.3 numaoa camaca swa~ou omm~oa. m ‘Il‘ll l I mega... ...... ...... snadoa. ommaou aou~oa nmanon. x. >m: can... than: 2—3 u...‘t. 4 mmuaon u .... ....II‘oIIII'O'O(I‘|.Oll-I|"O 5...... ...... 2...... ...... ...... 2..... ......9. 5...... ...... ...... 2mm... ...... ...... ..2.... 5...... ~...... ....... ...... ...... ...... 5...... ....... 2..... n...... ...... ...... ...... ..2.... ....... 2...... ...... .55... ...... ...... 25..... ...... .2.... -.~.. 5..... ...... 2..... ~...... 2..... ..mw... .3 ... ....... ...... ...... ...... ”w m N _ o om<~m ommN ab maxemmwmmco z~m hmm—u who: >m; Nan-u nowom mchpuzmuouuuu aoz o... ...... ...... .0 .ao..=m2 co... 107 >3: ow mean-a manaos. come-9 m3Nch. shadow. «Names. 0 amen-a cannon. «303.9 ndnuoa «mow-n finance. v smo‘.o n..... ..5... 35.... ozawoa ma.... n «mange noosoa mousoa 933.9: mnam-s. newnoa g >uz ana.«q Iho~z ~n...u ...... .aN... «~59.» mm-.a ”...... may... ”ms... .31.}. cos... ~m:..s 5.. .m . mmms.a Nam... 55.... m:a..a ms...» m5...w.. 5am... mom... ~no..s 5a...» om5... 5e»..... ~2~N.a n=n~.u 5:35.. som~.s e5.~.a ”.5... a on»... :m:n... :non.a .05... .nmn.a 3....u ; m 5 m 5 . . .m<.n omm5.o. mazoamwmmoo z.m .mm.u ...z 2.9 >m; «a... u.w.m mzo.».z..o_mmu uo= oo.~u.oc.o5 .wumcu mo acouuamz oocmm 108 nausea worsen omoaon 3.5.... .3QN... m. 3 ngnom mama-a mnmaou mama's. wammoa m uddaao mama-o. ouaaou. omodou «mane? m. >mz mam... Ibo—1 ow~3.3 3333...} mo...3 o.~a.u . «an... on»... N33... 5.33.3.3 .5m3.u. .3ma.a..3.m..3. n33... ...... «n5... .a5n.z§ 5a.... au~..3 53w... 3cm... 333... 33m... um...woa 3.3.... nm3~.3. 3m.~.a 35u~.m 33n~.3 w~m~.. 3535.30, ...... 3333.3 5mon.s 3.33.. 333... 03.3.3 ...... w kw .¢ m N _ o .m<_m 33m. 3. mazcummamou 2.3 .mc_u ...: z_m 3m; m3... u.m.3 wzo.»uz._u_uuu ..33..2~ .N3NN a...u.w3 mzomp3mz m3 .mmzzz -.... 33335.33. amnzgz 9.”. .... 3. :3_..mom 4._5_.. =aoz__mz.n wooo :uz mahowhmo 23mp3w2 Nafiumz to sea >0 tom“ bm town 3: o~zo mom ww—ozu~u_umm . Ae.n->.x.53 ooo.o he ooo.o3 .3 game o.3.m .Ammzucmv macamcmafia saw: HOumfidauaaum.umH:mcmuumm 109 0.2 MSU-83- 58! 0J5? OJOh' EFFICIENCY (RELATIVE) 0.05 - 0.0 IOO 80 60 ENEUTRON (MW) IZO Figure C.l. Relative detector efficiency versus neutron energy. Threshold energies shown are electron energies. APPENDIX D CALCULATION OF GT STRENGTH APPENDIX D CALCULATION OF THE GT STRENGTH Following the method prescribed by Taddeucci et al., and described in Chapter I (Ta 81), define do (E )(0°) K __ v; GT X l _ l r, F B(GT) ~E 1.1+ dQ Xdc51,.(O°Yx(N 2” T27 fuq) XW x T R2(Ep=120 MeV) =4.71 i=(E /E )l°5 KGT Neutron,F Neutron,GT The sum is over all l+ excitations, as obtained from the measured angular distributions. f(Aq) Ea.momentum transfer correction factor. To compute f(Aq), calculate momentum transfers for all 1+ excitations of interest at 0° and for the IAS for e:=o to 10°; estimate 6' for the IAS that has the same momentum transfer (Ag) as the excitation of interest at 0°; then 0 50 do , afi- IAS(9 ) f(Aq) = For the sake of uniformity, we obtained angular distribution for IAS by averaging over those for “2'““ and “88c. This Curve,displayed on the top of Figure 3.9,was used in extrac- ting 9'. 110 111 The computations are listed in Tables 0.1, D.2 and 0.3 for “2'““ and “8Ca for 1+ cross sections obtained from defining an experimenter's background similar to those shown in Figure 3.8. The l+ strengths derived by fitting our data (peak + background) to predictions of DWBA cross sections were also used to obtain GT strengths; this method was an applied to and “BCa only. The computations are shown 5 in Tables 0.4 and D.5. 112 rail. 14“.. . .wo.mm n cofiqupmHQ was. Eon mo w Km .3.3.3 u .xmceom N .33.3 .33.. m~.3 33... .5~.3H533.m 3~.3. .m..3 333.. 33.3 333.. 333.3H353.3 N..3 353.3 333.. 33.~ 333.. 3...3H333.. 33.3 333.3 33... 33.. 333.. 33..3H~35.. 33.. 333.3 333.. 53.3 333.. m.3.3H~3m.3. .3.3 m3. .. u- 333.. ‘ .5..3H333.. 33.3 x . 3 . 3 ...533. x 3.333 .3333 ol.3. .33 u 353 3 33 .03333533 r>mzc 3 .ou~3 new Accsouoxomn m.uou:meflummxo 23.3. numcmuum so .330. no co.umusdsoo H.Q manna numcmugm 3.53 2:3 mo 3 X .xmv eom 113 333.3 3..3 33... 33..3+333.3 33.3. 333.3 33.3 33... 333.33333.~ 33.3 333.3 33.3 333.. 33..3HN33.. .3.3 333.. 33.. 333.. 333.33333.3 33.3 3.3.3 33.. 3.3.. 333.33333.3 33.3 333.3 33.3 333.. 333.33.33.3 3..3 33. u 333.. 333.33333.3 33.3 333.3 3 333.3 333.333-.3 33.3 EU . .Aum\nzv 33 3 03.33 .eu.uzm\3.uzm3 A03vccxon A>mzvxm 6033 qu Avcsoumxomm m..0u:mfiaummxm £3.33 23333333 so .3303 no :0333353500 N.Q OHQMB 114 X 3.3.3. u .33. 333 w .3... 33.. 3..3 33... 333.33333.3 3.3. 333.3 33.. 33.3 .33.. 333.33333.33 33... 333.. .... 33.. 3.3.. 333.33333.3 33.3 33. u u 333.. 333.33333.3 33.3 333.3 3.. 333.3 .33.3 333.33333.3 33.3 333.3 3.. 333.3 333.3 33..3H333.. 3..3 333.. 3.. 333.3 333.3 333.3333..3 33.3 333.3 3.. 333.3 333.3 333.333.3.3 33.3 , Aum\nE. 333.333 .33.3 o..3. 3...ao.uzm\3.uzm. .03.33\33 A>mz.xm .3033 30w Accsoumxomm m.umu:meflummxm 23.3. numcmuum so .muou 30 :0333333200 3.3 3.333 115 mm.33 n numcmuum m.sm 59m mo 3 x x 90 m 003.3 a A m. m w 333.. 033.. 0~.3 mm... mm3.m 0.3. mom.. 033.. 03.m .m... mmm.3 0... 333.. 0.3.. 00.m 030.. 033.3 0.3 333.0 033.. 03.3 mm0.. 330.3 0.3 333.. 03... 0m.. 0m0.. mmm.3 0.3 ~.m.. 0.0.. m..0 300.. 333.0 0.m 330.. 00.. 00.0 333.0 .03.3 0.. . .33\32. s 333.33 .33.3 03.3. 3.3.33 uz3\3 323 3.3.33\33. A>3z.x3 .mumc mo m.m>.m:m «man 5033 nm>33mn mnumcmuum +. su33. 3033 new cumcwuum Bo .muou mo :03umusmfiou 3.0 mHQma 116 00.00 H numcmuum $.50 530 00 w x x 90 m 3.0.03 n A m. 00 m00.m 030.. 30.3 00... 3.0.0 0.0. 030.. 030.. «0.0 mm... 000.0 0.0. N0m.~ 0.3.. No.0 .00.. 0.0.0 0.0. 0.0.0 0mm.. mm.~ .00.. 003.0. 0... 303.~ 00... 30.. ~00.. 030... 0.0 000.0 000.. 00.0 330.. 000.0 0.3 000.0 000.. 00.0 000.0 .0..m 0.0 03... 000.. 00.0 000.0 303.0 0.0 N00. 000.. 00.0 000.0 003.0 0.. ..m\ne. v.3. 3.33 . .33. 3 o. . 3. 3.. 13.3231. 333. .03. 33>... .332. 33 .mumo no m.m>.m:m 403a Eouw 60>.Hmv numcmuum +. 03.3. 30.. 30. 333:3333 33 .330. 30 30.33333203 m.Q 0.909 LIST OF REFERENCES An Ar Au Be Be Be Bo Ch Co Do Er Fu Ga. Ga. 79 80 83 79 72 81 82 81 80 74 75 82 80 80 81 LIST OF REFERENCES B.D. Anderson, R.A. Cecil, and R. Madey, The (p,n) reaction and the nucleon-nucleon force, ed. C.D. Goodman, S.M. Austin, D. Bloom, J. Rapaport, and G.R. Satchler, Plenum Press, New York, (1979). B.D. Anderson, J.N. Knudsen, P.C. Tandy, J.W. Watson, and R. Madey, Phys. Rev. Lett. 4;, 699 (1980). N. Anantaraman, private communication. S.M. Austin, The (p,n) reaction and the nucleon-nucleon force, ed. C.D. Goodman, S.M. Austin, D. Bloom, J. Rapaport, and G.R. Satchler, Plenum Press, New York, (1979). G.F. Bertsch and A. Mekjian, Ann. Rev. of Nucl. Sci. 22, 25 (1972). G.F. Bertsch, Nucl. Phys. é§§£2 157c (1981). G.F. Bertsch and I. Hamamoto, Phys. Rev. £26, 1323 (1982). A. Bohr and B. Mottelson, Phys. Lett. AQQB, 10 (1981). C.W. Cheng and J.D. King, Ap. J. Suppl. Series 42, 475 (1980). V. Comparat, R. Frascaria, N- Marby, M. Morlet, and A. Willis, Nucl. Phys. A221, 403 (1974). R.R. Doering, A. Galonsky, D.M. Patterson, and G.F. Bertsch, Phys. Rev. Lett. 82, 1691 (1975). M. Ericson, Invited talk at the Intl. Conf. on Spin Excitations in Nuclei, Telluride, Colorado, 1982 to be published. G.M. Fuller, W.A. Fowler, and M.J. Newman, Ap. J. Suppl. Series 42, 447 (1980). C. Gaarde, J.S. Larsen, M.N. Harekh, S.Y. Van Der Werf, M. Igarashi, and A. Muller-Arnke, Nucl. Phys. A334, 248 (1980). C. Gaarde, J. Rapaport, T.N. Taddeucci, C.D. Goodman, C.C. Foster, D.E. Bainum, C.A. Goulding, M.B. Greenfield, D.J. Horen, and E. Sugarbaker, Nucl. Phys. A369, 258 (1981). 117 Ga G1 Go Go Go Go Go Go Gs Ik Lo Mo 0f 0k Os Se: 82 79 78a 78b 79 80 81 82 83 63 78 82 82 58 79 81 82 118 C. Gaarde, J.S. Larsen, and J. Rapaport, Intl. Conf. on Spin Excitations in Nuclei, Telluride, Colorado, 1982.* C.A. Goulding, The (p,n) reaction and the nucleon-nucleon force, ed. C.D. Goodman, S.M. Austin, D. Bloom, J. Rapaport, and G.R. Satchler, Plenum Press, New York, (1979). C.D. Goodman, J. Rapaport, D.E. Bainum, M.B. Greenfield, and C.A. Goulding, IEE Transactions on Nuclear Science, NS-ZS, S77 (1978). C.D. Goodman, J. Rapaport, D.E. Bainum, and C.E. Brient, N.I.M., 151, 125 (1978). C.D. Goodman, C.C. Foster, M.B. Greenfield, C.A. Goulding, D.A. Lind, and J. Rapaport, IEEE Transactions on Nuclear Science, NS—26, 2248 (1979). C.D. Goodman, C.A. Goulding, M.B. Greenfield, J. Rapaport, D.E. Bainum, C.C. Foster, W.G. Love, and F. Petrovich, Phys. Rev. Lett. 44, 1755 (1980). C.D. Goodman, C.C. Foster, D.E. Bainum, S.D. Bloom, C. Gaarde, J. Larsen, C.A. Goulding, D.J. HOren, T. Masterson, S. Grimes, J. Rapaport, T.N. Taddeucci, and E. Sugarbaker, Phys. Lett. 107B, 406 (1981). C.D. Goodman, Intl. Conf. on Spin Excitations in Nuclei, Tellu- ride, Colorado, 1982. to be published. A. Galonsky, private communication. K. Ikeda, S. Fujii, and J.I. Fujita, Phys. Lett. 3, 271 (1963). W.G. Love, A. Scott, F. Todd Baker, W.P. Jones, and J.D. Wiggins, Phys. Lett. 73B, 277 (1978). C.L. Morris, Intl. Conf. on Spin Excitations in Nuclei, Tellu— ride, Colorado, 1982, to be published. F. Osterfeld, Phys. Rev. Egg, 762 (1982). S. Okubo and R.R. Marshak, Ann. Phys. 4, 166 (1958). E. Oset and M. Rho, Phys. Rev. Lett., 42, 47 (1979). J. Rapaport, T.N. Taddeucci, C. Gaarde, C.D. Goodman, C.C. Foster, C.A. Goulding, D. Horen, E. Sugarbaker, T. Masterson, and D. Lind, Phys. Rev. C24, 335 (1981). H. Sagawa, Invited talk at the 5th Kyoto Summer Institute on Microsopic Theories of Nuclear Collective Motions (1982). St 80 Ta 81 Ta 82 TR 73 Ni 76 119 W. Steffen, B.D. Graf,W. Gross, D. Meuer, A. Richter, E. Spamer, 0. Titze, and W. Knfipfer, Phys. Lett. 95B, 23 (1980). T.N. Taddeucci, J. Rapaport, D.E. Bainum, C.D. Goodman, C.C. Foster, C. Gaarde, J. Larsen, C.A. Goulding, D.J. Horen, T. Masterson, and E. Sugarbaker, Phys. Rev. C25, 1094 (1981). T.N. Taddeucci, private communication. K. Takahashi, M. Yamada, and T. Kondoh, Atomic Data and Nuclear Data Tables, 12, 101 (1973). J.G. Wilson, in Cosmic Rays, Wykeham Publications (London) Ltd., 32, 53 (1976).